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Interactions among electronic and lattice degrees-of-freedom are foundational to various phases in condensed-matter physics, yet the dynamic interplay between excitonic and phononic quasiparticles represents an equivalent, underexplored…

We estimate the changes in lattice parameters due to iron isotope substitution in the iron-based high temperature superconductors using a variational calculation based on the anharmonicity of the Fe-As(Se) bond. For BaFe2As2 and 57Fe to…

Superconductivity · Physics 2011-09-29 Oleg Kim , Mats Granath

Raman scattering spectra of new Fe-based S=2 spin ladder compound BaFe$_2$Se$_2$O are measured in a temperature range between 15 K and 623 K. All six A$_{1g}$ and two B$_{1g}$ Raman active modes of BaFe$_2$Se$_2$O, predicted by the…

We report inelastic neutron scattering measurements of the magnetic excitations in SrFe2As2, the parent of a family of iron-based superconductors. The data extend throughout the Brillouin zone and up to energies of ~260meV. An analysis with…

Strongly Correlated Electrons · Physics 2011-06-17 R. A. Ewings , T. G. Perring , J. Gillett , S. D. Das , S. E. Sebastian , A. E. Taylor , T. Guidi , A. T. Boothroyd

A simple pseudopotential model is proposed, which allows the phonon spectra and temperature dependence of the lattice heat capacity of Ir and Rh be described with a high enough accuracy. A careful comparison of the calculated and…

Condensed Matter · Physics 2015-06-25 M. I. Katsnelson , I. I. Naumov , A. V. Trefilov , M. N. Khlopkin , K. Yu. Khromov

Infinite-layer (IL) nickelates have rapidly emerged as a new class of superconductors. However, due to the technical challenges of their topotactic synthesis, they have so far been realized primarily as thin films or polycrystalline powder…

The lattice dynamics of members of the M2Mo6Se6 family of materials with guest ions M = K, Rb, Cs, In, and Tl has been studied using inelastic x-ray scattering and Raman spectroscopy at room temperature, as well as by ab-initio…

We have successfully synthesized a new layered iron oxychalcogenide BaFe2OSe2 single crystal. This compound is built up of Ba and Fe-Se(O) layers alternatively stacked along the c-axis. The Fe-Se(O) layers contain double chains of…

Superconductivity · Physics 2015-06-05 Hechang Lei , Hyejin Ryu , John Warren , A. I. Frenkel , V. Ivanovski , B. Cekic , C. Petrovic

The interaction between electrons and lattice vibrations determines key physical properties of materials, including their electrical and heat transport, excited electron dynamics, phase transitions, and superconductivity. We present a new…

Materials Science · Physics 2018-07-04 Luis A. Agapito , Marco Bernardi

We report on first investigation of the lattice dynamics in the novel superconducting material Na$\_{0.35}$CoO$\_2$$\cdot$1.3H$\_2$O and the non-hydrated parent compound Na$\_{0.7}$CoO$\_2$ by inelastic x-ray scattering. The measured phonon…

Strongly Correlated Electrons · Physics 2007-05-23 Jean-Pascal Rueff , M. Calandra , M. D'astuto , Ph. Leininger , A. Shukla , A. Bossak , M. Krisch , H. Ishii , Y. Cai , P. Badica , T. Sasaki , K. Yamada , K. Togano

Here, we present the phonon calculations for thermodynamic properties, thermal expansion and lattice thermal conductivity of Fe$_{2}$VAl in the temperature range of $300-800$ K and compared with existing experiment. Phonon dispersion is…

Materials Science · Physics 2022-07-13 Shamim Sk , Sudhir K. Pandey

The lattice thermal conductivity ($\kappa$) of two ceramic materials, cerium dioxide (CeO$_2$) and magnesium oxide (MgO), is computed up to 1500 K using first principles and the phonon Boltzmann Transport Equation (PBTE) and compared to…

The Breit-Pauli R-matrix method developed under the Iron Project has been used to obtain extensive sets of oscillator strengths and transition probabilities for dipole allowed and intercombination fine structure transitions in carbon like…

Astrophysics · Physics 2009-10-31 Sultana N. Nahar

We successfully synthesized new layered iron oxypnictide Sr2CrO2(FeAs)2 by solid-state-reaction techniques. This is the first report on the Fe-substituted Sr2Mn3As2O2-type oxypnictides to our knowledge. A pellet of stoichiometric mixtures…

We have performaed molecular dynamics simulations of Fe(80)Ni(20) alloys using an inter-atomic potential of the EAM-type which allows the simulation of the martensite-austenite transition. We present results, showing the development of an…

Materials Science · Physics 2008-02-03 R. Meyer , P. Entel

The structural and magnetic phase transitions of the ternary iron arsenides SrFe2As2 and EuFe2As2 were studied by temperature-dependent x-ray powder diffraction and 57-Fe Moessbauer spectroscopy. Both compounds crystallize in the tetragonal…

The phonon dispersion relations of crystal lattices can often be well-described with the harmonic approximation. However, when the potential energy landscape exhibits more anharmonicity, for instance, in case of a weakly bonded crystal or…

Materials Science · Physics 2022-01-19 Jonathan Lahnsteiner , Menno Bokdam

We performed ab initio lattice-dynamics calculations of frame-cluster dodecaborides ZrB12 and LuB12. As a whole, our calculated phonon frequencies and atom-projected density of states are consistent with the results of available…

Chemical Physics · Physics 2019-10-22 N. M. Chtchelkatchev , M. V. Magnitskaya , E. S. Clementyev , P. A. Alekseev

Many theoretical models of iron-based superconductors have been proposed but Tc calculations based on the models are usually missing. We have chosen two models of iron-based superconductors in the literature and then compute the Tc values…

Superconductivity · Physics 2023-07-19 Wong Chi Ho , Rolf Lortz

Rare-earth orthoferrites are a promising platform for antiferromagnetic spintronics with a rich variety of terahertz spin and lattice dynamics phenomena. For instance, it has been experimentally demonstrated that the light-driven optical…