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One of the ultimate goals of molecular electronics is to create technologies that will complement - and eventually supersede - Si-based microelectronics technologies. To reach this goal, electronic properties that mimic at least some of the…

Mesoscale and Nanoscale Physics · Physics 2015-06-26 Bingqian Xu , Yonatan Dubi

We present a simple model of electrical transport through a metal-molecule-metal nanojunction that includes charging effects as well as aspects of the electronic structure of the molecule. The interplay of a large charging energy and an…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Matthias H. Hettler , Herbert Schoeller , Wolfgang Wenzel

Using self-consistent calculations based on Non-Equilibrium Green's Function (NEGF) formalism, the origin of negative differential resistance (NDR) in molecular junctions and quantum wires is investigated. Coupling of the molecule to…

Mesoscale and Nanoscale Physics · Physics 2008-08-21 Hosein Cheraghchi , Keivan Esfarjani

A new mechanism is proposed to explain the origin of negative differential resistance (NDR) in a strongly coupled single molecule-metal junction. A first-principles quantum transport calculation in a Fe-terpyridine linker molecule…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Ranjit Pati , Mike McClain , Anirban Bandyopadhyay

Negative differential resistance - a decrease in current with increasing bias voltage - is a counter-intuitive effect that is observed in various molecular junctions. Here, we present a novel mechanism that may be responsible for such an…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Yonatan Dubi

A negative differential resistance (NDR) in the nanotransport is often ascribed to electron correlations. We present a simple example which demonstrates that finite electrode bandwidths and energy dependent electrode density of states are…

Mesoscale and Nanoscale Physics · Physics 2010-05-12 Ioan Baldea , Horst Koppel

Carbon nanotube junctions are predicted to exhibit negative differential resistance, with very high peak-to-valley current ratios even at room temperature. We treat both nanotube p-n junctions and undoped metal-nanotube-metal junctions,…

Condensed Matter · Physics 2009-10-31 F. Leonard , J. Tersoff

A current constrained approach is proposed to calculate negative differential conductance in molecular nano-junctions. A four-site junction is considered where a steady-state current is forced by inserting only the two central sites within…

Mesoscale and Nanoscale Physics · Physics 2016-11-26 Prakash Parida , Swapan K. Pati , Anna Painelli

Combining insights from quantum chemistry calculations with master equations, we discuss a mechanism for negative differential resistance (NDR) in molecular junctions, operated in the regime of weak tunnel coupling. The NDR originates from…

Mesoscale and Nanoscale Physics · Physics 2013-01-10 Martin Leijnse , Wei Sun , Mogens Brøndsted Nielsen , Per Hedegård , Karsten Flensberg

Experimental results showing huge negative differential conductance in gold-hydrogen molecular nanojunctions are presented. The results are analyzed in terms of two-level system (TLS) models: it is shown that a simple TLS model cannot…

Mesoscale and Nanoscale Physics · Physics 2008-02-19 A. Halbritter , P. Makk , Sz. Csonka , G. Mihaly

Electron tunneling through a coupled quantum-dot dimer under a dc-bias is investigated. We find that a peak in the $I$-$V$ curve appears at low temperature when two discrete electronic states in the two quantum dots are aligned with each…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 S. D. Wang , Z. Z. Sun , N. Cue , X. R. Wang

We have calculated current-voltage characteristic curves for normal-superconducting junctions with Andreev reflections and different types of electronic bands. We found that when the normal band is narrow, of the order of the…

Superconductivity · Physics 2009-03-13 N. García , P. Esquinazi

We unravel the critical role of vibrational mode softening in single-molecule electronic devices at high bias. Our theoretical analysis is carried out with a minimal model for molecular junctions, with mode softening arising due to…

Mesoscale and Nanoscale Physics · Physics 2020-08-18 Junjie Liu , Dvira Segal

We present first-principles calculations on electron transport through Na nanowires at finite bias voltages. The nanowire exhibits a nonlinear current-voltage characteristic and negative differential conductance. The latter is explained by…

Materials Science · Physics 2016-08-31 Shigeru Tsukamoto , Kikuji Hirose

The interplay between the electron transport in metal/ferroelectric/metal junctions with ultrathin ferroelectric barriers and the polarization state of a barrier is investigated. Using a model which takes into account screening of…

Other Condensed Matter · Physics 2009-11-11 M. Ye. Zhuravlev , R. F. Sabirianov , S. S. Jaswal , E. Y. Tsymbal

Negative differential resistance (NDR) is tuned at junctions of electronically different dimer and trimer of Rose Bengal on an atomic flat gold (111) surface. Isolated molecule did not show any NDR. But it was induced to show double NDR…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Anirban Bandyopadhyay , Y. Wakayama

Negative differential conductance (NDC) is expected to be an essential property to realize fast switching in future electronic devices. We here present a thorough analysis on electron transportability of a simple atomic-scale model…

Materials Science · Physics 2009-11-07 Shigeru Tsukamoto , Masakazu Aono , Kikuji Hirose

Nonlinear electrical properties, such as negative differential resistance (NDR), are essential in numerous electrical circuits, including memristors. Several physical origins have been proposed to lead to the NDR phenomena in semiconductor…

Negative differential conductivity (NDC) is a widely exploited effect in modern electronic components. Here, a proof-of-principle is given for the observation of NDC in a quantum transport device for neutral atoms employing a multi-mode…

Quantum Gases · Physics 2017-08-24 Ralf Labouvie , Bodhaditya Santra , Simon Heun , Sandro Wimberger , Herwig Ott

We investigate the effect on molecular transport due to the different structural aspects of metal-molecule interfaces. The example system chosen is the prototypical molecular device formed by sandwiching the phenyl dithiolate molecule (PDT)…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Yongqiang Xue , Mark Ratner
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