English
Related papers

Related papers: Laser Induced Selective Alignment of Water Spin Is…

200 papers

Enrichment of nuclear spin isomers of molecules by infrared radiation resonant to molecular rovibrational transition is considered. Special attention is given to the enrichment by light-induced crossing of far separated ortho and para…

Chemical Physics · Physics 2007-05-23 Pavel Chapovsky

Laser-controlled entanglement between atomic qubits (`spins') and collective motion in trapped ion Coulomb crystals requires conditional momentum transfer from the laser. Since the spin-dependent force is derived from a spatial gradient in…

Atomic Physics · Physics 2021-12-06 Adam D West , Randall Putnam , Wesley C Campbell , Paul Hamilton

We theoretically consider the phenomenon of field-free long-lasting orientation of symmetric-top molecules ionized by two-color laser pulses. The anisotropic ionization produces a significant long-lasting orientation of the surviving…

Chemical Physics · Physics 2023-03-08 Long Xu , Ilia Tutunnikov , Yehiam Prior , Ilya Sh. Averbukh

The propensity of molecules to spatially align along the polarization vector of intense, pulsed light fields is related to readily-accessible parameters (molecular polarizabilities, moment of inertia, peak intensity of the light and its…

Atomic Physics · Physics 2009-11-06 S. Banerjee , D. Mathur , G. Ravindra Kumar

Random lasers with low spatial coherence have important potential applications in high quality imaging and displaying. Here, a random laser with tunable angular spectra is proposed and fabricated through directly coupling an asymmetric…

Optics · Physics 2021-10-08 Huihui Shen , Yaoxing Bian , Junyan Li , Weinian Liu , Hanyi Xue , Zhaona Wang

Traditionally, atomic spin orientation is achieved by the transfer of angular momentum from polarised light to an atomic system. We demonstrate the mechanism of orientation generation in room-temperature caesium vapours that combines three…

Atomic Physics · Physics 2020-02-05 Patrick Bevington , Rafal Gartman , Witold Chalupczak

Dimers of carbon disulfide (CS$_2$) molecules embedded in helium nanodroplets are aligned using a moderately intense, 160ps, non-resonant, circularly polarized laser pulse. It is shown that the intermolecular carbon-carbon (C-C) axis aligns…

Chemical Physics · Physics 2019-04-10 James D. Pickering , Benjamin Shepperson , Lars Christiansen , Henrik Stapelfeldt

Introducing spin-polarized carriers in semiconductor lasers reveals an alternative path to realize room-temperature spintronic applications, beyond the usual magnetoresistive effects. Through carrier recombination, the angular momentum of…

We present and discuss a new computationally inexpensive method to study, within the single active electron approximation, the interaction of a complex system with an intense ultrashort laser pulse. As a first application, we consider the…

We show that circularly polarized femtosecond laser pulses produce field-free alignment in linear and planar molecules. We study the rotational wavepacket evolution of O$_2$ and benzene created by circularly polarized light. For benzene, we…

Chemical Physics · Physics 2014-06-06 C T L Smeenk , P B Corkum

Selective control of light is essential for optical science and technology with numerous applications. Nanophotonic waveguides and integrated couplers have been developed to achieve selective coupling and spatial control of an optical beam…

We show that multiple filamentation patterns in high-power laser beams, can be described by means of two statistical physics concepts, namely self-similarity of the patterns over two nested scales, and nearest-neighbor interactions of…

Statistical Mechanics · Physics 2015-05-27 Wahb Ettoumi , Jérôme Kasparian , Jean-Pierre Wolf

The interaction of a short, few-cycle light pulse and an atom which is prepared initially in a superposition of two stationary states is shown to exhibit strong signatures of atomic coherence. For a given waveform of the laser pulse,…

Atomic Physics · Physics 2017-01-04 Viktor Ayadi , Mihaly G. Benedict , Peter Dombi , Peter Foldi

We show that the physical system consisting of trapped ions interacting with lasers may undergo a rich variety of quantum phase transitions. By changing the laser intensities and polarizations the dynamics of the internal states of the ions…

Quantum Physics · Physics 2009-11-10 D. Porras , J. I. Cirac

Arrays of 10 nm-diameter point contacts of exchange-coupled spin-majority/spin-minority ferromagnetic metals, integrated into infrared-terahertz range photon resonators, are fabricated and measured electrically and optically. Giant,…

Mesoscale and Nanoscale Physics · Physics 2013-11-27 V. Korenivski , A. Iovan , A. Kadigrobov , R. I. Shekhter

We propose a mechanism to produce a superposition of atomic and molecular states by a train of ultrashort laser pulses combined with weak control fields. By adjusting the repetition rate of the pump pulses and the intensity of the coupling…

Atomic Physics · Physics 2014-11-18 Anahit Gogyan , Stephane Guerin , Yuri Malakyan

It is predicted that nuclear spin conversion in molecules can be efficiently controlled by strong laser radiation resonant to rovibrational molecular transition. The phenomenon can be used for substantial enrichment of spin isomers, or for…

Chemical Physics · Physics 2009-11-06 P. L. Chapovsky

The parallel or antiparallel arrangement of electron spins plays a pivotal role in determining the properties of a physical system. To meet the demands for innovative technological solutions, extensive efforts have been dedicated to…

The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…

Laser pulses are known to induce symmetric demagnetization: equal loss of magnetic moments in the identical sublattices of antiferromagnets and ferromagnets at ultrashort timescales. Using time-dependent density functional theory, we show…

Materials Science · Physics 2026-02-19 Zhaobo Zhou , Sangeeta Sharma , John Kay Dewhurst , Junjie He