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This review paper summarizes the state-of-the-art in laboratory based interstellar ice chemistry. The focus is on atom addition reactions, illustrating how water, carbon dioxide and methanol can form in the solid state at astronomically…

Astrophysics of Galaxies · Physics 2015-07-13 Harold Linnartz , Sergio Ioppolo , Gleb Fedoseev

A recent suggestion that acetamide, \ce{CH3C(O)NH2}, could be readily formed on water-ice grains by the acid induced addition of water across the \ce{CN} bond is now shown to be valid. Computational modelling of the reaction between…

Astrophysics of Galaxies · Physics 2023-07-19 Boutheïna Kerkeni , John M. Simmie

Understanding the formation of molecules under conditions relevant to interstellar chemistry is fundamental to characterize the chemical evolution of the universe. Using reactive molecular dynamics simulations with model-based or…

Chemical Physics · Physics 2021-06-16 Meenu Upadhyay , Marco Pezzella , Markus Meuwly

Dimethyl ether is one of the most abundant interstellar complex organic molecules. Yet its formation route remains elusive. In this work, we have performed electronic structure and kinetics calculations to derive the rate coefficients for…

Context. There are only six molecules containing N-O bond that are detected in gaseous phase in interstellar medium. One of those is nitrous oxide (N2O), which was searched for but not found in solid form from as early as Infrared Space…

Astrophysics of Galaxies · Physics 2026-01-08 V. Karteyeva , R. Nakibov , I. Petrashkevich , M. Medvedev , A. Vasyunin

The study of warm molecular gas in the inner regions of protoplanetary disks is of key importance for the study of planet formation and especially for the transport of H2O and organic molecules to the surfaces of rocky planets/satellites.…

Earth and Planetary Astrophysics · Physics 2014-11-20 R. Meijerink , K. M. Pontoppidan , G. A. Blake , D. R. Poelman , C. P. Dullemond

We investigated the behavior of H$_2$, main constituent of the gas phase in dense clouds, after collision with amorphous solid water (ASW) surfaces, one of the most abundant chemical species of interstellar ices. We developed a general…

Chemical Physics · Physics 2020-03-20 G. Molpeceres , J. Kästner

In molecular clouds at temperatures as low as 10 K, all species except hydrogen and helium should be locked in the heterogeneous ice on dust grain surfaces. Nevertheless, astronomical observations have detected over 150 different species in…

Astrophysics of Galaxies · Physics 2018-10-12 Y. Oba , T. Tomaru , T. Lamberts , A. Kouchi , N. Watanabe

The detection of ozone (O3) in the surface ices of Ganymede, Jupiters largest moon, and of the Saturnian moons Rhea and Dione, has motivated several studies on the route of formation of this species. Previous studies have successfully…

We re-examine the constraints provided by Herschel Space Observatory data regarding cold water emission from protoplanetary disks. Previous disk models that were used to interpret observed water emission concluded that oxygen (O/H) is…

Earth and Planetary Astrophysics · Physics 2024-06-10 Maxime Ruaud , Uma Gorti

The first off-lattice Monte Carlo kinetics model of interstellar dust-grain surface chemistry is presented. The positions of all surface particles are determined explicitly, according to the local potential minima resulting from the…

Instrumentation and Methods for Astrophysics · Physics 2015-06-17 Robin T. Garrod

(Abridged) The water deuterium fractionation (HDO/H$_2$O abundance ratio) has traditionally been used to infer the amount of water brought to Earth by comets. Measuring this ratio in deeply-embedded low-mass protostars makes it possible to…

Solar and Stellar Astrophysics · Physics 2015-06-18 M. V. Persson , J. K. Jørgensen , E. F. van Dishoeck , D. Harsono

Molecular outflows contributing to the matter cycle of star forming galaxies are now observed in small and large systems at low and high redshift. Their physical origin is still unclear. In most theoretical studies only warm ionised/neutral…

Astrophysics of Galaxies · Physics 2021-05-28 Philipp Girichidis , Thorsten Naab , Stefanie Walch , Thomas Berlok

Context: In the laboratory, hydrogen peroxide (HOOH) was proven to be an intermediate product in the solid-state reaction scheme that leads to the formation of water on icy dust grains. When HOOH desorbs from the icy grains, it can be…

Solar and Stellar Astrophysics · Physics 2020-04-29 G. W. Fuchs , D. Witsch , D. Herberth , M. Kempkes , B. Stanclik , J. Chantzos , H. Linnartz , K. Menten , T. F. Giesen

The build-up of galaxies is regulated by a complex interplay between gravitational collapse, galaxy merging and feedback related to AGN and star formation. The energy released by these processes has to dissipate for gas to cool, condense,…

Astrophysics of Galaxies · Physics 2015-10-09 P. Guillard , F. Boulanger , M. D. Lehnert , P. N. Appleton , G. Pineau des Forêts

Cold cores in interstellar molecular clouds represent the very first phase in star formation. The physical conditions of these objects are studied in order to understand how molecular clouds evolve and how stellar masses are determined. The…

Astrophysics · Physics 2009-11-13 J. Harju , M. Juvela , S. Schlemmer , L. K. Haikala , K. Lehtinen , K. Mattila

We report on laboratory measurements of molecular hydrogen formation and recombination on an olivine slab as a function of surface temperature under conditions relevant to those encountered in the interstellar medium. On the basis of our…

Astrophysics · Physics 2009-10-30 V. Pirronello , O. Biham , C. Liu , L. Shen , G. Vidali

We have used a coupled dynamical and chemical model to examine the chemical changes induced by the passage of an interstellar shock in well shielded regions. Using this model we demonstrate that the formation of water in a shock will be…

Astrophysics · Physics 2009-10-31 Edwin A. Bergin , David A. Neufeld , Gary J. Melnick

The origin of Earth oceans is controversial. Earth could have acquired its water either from hydrated silicates (wet Earth scenario) or from comets (dry Earth scenario). [HDO]/[H2O] ratios are used to discriminate between the scenarios.…

Earth and Planetary Astrophysics · Physics 2015-05-14 Wing-Fai Thi , Peter Woitke , Inga Kamp

The abundance of interstellar ice constituents is usually expressed with respect to the water ice because, in denser regions, a significant portion of the interstellar grain surface would be covered by water ice. The binding energy (BE), or…

Astrophysics of Galaxies · Physics 2021-06-01 Ankan Das , Milan Sil , Rana Ghosh , Prasanta Gorai , Soutan Adak , Subhankar Samanta , Sandip K. Chakrabarti
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