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Time-domain femtosecond laser spectroscopic measurements of the ultrafast lattice dynamics in 2H-MoTe2 bulk crystals were carried out to understand the carrier-phonon interactions that govern electronic transport properties. An unusually…

Ultrafast relaxation dynamics of an athermal electron distribution is investigated in silver films using a femtosecond pump-probe technique with 18 fs pulses in off-resonant conditions. The results yield evidence for an increase with time…

Strongly Correlated Electrons · Physics 2022-09-29 Natalia Del Fatti , Roland Bouffanais , Fabrice Vallée , Christos Flytzanis

Time-resolved vibrational spectroscopy constitutes an invaluable experimental tool for monitoring hot-carrier induced surface reactions. However, the absence of a full understanding on the precise microscopic mechanisms causing the…

Materials Science · Physics 2019-01-14 D. Novko , J. C. Tremblay , M. Alducin , J. I. Juaristi

Soft x-rays were applied to induce graphitization of diamond through a non-thermal solid-to-solid phase transition. This process was observed within poly-crystalline diamond with a time-resolved experiment using ultrashort soft x-ray pulses…

A low twist angle between the two stacked crystal networks in bilayer graphene enables self-organized lattice reconstruction with the formation of a periodic domain. This superlattice modulates the vibrational and electronic structures,…

Structure-property relationships are the foundation of materials science. Linking microstructure and material properties is essential for predicting material response to driving forces, managing in-service material degradation, and…

Applied Physics · Physics 2019-08-07 Felix Hofmann , Michael P. Short , Cody A. Dennett

The degree of laser-induced graphitisation from a sp3-bonded to a sp2-bonded carbon fraction in a single crystal chemical vapour deposited (CVD) diamond under a varying fluence of an ultrashort pulsed laser (30 fs, 800 nm, 1 kHz)…

Chemical Physics · Physics 2022-03-30 Bakhtiar Ali , Han Xu , Dashavir Chetty , Robert T. Sang , Igor V. Litvinyuk , Maksym Rybachuk

Since graphene has no band gap, photoluminescence is not expected from relaxed charge carriers. We have, however, observed significant light emission from graphene under excitation by ultrashort (30-fs) laser pulses. Light emission was…

Mesoscale and Nanoscale Physics · Physics 2010-09-20 Chun Hung Lui , Kin Fai Mak , Jie Shan , Tony F. Heinz

The influence of laser frequency on laser-driven ion acceleration is investigated by means of two-dimensional particle-in-cell simulations. When ultrashort intense laser pulse at higher harmonic frequency irradiates a thin solid foil, the…

Plasma Physics · Physics 2014-07-29 Jan Psikal , Ondrej Klimo , Stefan Weber , Daniele Margarone

A class of chalcogenide alloy materials that shows significant changes in optical properties upon an amorphous-to-crystalline phase transition has lead to development of large data capacities in modern optical data storage. Among…

Materials Science · Physics 2011-01-13 Kotaro Makino , Junji Tominaga , Muneaki Hase

The absorbed laser energy of a femtosecond laser pulse in a transparent material induces a warm dense matter region which relaxation may lead to structural modifications in the surrounding cold matter. The modeling of the…

Using a combination of ultraviolet-vacuum ultraviolet reflectivity and spectroscopic ellipsometry, we observe a resonant exciton at an unusually high energy of 6.3eV in epitaxial graphene. Surprisingly, the resonant exciton occurs at room…

We review our recent time- and angle-resolved photoemission spectroscopy experiments, which measure the transient electronic structure of optically driven graphene. For pump photon energies in the near infrared…

Materials Science · Physics 2016-08-10 Isabella Gierz , Andrea Cavalleri

Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…

Materials Science · Physics 2010-07-06 Adrian Glaubitz

Graphite is the thermodynamically stable form of carbon, and yet is remarkably difficult to synthesise. A key step in graphite formation is the removal of defects at high temperature ($>$2300~$^{\circ}$C) that allow graphenic fragments to…

Light-induced phenomena in materials can exhibit exotic behavior that extends beyond equilibrium properties, offering new avenues for understanding and controlling electronic phases. So far, non-equilibrium phenomena in solids have been…

Graphene is at the center of a significant research effort. Near-ballistic transport at room temperature and high mobility make it a potential material for nanoelectronics. Its electronic and mechanical properties are also ideal for micro…

Materials Science · Physics 2010-03-03 Z. Sun , T. Hasan , F. Torrisi , D. Popa , G. Privitera , F. Wang , F. Bonaccorso , D. M. Basko , A. C. Ferrari

Collective lattice dynamics determine essential aspects of condensed matter, such as elastic and thermal properties. These exhibit strong dependence on the length-scale, reflecting the marked wavevector dependence of lattice excitations.…

We investigate the ultrafast dynamics of photo-induced non-thermal lattice disorder in a polycrystalline aluminium thin film to elucidate transient short- and long-range lattice distortions, their thermalization and electron-phonon coupling…

Materials Science · Physics 2026-01-06 Fernando Rodriguez Diaz , Kasra Amini