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The pyrochlore material Yb2Ti2O7 displays unexpected quasi-two-dimensional (2D) magnetic correlations within a cubic lattice environment at low temperatures, before entering an exotic disordered ground state below T=265mK. We report neutron…

Strongly Correlated Electrons · Physics 2012-02-13 K. A. Ross , L. R. Yaraskavitch , M. Laver , J. S. Gardner , J. A. Quilliam , S. Meng , J. B. Kycia , D. K. Singh , H. A. Dabkowska , B. D. Gaulin

We report on the study of unusual spin glass properties in the geometrically frustrated pyrochlore Tb$_{2}$Mo$_{2}$O$_{7}$, $T$$_{g}$$\simeq$24 K. The analysis of the nonlinear part of dc and complex susceptibilities, near the glass…

Strongly Correlated Electrons · Physics 2013-09-17 D. K. Singh , Y. S. Lee

Structural disorder in the magnetically frustrated pyrochlore system leads to intriguing magnetic states. We present the thermodynamic behavior and short range magnetic correlations in Tb$_{2}$Zr$_{2}$O$_{7}$ and…

Strongly Correlated Electrons · Physics 2026-04-16 Sujata Singh , Leon Carstens , M. Duc Le , R. Klingeler , C. S. Yadav

We present a parametric study of the diffuse magnetic scattering at (1/2,1/2,1/2) positions in reciprocal space, ascribed to a frozen antiferromagnetic spin ice state in single crystalline Tb2Ti2O7. Our high-resolution neutron scattering…

Strongly Correlated Electrons · Physics 2015-06-18 K. Fritsch , E. Kermarrec , K. A. Ross , Y. Qiu , J. R. D. Copley , D. Pomaranski , J. B. Kycia , H. A. Dabkowska , B. D. Gaulin

The geometrically-frustrated spin glass Y2Mo2O7 has been considered widely to be crystallographically ordered with a unique nearest neighbor magnetic exchange interaction, J. To test this assertion, we present x-ray-absorption…

Statistical Mechanics · Physics 2009-10-31 C. H. Booth , J. S. Gardner , G. H. Kwei , R. H. Heffner , F. Bridges , M. A. Subramanian

High resolution X-ray scattering measurements on single crystal Tb2Ti2O7 reveal finite structural correlations at low temperatures. This geometrically frustrated pyrochlore is known to exhibit a spin liquid, or cooperative paramagnetic…

Disordered Systems and Neural Networks · Physics 2009-11-13 J. P. C. Ruff , B. D. Gaulin , J. P. Castellan , K. C. Rule , J. P. Clancy , J. Rodriguez , H. A. Dabkowska

We present high-resolution single crystal time-of-flight neutron scattering measurements on the candidate quantum spin liquid pyrochlore Tb2Ti2O7 at low temperature and in a magnetic field. At ~70 mK and in zero field, Tb2Ti2O7 reveals…

Strongly Correlated Electrons · Physics 2013-04-16 K. Fritsch , K. A. Ross , Y. Qiu , J. R. D. Copley , T. Guidi , R. I. Bewley , H. A. Dabkowska , B. D. Gaulin

Tb2Ti2O7 is a pyrochlore antiferromagnet that has dynamical spins and only short-range correlations even at 50 mK; the lowest temperature explored so far, which is much smaller than the scale set by the Curie-Weiss temperature T_{CW}~14 K.…

Statistical Mechanics · Physics 2009-12-16 Hamid R. Molavian , Paul A. McClarty , Michel J. P. Gingras

Some frustrated pyrochlore antiferromagnets, such as Y2Mo2O7, show a spin-freezing transition and magnetic irreversibilities below a temperature Tf similar to what is observed nonlinear magnetization measurements on Y2Mo2O7 that provide…

Disordered Systems and Neural Networks · Physics 2009-10-28 M. J. P. Gingras , C. V. Stager , N. P. Raju , B. D. Gaulin , J. E. Greedan

The spin dynamics of geometrically frustrated pyrochlore antiferromagnets Y2Mo2O7 and Tb2Mo2O7 have been investigated using muon spin relaxation. A dramatic slowing down of the moment fluctuations occurs as one approaches the spin freezing…

Recent elastic and inelastic neutron scattering studies of the highly frustrated pyrochlore antiferromagnet Tb2Ti2O7 have shown some very intriguing features that cannot be modeled by the local <111> classical Ising model, naively expected…

Disordered Systems and Neural Networks · Physics 2007-05-23 Ying-Jer Kao , Matthew Enjalran , Adrian Del Maestro , Hamid R. Molavian , Michel J. P. Gingras

The nature of the low temperature ground state of the pyrochlore compound Tb2Ti2O7 remains a puzzling issue. Dynamic fluctuations and short-range correlations persist down to 50 mK, as evidenced by microscopic probes. In parallel,…

Strongly Correlated Electrons · Physics 2012-08-02 E. Lhotel , C. Paulsen , P. Dalmas de Réotier , A. Yaouanc , C. Marin , S. Vanishri

We report synchrotron radiation diffraction and muon spin rotation (muSR) measurements on the frustrated pyrochlore magnet Tb2Ti2O7. The powder diffraction study of a crushed crystal fragment does not reveal any structural change down to 4…

Strongly Correlated Electrons · Physics 2014-12-22 P. Dalmas de Reotier , A. Yaouanc , A. Bertin , C. Marin , S. Vanishri , D. Sheptyakov , A. Cervellino , B. Roessli , C. Baines

Although materials that exhibit nearest-neighbor-only antiferromagnetic interactions and geometrical frustration theoretically should not magnetically order in the absence of disorder, few such systems have been observed experimentally. One…

Strongly Correlated Electrons · Physics 2016-08-31 S. -W. Han , J. S. Gardner , C. H. Booth

By means of neutron scattering techniques we have investigated the frustrated pyrochlore magnet Ho_2Sn_2O_7, which was found to show a ferromagnetic spin-ice behavior below T \simeq 1.4 K by susceptibility measurements. High-resolution…

Disordered Systems and Neural Networks · Physics 2007-05-23 Hiroaki Kadowaki , Yoshinobu Ishii , Kazuyuki Matsuhira , Yukio Hinatsu

Neutron scattering, a.c. magnetic susceptibility and specific heat studies have been carried out on polycrystalline Dy2Zr2O7. Unlike the pyrochlore spin ice Dy2Ti2O7, Dy2Zr2O7 crystallizes into the fluorite structure and the magnetic Dy3+…

Disordered Systems and Neural Networks · Physics 2019-07-01 J. G. A. Ramon , C. W. Wang , L. Ishida , P. L. Bernardo , M. M. Leite , F. M. Vichi , J. S. Gardner , R. S. Freitas

Two geometrically frustrated pyrochlore stannates, undergoing long range magnetic order below 1K, were investigated at very low temperature. Anomalies in the behaviour of hyperfine quantities are found, by 155Gd Mossbauer spectroscopy in…

Strongly Correlated Electrons · Physics 2009-11-13 P. Bonville , I. Mirebeau , J. P. Sanchez

In the pyrochlore compounds, Tb$_2$Ti$_2$O$_7$ and Tb$_2$Sn$_2$O$_7$, only the Tb$^{3+}$ ions are magnetic. They exhibit quite abnormal -- and, in view of their chemical similarity, strikingly different -- magnetic behaviour, as probed by…

Strongly Correlated Electrons · Physics 2009-11-11 I. Mirebeau , A. Apetrei , I. N. Goncharenko , R. Moessner

The spin glass behavior of Y2Mo2O7 has puzzled physicists for nearly three decades. Free of bulk disorder within the resolution of powder diffraction methods, it is thought that this material is a rare realization of a spin glass resulting…

Elastic and inelastic neutron scattering studies have been carried out on the pyrochlore magnet Ho2Ti2O7. Measurements in zero applied magnetic field show that the disordered spin ice ground state of Ho2Ti2O7 is characterized by a pattern…

Strongly Correlated Electrons · Physics 2016-08-05 J. P. Clancy , J. P. C. Ruff , S. R. Dunsiger , Y. Zhao , H. A. Dabkowska , J. S. Gardner , Y. Qiu , J. R. D. Copley , T. Jenkins , B. D. Gaulin
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