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We present an \textit{ab initio} framework to calculate anharmonic phonon frequency and phonon lifetime that is applicable to severely anharmonic systems. We employ self-consistent phonon (SCPH) theory with microscopic anharmonic force…

Materials Science · Physics 2015-08-20 Terumasa Tadano , Shinji Tsuneyuki

The coupled nonequilibrium dynamics of electrons and phonons in monolayer MoS2 is investigated by combining first-principles calculations of the electron-phonon and phonon-phonon interaction with the time-dependent Boltzmann equation.…

Materials Science · Physics 2021-02-12 Fabio Caruso

We have successfully prepared the new layered oxypnictides $Sr_4Sc_2O_6M_2As_2$ (M=Fe and Co). They adopt the tetragonal structure, being the same as that of $Sr_4Sc_2O_6Fe_2P_2$. The lattice constants are a=0.4045 nm and c= 0.5802 nm for…

Superconductivity · Physics 2015-05-13 Y. L. Xie , R. H. Liu , T. Wu , G. Wu , Y. A. Song , D. Tan , X. F. Wang , H. Chen , J. J. Ying , Y. J. Yan , Q. J. Li , X. H. Chen

We explore the possibility of extracting information about lattice dynamics in simple crystal structures from the neutron pair-density function (PDF) through inverse data analysis. Contrary to the claims by Dimitrov, Louca, and Roeder…

Materials Science · Physics 2011-04-08 Matthias J. Graf , Il-Kyoung Jeong , Daniel L. Starr , R. H. Heffner

We introduce a torsional force field for sp$^2$ carbon to augment an in-plane atomistic potential of a previous work (Kalosakas et al, J. Appl. Phys. {\bf 113}, 134307 (2013)) so that it is applicable to out-of-plane deformations of…

We report inelastic light scattering experiments on CaFe_2As_2 in the temperature range of 4 to 290 K. In in-plane polarizations two Raman-active phonon modes are observed at 189 and 211 cm-1, displaying A_1g and B_1g symmetries,…

Superconductivity · Physics 2009-11-13 K. -Y. Choi , D. Wulferding , P. Lemmens , N. Ni , S. L. Bud'ko , P. C. Canfield

We present an exact real-space renormalization group (RSRG) method for evaluating the dynamic structure factor of an infinite one-dimensional quasiperiodic period-doubling (PD) lattice. We observe that for every normal mode frequency of the…

Condensed Matter · Physics 2009-10-31 Anathnath Ghosh , S. N. Karmakar

The alkali atoms, due to their small sizes and low charge ionic states, are most eligible to intercalate in the structural layers of V2O5. We have applied ab-initio density functional theory to study the dynamics of Li-ion in layers of…

Materials Science · Physics 2019-04-02 Baltej Singh , M. K. Gupta , R. Mittal , S. L. Chaplot

Intrinsic triferroicity is essential and highly sought for novel device applications, such as high-density multistate data storage. So far, the intrinsic triferroicity has only been discussed in three-dimensional systems. Herein on basis of…

Materials Science · Physics 2021-04-14 Shiying Shena , Yandong Ma , Xilong Xu , Baibiao Huang , Liangzhi Kou , Ying Dai

We report measurements of the temperature dependence of phonon densities of states in K0.8Fe1.6Se2 using inelastic neutron scattering technique. While cooling down to 150 K, a phonon peak splitting around 25 meV is observed and a new peak…

Superconductivity · Physics 2015-06-12 R. Mittal , M. K. Gupta , S. L. Chaplot , M. Zbiri , S. Rols , H. Schober , Y. Su , Th. Brueckel , T. Wolf

We report studies on the vibrational and elastic behavior of lithium oxide, Li2O around its superionic transition temperature. Phonon frequencies calculated using the ab-initio and empirical potential model are in excellent agreement with…

Materials Science · Physics 2012-06-04 M. K. Gupta , Prabhatasree Goel , R. Mittal , N. Choudhury , S. L. Chaplot

The mechanical properties of metal-organic frameworks (MOFs) are of high fundamental and also practical relevance. A particularly intriguing technique for determining anisotropic elastic tensors is Brillouin scattering, which so far has…

The recent discovery of superconductivity in oxypnictides with the critical temperature (TC) higher than McMillan limit of 39 K (the theoretical maximum predicted by Bardeen-Cooper-Schrieffer (BCS) theory) has generated great excitement.…

Superconductivity · Physics 2015-05-13 R. H. Liu , T. Wu , G. Wu , H. Chen , X. F. Wang , Y. L. Xie , J. J. Yin , Y. J. Yan , Q. J. Li , B. C. Shi , W. S. Chu , Z. Y. Wu , X. H. Chen

We have performed a first-principles study of the structural and vibrational properties of the three low-pressure (cubic, tetragonal, and especially monoclinic) phases of ZrO2, with special attention to the computation of the zone-center…

Materials Science · Physics 2009-11-07 Xinyuan Zhao , David Vanderbilt

The spectrum of singly-ionized iron (Fe II) has been recorded using high-resolution Fourier transform and grating spectroscopy over the wavelength range 900 {\AA} to 5.5 {\mu}m. The spectra were observed in high-current continuous and…

Instrumentation and Methods for Astrophysics · Physics 2015-03-13 Gillian Nave , Sveneric Johansson

Intriguing lattice dynamics has been predicted for aperiodic crystals that contain incommensurate substructures. Here we report inelastic neutron scattering measurements of phonon and magnon dispersions in Sr14Cu24O41, which contains…

The lattice thermal conductivity (LTC) of ZrSe$_2$, a typical layered transition metal disulfide, has been calculated using a hybrid approach that combines force field molecular dynamics (MD) simulation and Boltzmann transport equation…

Materials Science · Physics 2025-09-10 Yong Lu , Fawei Zheng

We report measurements of the phonon density of states as measured with inelastic x-ray scattering in SmFeAsO$_{1-x}$F$_y$ powders. An unexpected strong renormalization of phonon branches around 23 meV is observed as fluorine is substituted…

Direct manipulation of the atomic lattice using intense long-wavelength laser pulses has become a viable approach to create new states of matter in complex materials. Conventionally, a high frequency vibrational mode is driven resonantly by…

First principles predictions of lattice dynamics are of vital importance for a broad range of topics in materials science and condensed matter physics. The large-scale nature of lattice dynamics calculations and the desire to design novel…

Materials Science · Physics 2023-01-23 Jinliang Ning , James W. Furness , Jianwei Sun