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Honeycomb Na$_2$IrO$_3$ is a prototype spin-orbit Mott insulator and Kitaev magnet. We report a combined structural and electrical resistivity study of Na$_2$IrO$_3$ single crystals. Laue back-scattering diffraction indicates twinning with…

Strongly Correlated Electrons · Physics 2023-12-12 Franziska A. Breitner , Julian Kaiser , Anton Jesche , Philipp Gegenwart

Achieving large-area uniform two-dimensional (2D) metal-organic frameworks (MOFs) and controlling their electronic properties on inert surfaces is a big step towards future applications in electronic devices. Here we successfully fabricated…

We have varied the disorder in a two-dimensional electron system in silicon by applying substrate bias. When the disorder becomes sufficiently low, we observe the emergence of the metallic phase, and find evidence for a metal-insulator…

Strongly Correlated Electrons · Physics 2009-10-30 Dragana Popovic , A. B. Fowler , S. Washburn

We investigated a system based solely on a single molecular species, Cu(tmdt)$_{2}$, accommodating $d$ and ${\pi}$ orbitals within the molecule. $^{13}$C nuclear magnetic resonance measurements captured singlet-triplet excitations of…

Materials Science · Physics 2017-03-17 Rina Takagi , Takamasa Hamai , Hiro Gangi , Kazuya Miyagawa , Biao Zhou , Akiko Kobayashi , Kazushi Kanoda

The spin-orbit Mott insulator Sr3Ir2O7 provides a fascinating playground to explore insulator-metal transition driven by intertwined charge, spin, and lattice degrees of freedom. Here, we report high pressure electric resistance and…

The electrical control of a material's conductivity is at the heart of modern electronics. Conventionally, this control is achieved by tuning the density of mobile charge carriers. A completely different approach is possible in Mott…

The electronic structures of the metallic and insulating phases of the alloy series Ca(2-x)Sr(x)RuO4 (0 <= x <= 2) are calculated using LDA, LDA+U and Dynamical Mean-Field Approximation methods. In the end members the groundstate…

Strongly Correlated Electrons · Physics 2009-09-25 V. I. Anisimov , I. A. Nekrasov , D. E. Kondakov , T. M. Rice , M. Sigrist

Impedance spectroscopy measurements were performed in high quality Vanadium dioxide (VO2) thin films. This technique allows us investigate the resistive and capacitive contribution to the dielectric response near the metal-insulator…

Materials Science · Physics 2011-05-24 J. -G. Ramírez , Edgar J. Patiño , Rainer Schmidt , Amos Sharoni , M. E. Gómez , Ivan K. Schuller

The static and dynamic local spin susceptibility of the organic Mott insulator $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$, a model material of the spin- 1/2 triangular lattice, is studied by $^{13}$C NMR spectroscopy from room temperature down to 20…

Strongly Correlated Electrons · Physics 2007-05-23 Yasuhiro Shimizu , Kazuya Miyagawa , Kazushi Kanoda , Maesato Mitsuhiko , Gunzi Saito

The optical properties of a spherical topological insulator embedded concentrically in a single-electron system consisting of a core-shell GaAs quantum dot are analyzed, when the system is under a uniform external magnetic field. The…

Mesoscale and Nanoscale Physics · Physics 2020-05-29 Jorge David Castaño-Yepes , O. J. Franca , C. F. Ramirez-Gutierrez , J. C. del Valle

We performed angular and temperature-dependent electron-spin-resonance measurements in the quasi-two-dimensional organic conductor $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]I. The interlayer spin-diffusion is much weaker compared to the Cl- and…

We consider the possibility that the electrons injected into organic field-effect transistors are strongly correlated. A single layer of acenes can be modelled by a Hubbard Hamiltonian similar to that used for the kappa-(BEDT-TTF)(2)X…

Strongly Correlated Electrons · Physics 2009-11-07 Olivier Cepas , Ross H. McKenzie

A fully first principles theory capable of treating strongly correlated solids remains the outstanding challenge of modern day materials science. This is exemplified by the transition metal oxides, prototypical Mott insulators, that remain…

Strongly Correlated Electrons · Physics 2015-07-08 Y. Shinohara , S. Sharma , S. Shallcross , J. K. Dewhurst , N. N. Lathiotakis , E. K. U. Gross

Unveiling the physics that governs the intertwining between the nanoscale self-organization and the dynamics of insulator-to-metal transitions (\textit{IMT}) is key for controlling on demand the ultrafast switching in strongly correlated…

Many strongly correlated electronic materials, including high-temperature superconductors, colossal magnetoresistance and metal-insulator-transition (MIT) materials, are inhomogeneous on a microscopic scale as a result of domain structure…

Mesoscale and Nanoscale Physics · Physics 2012-09-05 Jiang Wei , Zenghui Wang , Wei Chen , David H. Cobden

The organic salt $\alpha$-(BEDT-TTF)$_2$I$_3$ is considered a model system for metal-insulator transition due to electronic charge ordering at $T_{\rm CO}=135$~K. The optical properties obtained from polarized reflection measurements above…

Strongly Correlated Electrons · Physics 2016-03-25 T. Peterseim , M. Dressel

Two-dimensional materials have proven to be a prolific breeding ground of new and unstudied forms of magnetism and unusual metallic states, particularly when tuned between their insulating and metallic phases. In this paper we present work…

Strongly Correlated Electrons · Physics 2019-01-02 C. R. S. Haines , M. J. Coak , G. I. Lampronti , C. Liu , H. Hamidov , A. R. Wildes , D. Daisenberger , P. Nahai-Williamson , S. S. Saxena

Resonant inelastic x-ray scattering at the N K edge reveals clearly resolved harmonics of the anion plane vibrations in the kappa-(BEDT-TTF)2Cu2(CN)3 spin-liquid insulator. Tuning the incoming light energy at the K edge of two distinct N…

We numerically investigate the dynamical properties of $\kappa$-type molecular conductors in their antiferromagnetic Mott insulating state. By treating the extended Hubbard model on the two-dimensional $\kappa$-type lattice within the…

Strongly Correlated Electrons · Physics 2021-06-22 Hitoshi Seo , Makoto Naka

Atom probe tomography requires needle-shaped specimens with a diameter typically below 100 nm, making them both very fragile and reactive, and defects (notches at grain boundaries or precipitates) are known to affect the yield and data…