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We study the impact of Rydberg molecule formation on the storage and retrieval of Rydberg polaritons in an ultracold atomic medium. We observe coherent revivals appearing in the retrieval efficiency of stored photons that originate from…

The chemical bond is one of the most powerful, yet controversial concepts in chemistry, explaining property trends in solids. Recently, a novel type of chemical bonding has been identified in several higher chalcogenides, characterized by a…

We show that the dipole-dipole interaction between two Rydberg atoms can give rise to long range molecules. The binding potential arises from two states that converge to different separated atom asymptotes. These states interact weakly at…

Atomic Physics · Physics 2015-06-05 Martin Kiffner , Hyunwook Park , Wenhui Li , Tom F. Gallagher

In the laser excitation of ultracold atoms to Rydberg states, we observe a dramatic suppression caused by van der Waals interactions. This behavior is interpreted as a local excitation blockade: Rydberg atoms strongly inhibit excitation of…

Atomic Physics · Physics 2009-11-10 D. Tong , S. M. Farooqi , J. Stanojevic , S. Krishnan , Y. P. Zhang , R. Côté , E. E. Eyler , P. L. Gould

We report on the observation of ultralong range interactions in a gas of cold Rubidium Rydberg atoms. The van-der-Waals interaction between a pair of Rydberg atoms separated as far as 100,000 Bohr radii features two important effects:…

Controlling strongly interacting many-body systems enables the creation of tailored quantum matter, with properties transcending those based solely on single particle physics. Atomic ensembles which are optically driven to a Rydberg state…

Techniques for producing cold and ultracold molecules are enabling the study of chemical reactions and scattering at the quantum scattering limit, with only a few partial waves contributing to the incident channel, leading to the…

Chemical Physics · Physics 2016-09-21 Jonathan Tennyson , Laura K. McKemmish , Tom Rivlin

In excited molecules, the interaction between the covalent Rydberg and ion-pair channels forms a unique class of excited Rydberg states, in which the infinite manifold of vibrational levels are the equivalent of atomic Rydberg states with a…

Atomic Physics · Physics 2016-06-22 Samuel Markson , Hossein Sadeghpour

We present a combined experimental and theoretical study of the effects of Rydberg interactions on Autler-Townes spectra of ultracold gases of atomic strontium. Realizing two-photon Rydberg excitation via a long-lived triplet state allows…

We explore the prospects for confining alkaline-earth Rydberg atoms in an optical lattice via optical dressing of the secondary core valence electron. Focussing on the particular case of strontium, we identify experimentally accessible…

Atomic Physics · Physics 2015-05-27 R. Mukherjee , J. Millen , R. Nath , M. P. A. Jones , T. Pohl

First-principles crystal structure search is performed to predict novel rubidium poly-nitrogen materials at high pressure by varying the stoichiometry, i. e. relative quantities of the constituent rubidium and nitrogen atoms. Three…

Materials Science · Physics 2017-11-29 Ashley S. Williams , Brad A. Steele , van I. Oleynik

Unusual chemical bonds are proposed. Each bond is almost covalent but is characterized by the thread of a small radius $\sim 0.6\times 10^{-11}$cm, between two nuclei in a molecule. The main electron density is concentrated outside the…

Chemical Physics · Physics 2015-01-07 B. Ivlev

This topical review addresses how Rydberg atoms can serve as building blocks for emerging quantum technologies. Whereas the fabrication of large numbers of artificial quantum systems with the uniformity required for the most attractive…

Atomic Physics · Physics 2020-01-08 C. S. Adams , J. D. Pritchard , J. P. Shaffer

We propose an experiment to demonstrate a novel blockade mechanism caused by long-range anisotropic interactions in an ultracold dipolar gas composed of the recently observed "butterfly" Rydberg molecules. At the blockade radius, the strong…

Atomic Physics · Physics 2017-09-21 Matthew T. Eiles , Hyunwoo Lee , Jesus Perez-Rios , Chris H. Greene

Present nuclear detection techniques prevents us from determining if the analogue of a Rydberg molecule exists for the nuclear case. But nothing in nature disallows their existence. As in the atomic case, Rydberg nuclear molecules would be…

Nuclear Theory · Physics 2017-11-22 C. A. Bertulani , T. Frederico , M. S. Hussein

We propose a mechanism of ground-state blockade between two $N$-type Rydberg atoms in virtue of Rydberg-antiblockade effect and Raman transition. Inspired by the quantum Zeno effect, the strong Rydberg antiblockade interaction plays a role…

Quantum Physics · Physics 2017-12-07 X. Q. Shao , D. X. Li , Y. Q. Ji , J. H. Wu , X. X. Yi

A twist between two systems offers the possibility to drastically change the underlying physical properties. To that end, we study the bandstructure of twisted moir\'e potentials in detail. At sets of commensurate twisting angles, the low…

Quantum Gases · Physics 2025-04-11 Dean Johnstone , Shanya Mishra , Zhaoxuan Zhu , Laurent Sanchez-Palencia

Cold Rydberg atoms exposed to strong magnetic fields possess unique properties which open the pathway for an intriguing many-body dynamics taking place in Rydberg gases consisting of either matter or anti-matter systems. We review both the…

Atomic Physics · Physics 2015-05-14 T. Pohl , H. R. Sadeghpour , P. Schmelcher

Feshbach resonances in ultra-cold atomic gases have led to some of the most important advances in atomic physics. They did not only enable ground breaking work in the BEC-BCS crossover regime [1], but are also widely used for the…

Atomic Physics · Physics 2018-07-04 Oliver Thomas , Carsten Lippe , Tanita Eichert , Herwig Ott

We introduce a computational method developed for study of long-range molecular Rydberg states of such systems that can be approximated by two electrons in a model potential of the atomic cores. Only diatomic molecules are considered. The…

Chemical Physics · Physics 2016-01-26 Michal Tarana , Roman Čurík
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