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Muon spin relaxation experiments have been performed in the pyrochlore iridate Pr_2Ir_2O_7 for temperatures in the range 0.025-250 K. Kubo-Toyabe relaxation functions are observed up to > 200 K, indicating static magnetism over this…

Strongly Correlated Electrons · Physics 2009-11-13 D. E. MacLaughlin , Y. Ohta , Y. Machida , S. Nakatsuji , G. M. Luke , K. Ishida , R. H. Heffner , Lei Shu , O. O. Bernal

We report the a.c. susceptibility study of Dy_xTb_{2-x}Ti_2O_7 with x in [0, 2]. In addition to the single-ion effect at Ts (single-ion effect peak temperature) corresponding to the Dy3+ spins as that in spin ice Dy_2Ti_2O_7 and a possible…

Materials Science · Physics 2015-03-13 Hui Xing , Mi He , Chunmu Feng , Hanjie Guo , Hao Zeng , Zhu-An Xu

Magnetic properties of a one-dimensional frustrated quantum spin system Rb2Cu2Mo3O12 is investigated by the muon spin relaxation (muSR) technique. Although this system shows an incommensurate spin correlation in neutron scattering, it has…

Strongly Correlated Electrons · Physics 2018-04-04 Seiko Ohira-Kawamura , Keisuke Tomiyasu , Akihiro Koda , Dita P. Sari , Retno Asih , Sungwon Yoon , Isao Watanabe , Kenji Nakajima

The frustrated pyrochlore iridate Pr$_2$Ir$_2$O$_7$ was proposed as a metallic quantum spin liquid located at a zero-field quantum critical point. Here we present the ultralow-temperature thermal conductivity measurements on the…

Strongly Correlated Electrons · Physics 2022-08-23 J. M. Ni , Y. Y. Huang , E. J. Cheng , Y. J. Yu , B. L. Pan , Q. Li , L. M. Xu , Z. M. Tian , S. Y. Li

Neutron scattering and magnetization measurements have been performed on the stuffed pyrochlore system Tb2+xTi2-2xNbxO7. We find that despite the introduction of chemical disorder and increasingly antiferromagnetic interactions, a spin…

Strongly Correlated Electrons · Physics 2010-02-25 B. G. Ueland , J. S. Gardner , A. J. Williams , M. L. Dahlberg , J. G. Kim , Y. Qiu , J. R. D. Copley , P. Schiffer , R. J. Cava

The ground state of the quantum spin ice candidate magnet Yb2Ti2O7 is known to be sensitive to weak disorder at the 1 percent level which occurs in single crystals grown from the melt. Powders produced by solid state synthesis tend to be…

Strongly Correlated Electrons · Physics 2016-03-09 J. Gaudet , K. A. Ross , E. Kermarrec , N. P. Butch , G. Ehlers , H. A. Dabkowska , B. D. Gaulin

We used a local susceptibility approach in extensive polarized neutron diffraction studies of the spin liquid \tbti. For a magnetic field applied along the [110] and [111] directions, we found that, at high temperature, all Tb moments are…

Strongly Correlated Electrons · Physics 2015-05-13 Arsen Gukasov , Huibo Cao , Isabelle Mirebeau , Pierre Bonville

Sc$_{2}$Ga$_{2}$CuO$_{7}$ (SGCO) crystallizes in a hexagonal structure (space group: $P$$6$$_{3}/mmc$),\textcolor{black}{{} which can be seen as an alternating stacking of single and double triangular layers. Combining neutron, x-ray, and…

Strongly Correlated Electrons · Physics 2015-11-25 R. Kumar , P. Khuntia , D. Sheptyakov , P. G. Freeman , H. M. Rønnow , B. Koteswararao , M. Baenitz , M. Jeong , A. V. Mahajan

High resolution time-of-flight neutron scattering measurements on Tb2Ti2O7 reveal a rich low temperature phase diagram in the presence of a magnetic field applied along [110]. In zero field at T=0.4 K, terbium titanate is a highly…

The layered triangular lattice owing to $1:2$ order of $B$ and $B'$ sites in the triple perovskite $A_3 B B'_2$O$_9$ family provides an enticing domain for exploring the complex phenomena of quantum spin liquids (QSLs). We report a…

Strongly Correlated Electrons · Physics 2024-08-07 K. Bhattacharya , S. Mohanty , A. D. Hillier , M. T. F. Telling , R. Nath , M. Majumder

We theoretically investigate the low-temperature phase of the recently synthesized Lu$_2$Mo$_2$O$_5$N$_2$ material, an extraordinarily rare realization of a $S=1/2$ three-dimensional pyrochlore Heisenberg antiferromagnet in which Mo$^{5+}$…

Supersolid, an exotic quantum state of matter that consists of particles forming an incompressible solid structure while simultaneously showing superfluidity of zero viscosity [1], is one of the long-standing pursuits in fundamental…

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

A comprehensive $^{31}$P nuclear magnetic resonance (NMR) study, combined with thermodynamic measurements and first-principle band-structure calculations, has been conducted to explore the ground state of the $S = 5/2$ double trillium…

Strongly Correlated Electrons · Physics 2025-12-08 Sebin J. Sebastian , Q. -P. Ding , A. A. Tsirlin , R. Nath , Y. Furukawa

The Ce$^{3+}$ pseudospin-$\frac{1}{2}$ degrees of freedom in the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ are known to possess dipole-octupole (DO) character, making it a candidate for novel quantum spin liquid (QSL) ground states at low…

The thermodynamic properties of the pyrochlore Yb2Ti2O7 material are calculated using the numericallinked-cluster (NLC) calculation method for an effective anisotropic-exchange spin-1/2 Hamiltonian with parameters recently determined by…

Strongly Correlated Electrons · Physics 2014-04-11 N. R. Hayre , K. A. Ross , R. Applegate , T. Lin , R. R. P. Singh B. D. Gaulin , M. J. P. Gingras

We investigated the possibility of temperature dependent lattice distortions in the pyrochlore compound Tb$_{2}$Ti$_{2}$O$_{7}$ by measuring the internal magnetic field distribution, using muon spin resonance, and comparing it to the…

Strongly Correlated Electrons · Physics 2015-06-25 Oren Ofer , Amit Keren , Chris Baines , Jason S. Gardner

Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental…

We present muon spin relaxation ($\mu$SR) and specific-heat versus temperature $C(T)$ measurements on polycrystalline and single-crystal samples of the pyrochlore magnet Yb$_2$Ti$_2$O$_7$. $C(T)$ exhibits a sharp peak at a $T_\mathrm{C}$ of…

Strongly Correlated Electrons · Physics 2014-05-28 Lieh-Jeng Chang , Martin R. Lees , Isao Watanabe , Adrian D. Hillier , Yukio Yasui , Shigeki Onoda

Quantum spin liquid (QSL) state in rare-earth triangular lattice has attracted much attention recently due to its potential application in quantum computing and communication. Here we report the single-crystal growth synthesis, crystal…

Strongly Correlated Electrons · Physics 2021-11-16 Jie Xing , Liurukara D. Sanjeewa , Andrew F. May , Athena S. Sefat