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We report cooperative magnetic orderings in a 6H-perovskite multiferroic system, Ba3HoRu2O9, via comprehensive neutron powder diffraction measurements. This system undergoes long-range antiferromagnetic ordering at TN1 ~ 50 K with a…

Strongly Correlated Electrons · Physics 2020-07-29 T. Basu , V. Caignaert , F. Damay , T. W. Heitmann , B. Raveau , X. Ke

We present a novel multiferroic double perovskite compound, CaZnFeOsO$_6$ (CZFOO), exhibiting combined ferroelectric and ferrimagnetic properties. Through ab initio density functional theory calculations, we predict CZFOO as a unique…

Materials Science · Physics 2024-08-22 Deepti Rajpoot , Paresh C. Rout , Nikita Acharya , Varadharajan Srinivasan

Investigation of the oxygen-deficient 112-type ordered oxides of the type LnBaCoMnO5+\delta (Ln = Nd, Eu) evidences certain unusual magnetic behavior at low temperatures, compared to the LnBaCo2O5+\delta cobaltites. One observes that the…

Materials Science · Physics 2015-05-18 Asish K. Kundu , V. Pralong , B. Raveau , V. Caignaert

SmFeO3 has attracted considerable attention very recently due to the reported multiferroic properties above room-temperature. We have performed powder and single crystal neutron diffraction as well as complementary polarization dependent…

A metastable perovskite BiFe0.5Sc0.5O3 synthesized under high-pressure (6 GPa) and high- temperature (1500 K) conditions was obtained in two different polymorphs, antipolar Pnma and polar Ima2, through an irreversible behaviour under a…

Layers of perovskites, found in 3D materials, 2D heterostructures, and nanotubes, often distort from high symmetry to facilitate dipole polarisation that is exploitable in many applications. Using density-functional theory calculations,…

Materials Science · Physics 2025-11-14 Shaowen Xu , Jeffrey R. Reimers , Fanhao Jia , Wei Ren

New double perovskites LaPbMSbO6, where M2+ = Mn2+, Co2+, and Ni2+, were synthesized as polycrystals by an aqueous synthetic route at temperatures below 1000 oC. All samples are monoclinic, space group P21/n, as obtained from Rietveld…

Materials Science · Physics 2013-03-11 D. G. Franco , R. E. Carbonio , G. Nieva

Using first-principles density functional theory we predict a ferroelectric ground state -- driven by off-centering of the magnetic Mn$^{4+}$ ion -- in perovskite-structure BaMnO$_3$. Our finding is surprising, since the competition between…

Materials Science · Physics 2009-05-28 James M. Rondinelli , Aaron S. Eidelson , Nicola A. Spaldin

There is great interest in hybrid organic-inorganic materials such as metal-organic frameworks (MOFs). The compounds [C(NH$_{2}$)$_{3}$]M(HCOO)$_{3}$, where M=Cu$^{2+}$ or Cr$^{2+}$ are Jahn-Teller (JT) active ions, are MOF with perovskite…

Materials Science · Physics 2014-03-27 Alessandro Stroppa , Paolo Barone , Prashant Jain , Jean Manuel Perez-Mato , Silvia Picozzi

Several M3 TeO6 (M = Mn, Co, Ni, Cu) oxides order antiferromagnetically at low temperatures (near or below 60 K), while displaying interesting dielectric properties at high temperatures (ferroelectricity below 1000 K in M = Ni case). We…

Strongly Correlated Electrons · Physics 2013-08-27 R. Mathieu , S. A. Ivanov , P. Nordblad , M. Weil

The electronic valence state of Mn in Pb(Zr0.2Ti0.8)O3/La0.8Sr0.2MnO3 multiferroic heterostructures is probed by near edge x-ray absorption spectroscopy as a function of the ferroelectric polarization. We observe a temperature independent…

Materials Science · Physics 2010-04-13 C. A. F. Vaz , J. Hoffman , Y. Segal , J. W. Reiner , R. D. Grober , Z. Zhang , C. H. Ahn , F. J. Walker

Cross-coupling of ordering parameters in multiferroic materials by multiple external stimuli other than electric field and magnetic field is highly desirable from both practical application and fundamental study points of view. Recently,…

Materials Science · Physics 2016-09-27 Tingting Jia , Hideo Kimura , Zhenxiang Cheng , Hongyang Zhao

The search for room-temperature magnetocaloric materials for refrigeration has led to investigations of double perovskites. In particular, a puzzle has appeared in the La$_2$MnNiO$_6$, La$_2$MnCoO$_6$ and La$_2$MnFeO$_6$ family of…

Strongly Correlated Electrons · Physics 2019-03-04 C. Gauvin-Ndiaye , T. E. Baker , P. Karan , É. Massé , M. Balli , N. Brahiti , M. A. Eskandari , P. Fournier , A. -M. S. Tremblay , R. Nourafkan

High quality epitaxial thin films of LaBiMn4/3Co2/3O6 perovskite were fabricated on (001)-oriented SrTiO3 and LaAlO3 substrates by the pulsed laser deposition technique. Magnetization measurements reveal a strong magnetic anisotropy and a…

Materials Science · Physics 2008-02-18 R. Ranjith , Asish K. Kundu , M. Filippi , B. Kundys , W. Prellier , B. Raveau , J. Laverdiere , M. P. Singh , S. Jandl

Hexagonal rare-earth ferrite RFeO$_3$ family represents a unique class of multiferroics exhibiting weak ferromagnetism, and a strong coupling between magnetism and structural trimerization is predicted. However, the hexagonal structure for…

We have deployed density functional theory, Wannier function analysis and mean-field calculations to investigate the double-double perovskite compound CaMnCrSbO_{6}. The crystallographically non-equivalent Mn atoms in the unit cell have…

Materials Science · Physics 2022-06-14 Rakshanda Dhawan , Padmanabhan Balasubramanian , Tashi Nautiyal

We investigate in this paper magnetic properties of the perovskite compound (La0.56Ce0.14)Sr0.30MnO3. The method we use here is Monte Carlo simulation, in which we take into account different kinds of interactions between nearest and…

Strongly Correlated Electrons · Physics 2016-08-24 Samia Yahyaoui , H. T. Diep

Quadruple perovskites ACu$_3$Fe$_2$Re$_2$O$_{12}$ attract considerable interest due to their high Curie temperatures (up to $710$K), which strongly depend on the A-site cation. In this work, we employ first-principles calculations to…

Erbium orthochromite, ErCrO3, is a distorted-perovskite which has antiferromagnetic ground state below 10 K while Cr3+ magnetic moments order at 133 K. The temperature dependence of magnetization is studied across different magnetic phases…

Strongly Correlated Electrons · Physics 2015-01-29 Brajesh Tiwari , M Krishna Surendra , M. S. Ramachandra Rao

The 5d5 iridate CaIrO3 is isostructural with the post-perovskite phase of MgSiO3, recently shown to occur under extreme pressure in the lower Earth's mantle. It therefore serves as an analogue of post-perovskite MgSiO3 for a wide variety of…

Strongly Correlated Electrons · Physics 2012-07-05 Nikolay A. Bogdanov , Vamshi M. Katukuri , Hermann Stoll , Jeroen van den Brink , Liviu Hozoi