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In many published articles isobaric behavior in DAC chambers has been reported On the other hand, a clear isochoric behavior in the chambers were reported. Thus, Isochoric or isobaric condition remain an open question. In isochoric…

Materials Science · Physics 2023-04-18 Joseph Gal , Lonia Friedlander

High values of deuterium compressibility under shock-wave compression, recently discovered in several experiments, are explained by an unusual dielectric-metal phase transition from a dense molecular gas into a liquid-metal atomic gas. This…

Plasma Physics · Physics 2014-08-27 A. L. Khomkin , A. S. Shumikhin

Solid-solid collapse transition in open framework structures is ubiquitous in nature. The real difficulty in understanding detailed microscopic aspects of such transitions in molecular systems arises from the interplay between different…

Soft Condensed Matter · Physics 2015-06-15 Rakesh S. Singh , Biman Bagchi

The pressure-induced transition of vanadium from BCC to rhombohedral structures is unique and intriguing among transition metals. In this work, the stability of these phases is revisited by using density functional theory. At finite…

Materials Science · Physics 2016-11-07 Yi X. Wang , Q. Wu , Xiang R. Chen , Hua Y. Geng

The moon-forming impact and the subsequent evolution of the proto-Earth is strongly dependent on the properties of materials at the extreme conditions generated by this violent collision. We examine the high pressure behavior of MgO, one of…

We present a systematic trend study of the symmetric tilt grain boundaries about the <110> axis in molybdenum. Our results show that multiple structural phases, some incorporating vacancies, compete for the boundary ground state. We find…

Materials Science · Physics 2007-05-23 D. Yesilleten , T. A. Arias

The nature of freezing and melting transitions for a system of model colloids interacting by a DLVO potential in a spatially periodic external potential is studied using extensive Monte Carlo simulations. Detailed finite size scaling…

Statistical Mechanics · Physics 2009-11-07 W. Strepp , S. Sengupta , P. Nielaba

We present calculations of the free energy, and hence the melting properties, of a simple tight-binding model for transition metals in the region of d-band filling near the middle of a d-series, the parameters of the model being designed to…

Materials Science · Physics 2015-05-13 C. Cazorla , D. Alfè , M. J. Gillan

Melting and freezing transitions in two dimensional systems are known to show highly unusual characteristics. Most of the earlier studies considered atomic systems; the melting behavior in two dimensional molecular solids is still largely…

Materials Science · Physics 2013-02-04 Rakesh S. Singh , Mantu Santra , Biman Bagchi

We have used diffusion quantum Monte Carlo (DMC) calculations to study the pressure-induced phase transition from the diamond to $\beta$-tin structure in silicon. The calculations employ the pseudopotential technique and systematically…

Materials Science · Physics 2016-08-16 D. Alfè , M. J. Gillan , M. D. Towler , R. J. Needs

At ambient pressure tin transforms from its ground-state semi-metal $\alpha$-Sn (diamond structure) phase to the compact metallic $\beta$-Sn phase at 13$^\circ$C (286K). There may be a further transition to the simple hexagonal $\gamma$-Sn…

Aiming to settle the controversial observations for halogen-bridged binuclear transition-metal (MMX) complexes, finite-temperature Hartree-Fock calculations are performed for a relevant two-band Peierls-Hubbard model. Thermal, as well as…

Strongly Correlated Electrons · Physics 2009-11-07 Shoji Yamamoto

We study the low-pressure (0 to 10 GPa) phase diagram of crystalline benzene using quantum Monte Carlo (QMC) and density functional theory (DFT) methods. We consider the $Pbca$, $P4_32_12$, and $P2_1/c$ structures as the best candidates for…

Chemical Physics · Physics 2016-08-23 Sam Azadi , R. E. Cohen

Manganese, in the a-Mn structure, has been studied using synchrotron powder x-ray diffraction in a diamond anvil cell up to 220 GPa at room temperature combined with density functional calculations (DFT). The experiment reveals an extended…

Elemental rare-earth metals provide a playground for studying novel electron correlation effects and complex magnetism. However, ab initio simulations of these systems remain challenging. Here, we employ fully charge self-consistent density…

Strongly Correlated Electrons · Physics 2024-12-23 Wenjun Ding , Yogesh K. Vohra , Cheng-Chien Chen

We present an accurate study of the static-nucleus electronic energy band gap of solid molecular hydrogen at high pressure. The excitonic and quasiparticle gaps of the $C2/c$, $Pc$, $Pbcn$, and $P6_3/m$ structures at pressures of 250, 300,…

Materials Science · Physics 2017-01-25 Sam Azadi , N. D. Drummond , W. M. C. Foulkes

The phase diagram of hydrogen is one of the most important challenges in high-pressure physics and astrophysics. Especially, the melting of dense hydrogen is complicated by dimer dissociation, metallization and nuclear quantum effect of…

Materials Science · Physics 2023-04-25 Hua Y. Geng , Q. Wu

The design of next generation \beta-type titanium implants requires detailed knowledge of the relevant stable and metastable phases at temperatures where metallurgical heat treatments can be performed. Recently, a standard specification for…

Materials Science · Physics 2017-07-26 S. Barzilai , C. Toher , S. Curtarolo , O. Levy

The insulator-to-metal transition in solid helium at high pressure is studied with first-principles simulations. Diffusion quantum Monte Carlo (DMC) calculations predict that the band gap closes at a density of 21.3 g/cc and a pressure of…

Computational Physics · Physics 2008-05-30 Saad Antoun Khairallah , Burkhard Militzer

Solid-solid phase transitions in metals are traditionally driven by changes in density or external pressure. Here we show that, under strong electronic excitation, structural stability is governed by the interplay between electronic effects…

Materials Science · Physics 2026-04-27 S. Azadi , S. M. Vinko , A. Principi , T. D. Kuehne , M. S. Bahramy