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Carbon dioxide (CO$_2$) is one of the most important interstellar molecules. While it is considered that it forms on the surface of interstellar dust grains, the exact contribution of different chemical mechanisms is still poorly…

The final step of the water formation network on interstellar grain surfaces starting from the H + O$_2$ route is the reaction between H and H$_2$O$_2$. This reaction is known to have a high activation energy and therefore at low…

Chemical Physics · Physics 2016-12-01 Thanja Lamberts , Pradipta Kumar Samanta , Andreas Köhn , Johannes Kästner

Formic acid (HCOOH) and carbon dioxide (CO2) are simple species that have been detected in the interstellar medium. The solid-state formation pathways of these species under experimental conditions relevant to prestellar cores are primarily…

Solar and Stellar Astrophysics · Physics 2019-06-26 D. Qasim , T. Lamberts , J. He , K. -J. Chuang , G. Fedoseev , S. Ioppolo , A. C. A. Boogert , H. Linnartz

We present the modeling results of deuterium fractionation of water ice, H2, and the primary deuterium isotopologues of H3+ adopting physical conditions associated with the star and planet formation process. We calculated the deuterium…

Astrophysics of Galaxies · Physics 2015-06-23 Jeong-Eun Lee , Edwin A. Bergin

Interstellar formamide (NH2CHO) has recently attracted significant attention due to its potential role as a molecular building block in the formation of precursor biomolecules relevant for the origin of life. Its formation, whether on the…

Earth and Planetary Astrophysics · Physics 2018-10-09 Albert Rimola , Dimitrios Skouteris , Nadia Balucani , Cecilia Ceccarelli , Joan Enrique-Romero , Vianney Taquet , Piero Ugliengo

Context. Interstellar ice is the main form of metal species in dark molecular clouds. Experiments and observations have shown that the ice is significantly processed after the freeze-out of molecules onto grains. The processing is caused by…

Astrophysics of Galaxies · Physics 2013-06-14 Juris Kalvāns , Ivar Shmeld

Context. The formation of water on the dust grains in the interstellar medium may proceed with hydrogen peroxide (H2O2) as an intermediate. Recently gas-phase H2O2 has been detected in {\rho} Oph A with an abundance of ~1E-10 relative to…

Astrophysics of Galaxies · Physics 2015-06-03 Fujun Du , Berengere Parise , Per Bergman

Water is present during all stages of star formation: as ice in the cold outer parts of protostellar envelopes and dense inner regions of circumstellar disks, and as gas in the envelopes close to the protostars, in the upper layers of…

Solar and Stellar Astrophysics · Physics 2015-06-04 Magnus V. Persson , Jes K. Jørgensen , Ewine F. van Dishoeck

Recent interferometer observations have found that the D2O/HDO abundance ratio is higher than that of HDO/H2O by about one order of magnitude in the vicinity of low-mass protostar NGC 1333-IRAS 2A, where water ice has sublimated. Previous…

Astrophysics of Galaxies · Physics 2016-02-10 K. Furuya , E. F. van Dishoeck , Y. Aikawa

Complex organic molecules (COMs) can be produced by energetic processing of interstellar ice mantles accreted on top of dust grains. Two COMs with proposed energetic ice formation pathways are formamide and acetaldehyde. Both have been…

Solar and Stellar Astrophysics · Physics 2020-05-20 Rafael Martin-Domenech , Karin I. Oberg , Mahesh Rajappan

The ULIRG Mrk 231 exhibits very strong water rotational lines between \lambda = 200-670\mu m, comparable to the strength of the CO rotational lines. High redshift quasars also show similar CO and H2O line properties, while starburst…

Astrophysics of Galaxies · Physics 2015-06-03 R. Meijerink , S. Cazaux , M. Spaans

Many chemical models of dense interstellar clouds predict that the majority of gas-phase elemental nitrogen should be present as N2, with an abundance approximately five orders of magnitude less than that of hydrogen. As a homonuclear…

The interstellar medium is characterized by a rich and diverse chemistry. Many of its complex organic molecules are proposed to form through radical chemistry in icy grain mantles. Radicals form readily when interstellar ices (composed of…

Astrophysics of Galaxies · Physics 2016-09-13 Karin I. Oberg

Ice chemistry in the dense, cold interstellar medium (ISM) is probably responsible for the formation of interstellar complex organic molecules (COMs). Recent laboratory experiments performed at T=4 K have shown that irradiation of CO:N2 ice…

Astrophysics of Galaxies · Physics 2024-01-09 Rafael Martín-Doménech , Alexander DelFranco , Karin I. Öberg , Mahesh Rajappan

The chemical inventory of protoplanetary midplanes is the basis for forming planetesimals. Among them, solid-state reactions based on CO/CO$_2$ toward molecular complexity on interstellar dust grains have been studied in theoretical and…

Solar and Stellar Astrophysics · Physics 2023-10-31 K. -J. Chuang , C. Jaeger , N. -E. Sie , C. -H. Huang , C. -Y. Lee , Y. -Y. Hsu , Th. Henning , Y. -J. Chen

With the advent of JWST ice observations, dedicated studies on the formation reactions of detected molecules are becoming increasingly important. One of the most interesting molecules in interstellar ice is CO$_2$. Despite its simplicity,…

Astrophysics of Galaxies · Physics 2024-10-22 Atsuki Ishibashi , Germán Molpeceres , Hiroshi Hidaka , Yasuhiro Oba , Thanja Lamberts , Naoki Watanabe

Context: The presence of water in the wind of the extreme carbon star IRC+10216 has been confirmed by the Herschel telescope. The regions where the high-J H2O lines have been detected are close to the star at radii r \geq 15 R\ast. Aims: We…

Solar and Stellar Astrophysics · Physics 2011-01-20 Isabelle Cherchneff

Understanding water deuterium fractionation is important for constraining the mechanisms of water formation in interstellar clouds. Observations of HDO and H$_2^{18}$O transitions were carried out towards the high-mass star-forming region…

The successive addition of H atoms to CO in the solid phase has been hitherto regarded as the primary route to form methanol in dark molecular clouds. However, recent Monte Carlo simulations of interstellar ices alternatively suggested the…

Astrophysics of Galaxies · Physics 2022-06-15 Julia C. Santos , Ko-Ju Chuang , Thanja Lamberts , Gleb Fedoseev , Sergio Ioppolo , Harold Linnartz

Infrared spectroscopic observations toward objects obscured by dense cloud material show that H$_2$O, CO and, likely, CO$_2$ are important constituents of interstellar ice mantles. In order to accurately calculate the column densities of…

Astrophysics · Physics 2008-02-03 P. A. Gerakines , W. A. Schutte , J. M. Greenberg , Ewine F. van Dishoeck