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Related papers: Laser Induced Selective Alignment of Water Spin Is…

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Precise control of hyperfine matterwaves via Raman excitations is instrumental to a class of atom-based quantum technology. We investigate the Raman spinor control technique for alkaline atoms in an intermediate regime of single-photon…

Atomic Physics · Physics 2023-05-31 Liyang Qiu , Haidong Yuan , Saijun Wu

We demonstrate that the current laser technology used for field-free molecular alignment via a cascade of Raman rotational transitions allows for observing long-discussed non-linear quantum phenomena in the dynamics of the periodically…

Quantum Physics · Physics 2015-05-30 Johannes Floß , Ilya Sh. Averbukh

We demonstrate a hard x-ray probe of laser-aligned small molecules. To align small molecules with optical lasers, high intensities at nonresonant wavelengths are necessary. We use 95 ps pulses focused to 40 mum from an 800 nm Ti:sapphire…

We provide a detailed theoretical analysis of molecular rotational excitation by a chiral pulse train -- a sequence of linearly polarised pulses with the polarisation direction rotating from pulse to pulse by a controllable angle. Molecular…

Quantum Physics · Physics 2013-05-30 Johannes Floß , Ilya Sh. Averbukh

Spin-polarized particle beams are of interest for applications like deep-inelastic scattering, e.g. to gain further understanding of the proton's nuclear structure. With the advent of high-intensity laser facilities, laser-plasma-based…

Plasma Physics · Physics 2025-11-06 Lars Reichwein , Zheng Gong , Chuan Zheng , Liangliang Ji , Alexander Pukhov , Markus Büscher

Half-cycle laser pulse is applied on an absorbed molecule to investigate its alignment and orientation behavior. Crossover from field-free to hindered rotation motion is observed by varying the angel of hindrance of potential well. At small…

Atomic Physics · Physics 2007-05-23 Y. Y. Liao , Y. N. Chen , D. S. Chuu

Chiral molecules with broken parity symmetries can be modeled as quantum systems with cyclic-transition structures. By using these novel properties, we design two-step laser pulses to distinguish left- and right-handed molecules from the…

Quantum Physics · Physics 2015-05-19 W. Z. Jia , L. F. Wei

Coherent control of chaotic molecular systems, using laser-assisted alignment of sulphur dioxide (SO$_2$) molecules in the presence of a static electric field as an example, is considered. Conditions for which the classical version of this…

Chemical Physics · Physics 2017-04-26 Johannes Floß , Paul Brumer

Controlling the directionality of spin waves is a key ingredient in wave-based computing methods such as magnonics. In this paper, we demonstrate this particular aspect by using an all-optical point-like source of continuous spin waves…

Mesoscale and Nanoscale Physics · Physics 2021-01-27 S. Muralidhar , R. Khymyn , A. A. Awad , A. Alemán , D. Hanstorp , J. Åkerman , .

We provide an analytic study of the dynamics of semiconductor lasers with injection (pump) of spin-polarized electrons, previously considered in the steady-state regime. Using complementary approaches of quasi-static and small signal…

Materials Science · Physics 2015-05-18 Jeongsu Lee , William Falls , Rafal Oszwaldowski , Igor Zutic

Most laser-induced femtosecond magnetism investigations are done in magnetic thin films. Nanostructured magnetic dots, with their reduced dimensionality, present new opportunities for spin manipulation. Here we predict that if a magnetic…

Materials Science · Physics 2015-05-27 G. P. Zhang , M. S. Si , T. F. George

We use an optical centrifuge to align asymmetric top $\mathrm{SO_2}$ molecules by adiabatically spinning their most polarizable O-O axis. The effective centrifugal potential in the rotating frame confines sulfur atoms to the plane of the…

Chemical Physics · Physics 2016-05-11 A. Korobenko , V. Milner

We have experimentally and theoretically investigated the mixed-field orientation of rotational-state-selected OCS molecules and we achieve strong degrees of alignment and orientation. The applied moderately intense nanosecond laser pulses…

CS$_2$ is identified as a molecule for which distinction can be made between dynamic and geometric alignment induced by intense laser fields. Measured anisotropic angular distributions of fragment ions arise from (i) dynamic alignment of…

Atomic Physics · Physics 2009-10-31 S. Banerjee , G. R. Kumar , D. Mathur

The optical pump-probe technique is a common tool for investigation of ultrafast spin dynamics, which usually utilizes single-diode detection averaging the dynamics over the pumped area. Using ultrafast imaging technique, we show…

Applied Physics · Physics 2025-07-15 T. T. Gareev , N. E. Khokhlov , L. Körber , A. V. Kimel

We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecular interaction with either a pair of pulses (a "double kick"…

Optics · Physics 2015-06-11 C. Bloomquist , S. Zhdanovich , A. A. Milner , V. Milner

Para- and ortho- isomers of water have different chemical and physical properties. Excitations by magnetic field, laser emission or hydrodynamic cavitation are reported to change energetic levels and spin configurations of water molecules…

Chemical Physics · Physics 2022-05-18 Serge Kernbach

We present a comprehensive study of enantioselective orientation of chiral molecules excited by a pair of delayed cross-polarized femtosecond laser pulses. We show that by optimizing the pulses' parameters, a significant (~ 10%) degree of…

Optics · Physics 2022-07-20 Long Xu , Ilia Tutunnikov , Yehiam Prior , Ilya Sh. Averbukh

Spin-orbit coupling (SOC) can give rise to interesting physics, from spin Hall to topological insulators, normally in condensed matter systems. Recently, this topical area has extended into atomic quantum gases in searching for…

Quantum Gases · Physics 2012-04-11 Z. F. Xu , L. You

Formation of laser-induced periodic surface structures (LIPSS or ripples) was studied on a metallic surface of polished copper by using irradiation with multiple femtosecond laser pulses in different environmental conditions (air, water,…

Pattern Formation and Solitons · Physics 2018-08-16 Stella Maragkaki , Abdallah Elkalash , Evgeny L. Gurevich