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We present a new physical model resolving a long-standing mystery of the power-law distributions of the blinking times in single colloidal quantum dot fluorescence. The model considers the non-radiative relaxation of the exciton through…

Statistical Mechanics · Physics 2009-11-16 Pavel A. Frantsuzov , Sandor Volkan-Kacso , Bolizsar Janko

Fluctuations in the fluorescence from macroscopic ensembles of colloidal semiconductor quantum dots have the spectral form of 1/f noise. The measured power spectral density reflects the fluorescence intermittency of individual dots with…

Materials Science · Physics 2009-11-10 Matthew Pelton , David Grier , Philippe Guyot-Sionnest

The power spectrum of quantum dot fluorescence exhibits $1/f^\beta$ noise, related to the intermittency of these nanosystems. As in other systems exhibiting $1/f$ noise, this power spectrum is not integrable at low frequencies, which…

Statistical Mechanics · Physics 2015-06-18 Sanaz Sadegh , Eli Barkai , Diego Krapf

Photo-luminescence intermittency (blinking) in semiconductor nanocrystals (NCs), a phenomenon ubiquitous to single-emitters, is generally considered to be temporally random intensity fluctuations between bright (On) and dark (Off) states.…

Mesoscale and Nanoscale Physics · Physics 2020-01-29 Amitrajit Mukherjee , Korak Kumar Ray , Chinmay Phadnis , Arunasish Layek , Soumya Bera , Arindam Chowdhury

We report the observation of power law dynamics on nanosecond to microsecond time scales in the fluorescence decay from semiconductor nanocrystals, and draw a comparison between this behavior and power-law fluorescence blinking from single…

Other Condensed Matter · Physics 2008-01-27 P. H. Sher , J. M. Smith , P. A. Dalgarno , R. J. Warburton , X. Chen , P. J. Dobson , S. M. Daniels , N. L. Pickett , P. O'Brien

Abrupt fluorescence intermittency or blinking is long recognized to be characteristic of single nano-emitters. Extended quantum-confined nanostructures also undergo spatially heterogeneous blinking, however, there is no such precedence in…

Mesoscale and Nanoscale Physics · Physics 2018-08-27 Nithin Pathoor , Ansuman Halder , Amitrajit Mukherjee , Jaladhar Mahato , Shaibal K. Sarkar , Arindam Chowdhury

Recent experiments on blinking quantum dots and weak turbulence in liquid crystals reveal the fundamental connection between $1/f$ noise and power law intermittency. The non-stationarity of the process implies that the power spectrum is…

Statistical Mechanics · Physics 2015-06-11 Markus Niemann , Holger Kantz , Eli Barkai

The photoluminescence intermittency (blinking) of quantum dots is interesting because it is an easily-measured quantum process whose transition statistics cannot be explained by Fermi's Golden Rule. Commonly, the transition statistics are…

Mesoscale and Nanoscale Physics · Physics 2023-01-23 Roberto N. Munoz , Laszlo Frazer , Gangcheng Yuan , Paul Mulvaney , Felix A. Pollock , Kavan Modi

Intermittent photoluminescence of colloidal core/shell semiconductor nanocrystals of spherical and branched shape was studied under CW-laser excitation. Luminescent multichannel registration system was applied for the fluorescence detection…

Optics · Physics 2011-12-13 A. G. Vitukhnovsky , M. M. Kovalev , V. V. Lidsky , E. M. Khokhlov

The interpretation of the electronic kinetic processes in the quantum zero dimensional nanostructures is considered. The main mechanism of the processes is supposed to be the interaction of electrons with the optical phonons. An emphasis is…

Mesoscale and Nanoscale Physics · Physics 2012-01-05 K. Kral , M. Mensik

We study the spontaneous emission from a regular lateral array or a randomly distributed ensemble of quantum dots under strong excitation (full inversion) conditions. We focus on the similarities and differences between the cases of random…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 Wildan Abdussalam , Paweł Machnikowski

Colloidal semiconductor quantum dots (QDs) are excellent luminescent nanomaterials for a broad range of optoelectronic applications. Their photoluminescence blinking, however, hinders their practical use in many aspects. It has been shown…

Optics · Physics 2024-02-27 Zhiyuan Wang , Jianwei Tang , Jiahao Han , Juan Xia , Tianzi Ma , Xue-Wen Chen

We report quantum interference effects in InAs semiconductor nanowires strongly coupled to superconducting electrodes. In the normal state, universal conductance fluctuations are investigated as a function of magnetic field, temperature,…

Mesoscale and Nanoscale Physics · Physics 2020-11-04 Yong-Joo Doh , Aarnoud L. Roest , Erik P. A. M. Bakkers , Silvano De Franceschi , Leo P. Kouwenhoven

The surface of semiconductor nanostructures has a major impact on their electronic and optical properties. Disorder and defects in the surface layer typically cause degradation of charge carrier transport and radiative recombination…

In this work, we report a new nanoscale phenomenon observed as photoemission intermittency (On-Off electron emission), manifested as stochastic bursts in electron yield at quasi-one-dimensional organic wires and silver nanoparticles…

Materials Science · Physics 2026-05-22 Moha Naeimi , Waqas Pervez , Frithjof Harmsen , Ingo Barke , Sylvia Speller

The most abundant particles in the Universe are photons and neutrinos. Both types of particles are whirling around everywhere, since the early Universe. Hence the neutrinos are all around us, and permanently pass through our planet and our…

Popular Physics · Physics 2016-01-20 Alexis Aguilar-Arevalo , Wolfgang Bietenholz

Dielectric nanoparticles can be engineered to scatter light predominantly in the transverse direction, a phenomenon known as the transverse Kerker effect. Although complete cancelation of forward scattering from a single object is forbidden…

We examine cyclic phantom models for the universe, in which the universe is dominated sequentially by radiation, matter, and a phantom dark energy field, followed by a standard inflationary phase. Since this cycle repeats endlessly, the…

Cosmology and Nongalactic Astrophysics · Physics 2013-05-30 Hui-Yiing Chang , Robert J. Scherrer

We observe experimentally that ensembles of quantum dots in three-dimensional (3D) photonic crystals reveal strongly nonexponential time-resolved emission. These complex emission decay curves are analyzed with a continuous distribution of…

Systems containing few Fermions (e.g., electrons) are of great current interest. Fluorescence occurs when electrons drop from one level to another without changing spin. Only electron gases in a state of equilibrium are considered. When the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Arnaud , L. Chusseau , F. Philippe
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