English

Intertwined magnetic and nematic orders in semiconducting KFe$_{0.8}$Ag$_{1.2}$Te$_2$

Strongly Correlated Electrons 2019-03-05 v1

Abstract

Superconductivity in the iron pnictides emerges from metallic parent compounds exhibiting intertwined stripe-type magnetic order and nematic order, with itinerant electrons suggested to be essential for both. Here we use X-ray and neutron scattering to show that a similar intertwined state is realized in semiconducting KFe0.8_{0.8}Ag1.2_{1.2}Te2_2 (K5_5Fe4_4Ag6_6Te10_{10}) without itinerant electrons. We find Fe atoms in KFe0.8_{0.8}Ag1.2_{1.2}Te2_2 form isolated 2×22\times2 blocks, separated by nonmagnetic Ag atoms. Long-range magnetic order sets in below TN35T_{\rm N}\approx35 K, with magnetic moments within the 2×22\times2 Fe blocks ordering into the stripe-type configuration. A nematic order accompanies the magnetic transition, manifest as a structural distortion that breaks the fourfold rotational symmetry of the lattice. The nematic orders in KFe0.8_{0.8}Ag1.2_{1.2}Te2_2 and iron pnictide parent compounds are similar in magnitude and how they relate to the magnetic order, indicating a common origin. Since KFe0.8_{0.8}Ag1.2_{1.2}Te2_2 is a semiconductor without itinerant electrons, this indicates that local-moment magnetic interactions are integral to its magnetic and nematic orders, and such interactions may play a key role in iron-based superconductivity.

Keywords

Cite

@article{arxiv.1901.11206,
  title  = {Intertwined magnetic and nematic orders in semiconducting KFe$_{0.8}$Ag$_{1.2}$Te$_2$},
  author = {Yu Song and Huibo Cao and B. C. Chakoumakos and Yang Zhao and Aifeng Wang and Hechang Lei and C. Petrovic and Robert J. Birgeneau},
  journal= {arXiv preprint arXiv:1901.11206},
  year   = {2019}
}

Comments

supplemental material available upon request, to be published in PRL