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Spin correlations of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been investigated by using inelastic neutron scattering on single crystalline samples ($x=-0.007, 0.000,$ and $0.003$), which have the putative…

Strongly Correlated Electrons · Physics 2019-01-08 Hiroaki Kadowaki , Mika Wakita , Björn Fåk , Jacques Ollivier , Seiko Ohira-Kawamura , Kenji Nakajima , Jeffrey W. Lynn

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

We present here magnetization, specific heat and Raman studies on single-crystalline specimens of the first pyrochlore member $Sm_2Ti_2O_7$ of the rare-earth titanate series. Its analogous compound $Sm_2Zr_2O_7$ in the rare-earth zirconate…

Materials Science · Physics 2009-11-13 Surjeet Singh , Surajit Saha , S. K. Dhar , R. Suryanarayanan , A. K. Sood , A. Revcolevschi

We report the low-temperature magnetothermal properties and spin dynamics of a mixed pyrochlore, Dy2GaSbO7 through the coordination of measurements of dc magnetization, ac susceptibility, and heat capacity, and CF computation. In Dy2GaSbO7,…

Materials Science · Physics 2021-04-19 Saikat Nandi , Yatramohan Jana , Jahangir Alam , Pallab Bag , S. S. Islam , Ramesh Nath

We investigated the nature of the spin glass-like phase transition in the geometrically frustrated pyrochlore lattices Y$_{2}$Mo$_{2}$O$_{7}$ using the local probes nuclear and muon magnetic resonances, and the field-dependent long range…

Strongly Correlated Electrons · Physics 2010-09-24 Oren Ofer , Amit Keren , Jason S. Gardner , Yang Ren , W. A. MacFarlane

The pyrochlore material $\rm Ho_{2}Ti_{2}O_{7}$ has been suggested to show ``spin ice'' behaviour. We present neutron scattering and specific heat results that establish unambiguously that Ho$_2$Ti$_2$O$_7$ exhibits spin ice correlations at…

We report high resolution single crystal x-ray diffraction measurements of the frustrated pyrochlore magnet Tb2Ti2O7, collected using a novel low temperature pulsed magnet system. This instrument allows characterization of structural…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , Z. Islam , J. P. Clancy , K. A. Ross , H. Nojiri , Y. H. Matsuda , H. A. Dabkowska , A. D. Dabkowski , B. D. Gaulin

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

Disordered Systems and Neural Networks · Physics 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

Dy2Ti2O7 is a geometrically frustrated magnetic material with a strongly correlated spin ice regime that extends from 1 K down to as low as 60 mK. The diffuse elastic neutron scattering intensities in the spin ice regime can be remarkably…

Statistical Mechanics · Physics 2008-08-02 Taras Yavors'kii , Tom Fennell , Michel J. P. Gingras , Steven T. Bramwell

The very low temperature properties of two pyrochlore compounds, Yb2Ti2O7 and Gd2Sn2O7, were investigated using an ensemble of microscopic and bulk techniques. In both compounds, a first order transition is evidenced, as well as spin…

Static and dynamical properties of the magnetic moment system of pyrochlore compound Tb2Ti2O7 with strong magnetic frustration, have been investigated down to the temperature T=0.4 K by neutron scattering on a single crystal sample. The…

We have studied magnetically frustrated Tb$_2$Sn$_2$O$_7$ by neutron diffraction and high resolution energy-resolved neutron scattering. At 0.1 K, we observe short range magnetic correlations with a typical scale of 4 \AA, close to the near…

Strongly Correlated Electrons · Physics 2009-11-13 I. Mirebeau , H. Mutka , P. Bonville , A. Apetrei , A. Forget

The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

Statistical Mechanics · Physics 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

High resolution X-ray powder-diffraction experiments on a well-characterized polycrystalline sample of the spin liquid Tb2Ti2O7 reveal that it shows normal positive thermal-expansion above 4 K, which does not agree with the intriguing…

Strongly Correlated Electrons · Physics 2011-12-14 Kazuki Goto , Hiroshi Takatsu , Tomohiro Taniguchi , Hiroaki Kadowaki

We have studied (Tb$_{1-x}$La$_x$)$_2$Mo$_2$O$_7$ pyrochlores by neutron diffraction and $\mu$SR at ambient and under applied pressure. Substitution of Tb for La expands the lattice and induces a change from a spin-glass like state…

Strongly Correlated Electrons · Physics 2007-05-23 A. Apetrei , I. Mirebeau , I. Goncharenko , D. Andreica , P. Bonville

We report measurements performed on a polycrystalline sample of the pyrochlore compound Nd2Sn2O7. It undergoes a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in-all-out magnetic structure of the Nd3+ magnetic…

Strongly Correlated Electrons · Physics 2015-11-04 A. Bertin , P. Dalmas de Reotier , B. Fak , C. Marin , A. Yaouanc , A. Forget , D. Sheptyakov , B. Frick , C. Ritter , A. Amato , C. Baines , P. J. C. King

We report a study of the low temperature bulk magnetic properties of the spin ice compound Dy2Ti2O7 with particular attention to the (T < 4 K) spin freezing transition. While this transition is superficially similar to that in a spin glass,…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

Magnetization and susceptibility studies on single crystals of the pyrochlore Ho$_{2}$Ti$_{2}$O$_{7}$ are reported for the first time. Magnetization isotherms are shown to be qualitatively similar to that predicted by the nearest neighbor…

Disordered Systems and Neural Networks · Physics 2009-11-07 A. L. Cornelius , J. S. Gardner

We present single-crystal neutron-diffuse-scattering measurements with polarization analysis on the spin ice Ho2-xYxTi2O7 (x = 0, 0.3, and 1). At 2 K, the spin flip scattering patterns are typical of a nearest-neighbor spin ice and the…

Strongly Correlated Electrons · Physics 2010-11-11 L. J. Chang , Y. Su , Y. -J. Kao , Y. Z. Chou , R. Mittal , H. Schneider , Th. Brueckel , G. Balakrishnan , M. R. Lees

We present an interpretation of zero field diffuse neutron scattering and of high field magnetisation data at very low temperature in the frustrated pyrochlore system Tb2Ti2O7. This material has antiferromagnetic exchange interactions and…

Strongly Correlated Electrons · Physics 2013-12-16 P. Bonville , A. Gukasov , I. Mirebeau , S. Petit