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An orbital ordering occurs in many transition metal compounds with Jahn-Teller ions and plays an important role in these materials. At the same time, exchange interactions in orbitally degenerate systems are inherently frustrated, even in…

Strongly Correlated Electrons · Physics 2009-11-10 Daniel Khomskii , Maxim Mostovoy

Spin wave excitations were measured in the ferromagnetic phase of Nd$_{1/2}$Sr$_{1/2}$MnO$_{3}$ by neutron scattering. This compound is located in proximity to the A-type antiferromagnetic state, and it shows a clear anisotropy and…

Strongly Correlated Electrons · Physics 2009-10-31 R. Kajimoto , H. Yoshizawa , H. Kawano-Furukawa , H. Kuwahara , Y. Tomioka , Y. Tokura

Motivated by recent experiments, we present a comprehensive theoretical study of the geometrically frustrated strongly correlated magnetic insulator Mn$_3$O$_4$ spinel oxide based on a microscopic Hamiltonian involving lattice, spin and…

Strongly Correlated Electrons · Physics 2017-08-23 Santanu Pal , Siddhartha Lal

Resonant soft x-ray diffraction has been used to probe the temperature dependent orbital and magnetic structure of $\mathrm{LaSr_{2}Mn_{2}O_7}$. Previous crystallographic studies have shown that this material has almost no MnO$_{6}$ oxygen…

Strongly Correlated Electrons · Physics 2007-05-23 S. B. Wilkins , N. Stojic , T. A. W. Beale , N. Binggeli , P. Bencok , S. Stanescu , J. F. Mitchell , P. Abbamonte , P. D. Hatton , M. Altarelli

Spin correlations in metallic and insulating phases of $V_2O_3$ and its derivatives are investigated using magnetic neutron scattering. Metallic samples have incommensurate spin correlations varying little with hole doping. Paramagnetic…

Strongly Correlated Electrons · Physics 2009-10-28 Wei Bao , C. Broholm , G. Aeppli , P. Dai , J. M. Honig , P. Metcalf

We employ the combination of the density functional and the dynamical mean-field theory (LDA+DMFT) to investigate the electronic structure and magnetic properties of SrCoO3, monocrystal of which were prepared recently. Our calculations lead…

Strongly Correlated Electrons · Physics 2012-09-25 J. Kuneš , V. Křápek , N. Parragh , G. Sangiovanni , A. Toschi , A. V. Kozhevnikov

Single crystals of electron-doped SrMnO3 with a cubic perovskite structure have been systematically investigated as the most canonical (orbital-degenerate) double-exchange system, whose ground states have been still theoretically…

Strongly Correlated Electrons · Physics 2015-05-20 H. Sakai , S. Ishiwata , D. Okuyama , A. Nakao , H. Nakao , Y. Murakami , Y. Taguchi , Y. Tokura

Magnetic and orbital structures in KCuF$_{3}$ are revisited by the cluster self-consistent field approach developed recently. We clearly showed that due to the inherent frustration, the ground state of the system with the superexchange and…

Strongly Correlated Electrons · Physics 2007-05-23 Dong-Meng Chen , Liang-Jian Zou

We study the ground-state properties of a spin-1 Heisenberg model on a square lattice with the first- and second-nearest-neighbor antiferromagnetic couplings $J_1$ and $J_2$ and a three-spin scalar chirality term $J_\chi$. Using the density…

Strongly Correlated Electrons · Physics 2022-04-06 Yixuan Huang , W. Zhu , Shou-Shu Gong , Hong-Chen Jiang , D. N. Sheng

We report a new tetragonal ground-state for perovskite-structured PbCrO3 from DFT+U calculations, and explain its anomalously large volume. The new structure is stabilized due to orbital ordering of Cr-d in the presence of a large…

Materials Science · Physics 2015-05-27 P. Ganesh , R. E. Cohen

The orbital, lattice, and spin ordering phenomena in KCuF3 are investigated by means of LDA+U calculations, based on ab-initio pseudopotentials.We examine the Cu-3d orbital ordering and the associated Jahn-Teller distortion in several…

Strongly Correlated Electrons · Physics 2009-11-10 N. Binggeli , M. Altarelli

Using density functional theory we investigate the lattice instability and electronic structure of recently discovered ferroelectric metal LiOsO$_3$. We show that the ferroelectric-like lattice instability is related to the Li-O distortion…

Materials Science · Physics 2015-03-19 Gianluca Giovannetti , Massimo Capone

The 6H-perovskite Ba3RRu2O9 (R = rare-earth), composed of Ru2O9 dimers connected through RO6 octahedra, exhibits an intriguing variety of magnetic ground states, ranging from non-magnetic to ferromagnetic and antiferromagnetic, depending on…

Materials Science · Physics 2025-06-13 E. Kushwaha , G. Roy , A. M. dos Santos , M. Kumar , S. Ghosh , T. Heitmann , T. Basu

We present a theory of spin and orbital states in Mott insulator $LaTiO_3$. The spin-orbital superexchange interaction between $d^1(t_{2g})$ ions in cubic crystal suffers from a pathological degeneracy of orbital states at classical level.…

Strongly Correlated Electrons · Physics 2009-10-31 G. Khaliullin , S. Maekawa

Motivated by the absence of cooperative Jahn-Teller effect and of magnetic ordering in LiNiO$_2$, a layered oxide with triangular planes, we study a general spin-orbital model on the triangular lattice. A mean-field approach reveals the…

Strongly Correlated Electrons · Physics 2009-11-10 F. Vernay , K. Penc , P. Fazekas , F. Mila

Ground-state properties of layered nickelates are investigated based on the orbital-degenerate Hubbard model coupled with lattice distortions, by using umerical techniques. The N\'eel state composed of spin S=1 ions is confirmed in the…

Strongly Correlated Electrons · Physics 2009-11-10 Takashi Hotta , Elbio Dagotto

We study theoretically low-temperature phases of a recently synthesized compound Sr$_2$CoO$_3$F under pressure. The analysis combining LDA+DMFT and a strong-coupling effective model points to the existence of not only normal paramagnetic…

Strongly Correlated Electrons · Physics 2019-05-15 Juan Fernández Afonso , Andrii Sotnikov , Atsushi Hariki , Jan Kuneš

Different types of order are discussed in the context of strongly correlated transition metal oxides, involving pure compounds and $3d^{3}-4d^{4}$ and $3d^{2}-4d^{4}$ hybrids. Apart from standard, long-range spin and orbital orders we…

Strongly Correlated Electrons · Physics 2019-10-24 Wojciech Brzezicki

Frustration refers to competition between different interactions that cannot be simultaneously satisfied, a familiar feature in many magnetic solids. Strong frustration results in highly degenerate ground states, and a large suppression of…

Strongly Correlated Electrons · Physics 2007-07-03 Doron Bergman , Jason Alicea , Emanuel Gull , Simon Trebst , Leon Balents

Crystal and magnetic structures of the high-pressure stabilized perovskite phase of TlMnO3 have been studied by neutron powder diffraction. The crystal structure involves two types of primary structural distortions: a+b-b-octahedral tilting…

Strongly Correlated Electrons · Physics 2019-03-07 Dmitry D. Khalyavin , Pascal Manuel , Wei Yi , Alexei A. Belik