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The structural and magnetic properties of YVO3, NdVO3 and TbVO3 were investigated by single-crystal and powder neutron diffraction. YVO3 shows a structural phase transition at 200 K from an orthorhombic structure with the space group Pbnm…

Strongly Correlated Electrons · Physics 2009-11-11 M. Reehuis , C. Ulrich , P. Pattison , B. Ouladdiaf , M. C. Rheinstadter , M. Ohl , L. P. Regnault , M. Miyasaka , Y. Tokura , B. Keimer

Intrinsic, in-plane anisotropy of electrical resistivity was studied on mechanically detwinned single crystals of SrFe$_2$As$_2$ above and below the temperature of the coupled structural/magnetic transition, $T_{\textrm{TO}}$. Resistivity…

We present single-crystal neutron-diffraction data for the spin-chain compound Ca3Co2O6. The intensity and line shapes of the two families of Bragg peaks characterising both the antiferromagnetic and the ferromagnetic components of the…

Strongly Correlated Electrons · Physics 2017-04-03 C. L. Fleck , M. R. Lees , S. Agrestini , G. J. McIntyre , O. A. Petrenko

We use powder neutron diffraction to study the spin and lattice structures of polycrystalline samples of nonsuperconducting PrFeAsO and superconducting PrFeAsO0.85F0.15 and PrFeAsO0.85. We find that PrFeAsO exhibits an abrupt structural…

Raman scattering can detect spontaneous point-group symmetry breaking without resorting to single-domain samples. Here we use this technique to study $\mathrm{BaFe_2As_2}$, the parent compound of the "122" Fe-based superconductors. We show…

Superconductivity · Physics 2015-11-10 Xiao Ren , Lian Duan , Yuwen Hu , Jiarui Li , Rui Zhang , Huiqian Luo , Pengcheng Dai , Yuan Li

In low-dimensional metallic systems, lattice distortion is usually coupled to a density-wave-like electronic instability due to Fermi surface nesting (FSN) and strong electron-phonon coupling. However, the ordering of other electronic…

Strongly Correlated Electrons · Physics 2018-12-26 D. W. Song , J. Li , D. Zhao , L. K. Ma , L. X. Zheng , S. J. Li , L. P. Nie , X. G. Luo , Z. P. Yin , T. Wu , X. H. Chen

We report a combination of X-ray and neutron diffraction studies, Mossbauer spectroscopy and muon spin relaxation (muSR) measurements to probe the structure and magnetic properties of the semiconducting beta-Ce2O2FeSe2 oxychalcogenide. We…

We have determined the spatial distribution of the magnetisation induced by a field of 9 T in the tetragonal phase of BaFe2As2 using polarised neutron diffraction. Magnetic structure factors derived from the polarisation dependence of the…

Strongly Correlated Electrons · Physics 2012-07-03 P. J. Brown , T. Chatterji , A. Stunault , Y. Su , Y. Xiao , R. Mittal , T. Brueckel , T. Wolf , P. Adelmann

The crystal structure and the magnetism of BaMn$_2$O$_3$ have been studied by thermodynamic and by diffraction techniques using large single crystals and powders. BaMn$_2$O$_3$ is a realization of a $S = 5/2$ spin ladder as the magnetic…

Strongly Correlated Electrons · Physics 2015-05-20 M. Valldor , O. Heyer , A. C. Komarek , A. Senyshyn , M. Braden , T. Lorenz

It has recently been demonstrated that dynamical magnetic correlations measured by neutron scattering in iron chalcogenides can be described with models of short-range correlations characterized by particular {choices of four-spin…

We report neutron diffraction studies of TbCo$_2$Zn$_{20}$ and TbFe$_2$Zn$_{20}$, two isostructural compounds which exhibit dramatically different magnetic behavior. In the case of TbCo$_2$Zn$_{20}$, magnetic Bragg peaks corresponding to…

Strongly Correlated Electrons · Physics 2015-05-18 W. Tian , A. D. Christianson , J. L. Zarestky , S. Jia , S. L. Bud'ko , P. C. Canfield , P. M. B. Piccoli , A. J. Schultz

Structural, magnetic, electrical transport, and heat capacity data are reported for single crystals of TlFe1.6Se2. This compound crystallizes in a tetragonal structure similar to the ThCr2Si2 structure, but with vacancies in the Fe layer.…

The magnetic structures and the magnetic phase transitions in the Mn-doped orthoferrite TbFeO$_3$ studied using neutron powder diffraction are reported. Magnetic phase transitions are identified at $T^\mathrm{Fe/Mn}_N \approx$ 295~K where a…

Strongly Correlated Electrons · Physics 2016-02-17 Harikrishnan S. Nair , Tapan Chatterji , C. M. N. Kumar , T. Hansen , Hariharan Nhalil , Suja Elizabeth , A. M. Strydom

The 1111 compounds with an alternating sequence of fluorite and antifluorite layers serve as structural hosts for the vast family of Fe-based superconductors. Here, we use neutron powder diffraction and density-functional-theory (DFT)…

Strongly Correlated Electrons · Physics 2023-02-22 Igor V. Plokhikh , Alexander A. Tsirlin , Dmitry D. Khalyavin , Henry E. Fischer , Andrei V. Shevelkov , Arno Pfitzner

Superconductivity in the iron pnictides emerges from metallic parent compounds exhibiting intertwined stripe-type magnetic order and nematic order, with itinerant electrons suggested to be essential for both. Here we use X-ray and neutron…

Strongly Correlated Electrons · Physics 2019-03-05 Yu Song , Huibo Cao , B. C. Chakoumakos , Yang Zhao , Aifeng Wang , Hechang Lei , C. Petrovic , Robert J. Birgeneau

The measurements of the magnetic susceptibility, magnetization, electrical resistivity and magnetoresistance have been performed for the Fe intercalated compound Fe0.5TiS2. According to X-ray diffraction measurements the Fe0.5TiS2 compound…

Nematicity, defined as broken rotational symmetry, has recently been observed in competing phases proximate to the superconducting phase in the cuprate high temperature superconductors. Similarly, the new iron-based high temperature…

Single crystals of SrMn$_2$Ni$_6$Te$_3$O$_{18}$, a member of the ferroaxial-type magnetic oxide family $AB_{2}C_{6}$Te$_3$O$_{18}$ ($A$ = Pb, Sr; $B$ = Mn, Cd; $C$ = Ni, Co), have been successfully grown, and their structural, magnetic,…

Materials Science · Physics 2026-04-24 Ryoya Nakamura , Shinichiro Asai , Yusuke Nambu , Takatsugu Masuda , Kenta Kimura

Iron-based superconductors can be categorized as two types of parent compounds by considering the nature of their temperature-induced phase transitions; namely, first order transitions for 122- and 11-type compounds and second-order…

In contrast to the simultaneous structural and magnetic first order phase transition $T_{0}$ previously reported, our detailed investigation on an underdoped Ba$_{0.84}$K$_{0.16}$Fe$_{2}$As$_{2}$ single crystal unambiguously revealed that…

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