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Third-order bound-charge electronic nonlinearities of Si nanocrystals (NCs) embedded in a wide band-gap matrix representing silica are theoretically studied using an atomistic pseudopotential approach. Nonlinear refractive index, two-photon…

Materials Science · Physics 2016-08-17 Hasan Yıldırım , Ceyhun Bulutay

Embedded Si and Ge nanocrystals (NCs) in wide band-gap matrices are studied theoretically using an atomistic pseudopotential approach. From small clusters to large NCs containing on the order of several thousand atoms are considered.…

Materials Science · Physics 2007-11-27 C. Bulutay

We demonstrate third harmonic generation in plasmonic antennas made of highly doped germanium and designed to be resonant in the mid infrared. Owing to the near-field enhancement, the result is an ultrafast, sub-diffraction, coherent light…

We compute from first principles the infrared dispersion of the nonlinear susceptibility $\chi^{(2)}$ in zincblende semiconductors. At terahertz frequencies the nonlinear susceptibility depends not only on the purely electronic response…

Materials Science · Physics 2009-12-17 Eric Roman , Jonathan R. Yates , Marek Veithen , David Vanderbilt , Ivo Souza

We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…

Mesoscale and Nanoscale Physics · Physics 2017-04-13 Peter R. Wiecha , Arnaud Arbouet , Houssem Kallel , Priyanka Periwal , Thierry Baron , Vincent Paillard

The effective linear and third-order nonlinear optical properties of metallic colloidal crystal immersed in a graded-index host fluid are investigated theoretically. The local electric fields are extracted self-consistently based on the…

Materials Science · Physics 2007-05-23 J. J. Xiao , K. W. Yu

Germanium self-assembled nanoislands and quantum dots are very prospective for CMOS-compatible optoelectronic integrated circuits but their luminescence intensity is still insufficient for many practical applications. Here, we demonstrate…

We study a hybrid system consisting of a narrowband atomic optical resonance and the long-range periodic order of an opaline photonic nanostructure. To this end, we have infiltrated atomic cesium vapor in a thin silica opal photonic…

The phenomenological boundary conditions for the envelope wave function, which is applicable for contacts of semiconductors with the rather different crystal symmetry are proposed. It is shown that the boundary conditions are determined by…

Materials Science · Physics 2008-02-03 Leonid S. Braginsky

The structural, electronic and optical properties of Si nanocrystals of different size and shape, passivated with hydrogens, OH groups, or embedded in a SiO2 matrix are studied. The comparison between the embedded and free, suspended…

Materials Science · Physics 2010-09-01 Roberto Guerra , Elena Degoli , Stefano Ossicini

Germanium is a strong candidate as a laser source for silicon photonics. It is widely accepted that the band structure of germanium can be altered by tensile strain so as to reduce the energy difference between its direct and indirect band…

Irradiance dependence of excitonic nonlinear absorption in Cadmium Sulfide (CdS) nanocrystals has been studied by using Z-scan method with nanosecond laser pulses. The wavelength dependence of nonlinear absorption has also been measured…

Materials Science · Physics 2009-11-11 J. He , W. Ji , G. H. Ma , S. H. Tang , H. I. Elim , W. X. Sun , Z. H. Zhang , W. S. Chin

Silicon photonics has attracted significant interest in recent years due to its potential in integrated photonics components (1,2) as well as all-dielectric meta-optics elements.(3) Strong photon-photon interactions, aka optical…

Using a hydrodynamic approach we examine bulk- and surface-induced second and third harmonic generation from semiconductor nanowire gratings having a resonant nonlinearity in the absorption region. We demonstrate resonant, broadband and…

Optical bound state in the continuum (BIC) is characterized by infinitely high quality factor resulting in drastic enhancement of light-matter interaction phenomena. We study the optical response of a one-dimensional photonic crystal slab…

Optics · Physics 2018-07-04 S. D. Krasikov , A. A. Bogdanov , I. V. Iorsh

We discuss the recent advances in meta-optics and nanophotonics associated with the physics of bound states in the continuum (BICs). Such resonant states appear due to a strong coupling between leaky modes in optical guiding structures…

Optics · Physics 2018-10-23 Kirill Koshelev , Andrey Bogdanov , Yuri Kivshar

We consider light absorption in a germanium grating placed on top of photonic-crystalline substrate. Such a system supports an optical Tamm state decoupled from the continuous spectrum with its frequency within the photonic band gap. We…

Resonant photonic nanostructures exhibiting enhanced nonlinear responses and efficient frequency conversion are an emergent platform in nonlinear optics. High-index semiconductor metasurfaces with rapidly tuned high-Q resonances enable a…

Two approaches (micro- and macro- investigations) are used to determine the dimension dependences of the optical parameters of the nanometer-scale layers of materials. It is shown that both an index of refraction and coefficient of…

Materials Science · Physics 2016-10-13 T. A. Kudykina , A. I. Pervak

We have calculated the contribution of intersubband transitions to the third order optical nonlinear susceptibility, $\chi^{(3)}(\omega,\omega,\omega)$ for nonresonant as well as resonant third harmonic generation and…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Sanghamitra Mukhopadhyay , K. C. Rustagi
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