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Perturbed angular correlation spectroscopy combined with $ab-initio$ electronic structure calculations is used to unravel the structural phase transition path from the low-temperature polar structure to the high-temperature structural phase…

Triangular-lattice cobaltates with glaserite-type $X_2Y$Co($T$O$_4)_2$ structure provide an ideal platform to investigate intriguing quantum magnetism. Here we report a comprehensive study of the structural and magnetic properties of a…

Strongly Correlated Electrons · Physics 2026-03-10 Tengfei Peng , Xiaobai Ma , Xinyang Liu , Feiran Shen , Lunhua He , Junsen Xiang , Wenyun Yang , Wentao Jin

Neutron and x-ray diffraction measurements are presented for powders and single crystals of CaCo{1.86}As2. The crystal structure is a collapsed-tetragonal ThCr2Si2-type structure as previously reported, but with 7(1)% vacancies on the Co…

We report a detailed examination the magnetic structure of anhydrous cupric chloride CuCl2 carried out by powder neutron diffraction, magnetic susceptibility and specific heat measurements on polycrystalline and single crystal samples as…

Strongly Correlated Electrons · Physics 2009-04-21 M. G. Banks , R. K. Kremer , C. Hoch , A. Simon , B. Ouladdiaf , J. -M. Broto , H. Rakoto , C. Lee , M. -H. Whangbo

The alkaline-earth orthovanadate Sr$_3$V$_2$O$_8$ with the palmierite structure is reported to host a dielectric anomaly as well as a structural phase transition above the room temperature. With V$^{5+}$ ions and tetrahedral oxygen…

Materials Science · Physics 2023-11-28 Amartyajyoti Saha , Turan Birol

Depending on the crystal growth conditions, an orthorhombic (O-type) or a tetragonal (T-type) structure can be found in the solid solution Cs2CuCl4-xBrx (0 < x < 4). Here we present measurements of the temperature-dependent magnetic…

We have grown a YCrO$_3$ single crystal by the floating-zone method and studied its temperature-dependent crystalline structure and magnetization by X-ray powder diffraction and PPMS DynaCool measurements. All diffraction patterns were well…

Strongly Correlated Electrons · Physics 2024-03-08 Qian Zhao , Yinghao Zhu , Si Wu , Junchao Xia , Pengfei Zhou , Kaitong Sun , Hai-Feng Li

Ferroelectric ceramics (Ba0.85Ca0.15)(Ti0.9Zr0.1-xSnx)O3 (x=0.00, 0.02, 0.04, 0.06) were prepared by a sol-gel method. Structural investigation revealed the co-existence of tetragonal (P4mm) and orthorhombic (Pmm2) symmetries at room…

We report a ferroelectric order at ~ 98 K for NiFe2O4, which carries an inverse spinel structure with a centrosymmetric Fd3m structure at room temperature. The value of spontaneous electric polarization is considerably high as ~ 0.29…

Materials Science · Physics 2019-05-10 J. K. Dey , A. Chatterjee , S. Majumdar , A. -C. Dippel , O. Gutowski , M. v. Zimmermann , S. Giri

Microstructure properties, phase transitions, and charge ordering in the LuFe2O4 materials have been extensively investigated by means of transmission electron microscopy (TEM). The (001) twins as a common defect frequently appear in the…

Strongly Correlated Electrons · Physics 2007-05-23 Y. Zhang , H. X. Yang , C. Ma , H. F. Tian , J. Q. Li *

The phase diagram of Ca$_{2-x}$Sr$_x$RuO$_4$ has been studied by neutron diffraction on powder and single-crystalline samples. The experiments reveal antiferromagnetic order and structural distortions characterized by tilts and rotations of…

Superconductivity · Physics 2009-10-31 O. Friedt , M. Braden , G. Andre , P. Adelmann , S. Nakatsuji , Y. Maeno

Neutron diffraction studies have been carried out in the temperature(T) range between 10 K and 130 K on a single crystal of YBaCo4O7, which has the stacking of kagome and triangular lattices of CoO4 tetrahedra along the c-axis. Structural…

Strongly Correlated Electrons · Physics 2009-11-11 Minoru Soda , Yukio Yasui , Taketo Moyoshi , Masatoshi Sato , Naoki Igawa , Kazuhisa Kakurai

SrEr$_2$O$_4$ has been characterised by low-temperature powder neutron diffraction, as well as single crystal specific heat and magnetisation measurements. Magnetisation measurements show that the magnetic system is highly anisotropic at…

Strongly Correlated Electrons · Physics 2008-11-18 O. A. Petrenko , G. Balakrishnan , N. R. Wilson , S. de Brion , E. Suard , L. C. Chapon

We report on the crystallographic information such as lattice parameters, atomic positions, bond lengths and angles, and local crystalline distortion size and mode of single-crystal YCrO$_3$ compound by a high-resolution synchrotron X-ray…

Materials Science · Physics 2024-03-08 Qian Zhao , Si Wu , Yinghao Zhu , Junchao Xia , Hai-Feng Li

We have synthesized single crystals of Na$_3$Co$_2$SbO$_6$ and characterized the structure and magnetic order by measuring anisotropic magnetic properties, heat capacity, x-ray and neutron single crystal diffraction. Magnetic properties and…

Strongly Correlated Electrons · Physics 2019-07-17 J. -Q. Yan , S. Okamoto , Y. Wu , Q. Zheng , H. D. Zhou , H. B. Cao , M. A. McGuire

Using synchrotron X-rays and neutron diffraction we disentangle spin-lattice order in highly frustrated ZnCr$_2$O$_4$ where magnetic chromium ions occupy the vertices of regular tetrahedra. Upon cooling below 12.5 K the quandary of…

Strongly Correlated Electrons · Physics 2009-05-14 S. Ji , S. -H. Lee , C. Broholm , T. Y. Koo , W. Ratcliff , S-W. Cheong , P. Zschack

The determination by powder neutron diffraction of the ambient temperature crystal structures of compounds in the NaxCoO2 family, for 0.3 < x <= 1.0, is reported. The structures consist of triangular CoO2 layers with Na ions distributed in…

Strongly Correlated Electrons · Physics 2009-11-10 Q. Huang , M. L. Foo , R. A. Pascal , J. W. Lynn , B. H. Toby , Tao He , H. W. Zandbergen , R. J. Cava

Spinel compounds AB$_{2}$X$_{4}$ consist of both tetrahedral (AX$_{4}$) and octahedral (BX$_{6}$) environments with the former forming a diamond lattice and the latter a geometrically frustrated pyrochlore lattice. Exploring the fascinating…

Chemical Physics · Physics 2023-03-29 Qiang Zhang , Wei Tian , Roshan K. Nepal , Ashfia Huq , Stephen Nagler , J. F. DiTusa , Rongying Jin

The crystal structure of the copper(II) tellurium(IV) oxochloride Cu$_{4}$Te$_{5}$O$_{12}$Cl$_{4}$ (Cu-45124) is composed of weakly coupled tetrahedral Cu clusters and shows crystallographic similarities with the intensively investigated…

Strongly Correlated Electrons · Physics 2010-03-09 Rie Takagi , Mats Johnsson , Vladimir Gnezdilov , Reinhard K. Kremer , Wolfram Brenig , Peter Lemmens

The magnetic behavior of the compound, Gd3Ru4Al12, which has been reported to crystallize in a hexagonal structure about two decades ago, had not been investigated in the past literature despite interesting structural features (that is,…

Strongly Correlated Electrons · Physics 2016-06-22 Venkatesh Chandragiri , Kartik K Iyer , E. V. Sampathkumaran