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In this work, we devise a fast and effective nuclear spin hyperpolarization scheme, which is in principle magnetic field and temperature independent. We use this scheme to experimentally demonstrate polarizations of up to 66% for phosphorus…

We demonstrate that the dynamic nuclear polarization (DNP) of phosphorus donors in silicon can be very effective in a magnetic field of 4.6 T and at temperatures below 1 K. The DNP occurs due to the Overhauser effect following a cross…

We demonstrate a method which can hyperpolarize both the electron and nuclear spins of 31P donors in Si at low field, where both would be essentially unpolarized in equilibrium. It is based on the selective ionization of donors in a…

We present the results of experiments on dynamic nuclear polarization and relaxation of 75As in silicon crystals. Experiments are performed in strong magnetic fields of 4.6 T and temperatures below 1 K. At these conditions donor electron…

Materials Science · Physics 2016-11-15 J. Järvinen , J. Ahokas , S. Sheludyakov , O. Vainio , L. Lehtonen , S. Vasiliev , D. Zvezdov , L. Vlasenko

Optically polarizable nitrogen-vacancy (NV) center in diamond enables the hyperpolarization of $^{13}$C nuclear spins at low magnetic field and room temperature. However, achieving a high level of polarization comparable to conventional…

Quantum Physics · Physics 2024-10-01 Vladimir V. Kavtanyuk , Changjae Lee , Keunhong Jeong , Jeong Hyun Shim

Single crystal silicon is an excellent system in which to explore dynamic nuclear polarization (DNP), as it exhibits a continuum of properties from metallic to insulating as a function of doping concentration and temperature. At low doping…

Materials Science · Physics 2011-09-09 Anatoly E. Dementyev , David G. Cory , Chandrasekhar Ramanathan

Coupled electron-nuclear spins represent a promising quantum system, where the optically induced electron spin polarization can be dynamically transferred to nuclear spins via the hyperfine interaction. Most experiments on dynamic nuclear…

Materials Science · Physics 2026-01-13 A. N. Anisimov , A. V. Poshakinskiy , G. V. Astakhov

Donor spins in silicon are some of the most promising qubits for upcoming solid-state quantum technologies. The nuclear spins of phosphorus donors in enriched silicon have among the longest coherence times of any solid-state system as well…

Nuclear spin hyperpolarization provides a promising route to overcome the challenges imposed by the limited sensitivity of nuclear magnetic resonance. Here we demonstrate that dissolution of spin-polarized pentacene-doped naphthalene…

Dynamic nuclear polarization transfers spin polarization from electrons to nuclei. We have achieved this by a new method, simultaneously exciting transitions of electronic and nuclear spins. The efficiency of this technique improves with…

Quantum Physics · Physics 2008-09-11 G. W. Morley , K. Porfyrakis , A. Ardavan , J. van Tol

We experimentally demonstrate the inductive readout of optically hyperpolarized phosphorus-31 donor nuclear spins in an isotopically enriched silicon-28 crystal. The concentration of phosphorus donors in the crystal was 1.5 x 10$^{15}$…

We investigate the dynamic polarization of nuclear spins in a nominally undoped GaAs/Al$_{0.35}$Ga$_{0.65}$As quantum well using two complementary experimental approaches: time-resolved Kerr rotation and optical orientation measurements of…

Mesoscale and Nanoscale Physics · Physics 2025-12-24 M. Kotur , D. Kudlacik , N. E. Kopteva , E. Kirstein , D. R. Yakovlev , K. V. Kavokin , M. Bayer

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

We demonstrate the coherent control and electrical readout of the nuclear spins of ionized phosphorus donors in natural silicon. By combining pulsed illumination with coherent electron spin manipulation, we selectively ionize the donor…

Materials Science · Physics 2012-01-17 Lukas Dreher , Felix Hoehne , Martin Stutzmann , Martin S. Brandt

The electron-nuclei (hyperfine) interaction is central to spin qubits in solid state systems. It can be a severe decoherence source but also allows dynamic access to the nuclear spin states. We study a double quantum dot exposed to an…

Mesoscale and Nanoscale Physics · Physics 2013-06-13 Gunnar Petersen , Eric A. Hoffmann , Dieter Schuh , Werner Wegscheider , Geza Giedke , Stefan Ludwig

We use above-bandgap optical excitation, via a 1047 nm laser, to hyperpolarize the $^{31}$P spins in low-doped (N$_D =6\times10^{15}$ cm$^{-3}$) natural abundance silicon at 4.2 K and 6.7 T, and inductively detect the resulting NMR signal.…

Mesoscale and Nanoscale Physics · Physics 2018-11-21 P. Gumann , H. Haas , S. Sheldon , L. Zhu , M. L. W. Thewalt , D. G. Cory , C. Ramanathan

Pulsed electrically-detected magnetic resonance of phosphorous (31P) in bulk crystalline silicon at very high magnetic fields (B > 8.5 T) and low temperatures (T = 2.8 K) is presented. We find that the spin-dependent capture and reemission…

Quantum Physics · Physics 2009-09-25 G. W. Morley , D. R. McCamey , H. A. Seipel , L. -C. Brunel , J. van Tol , C. Boehme

We report hyperpolarization of the electronic spins associated with substitutional nitrogen defects in bulk diamond crystal. Hyperpolarization is achieved by optical pumping of nitrogen vacancy centers followed by rapid cross relaxation at…

Mesoscale and Nanoscale Physics · Physics 2017-02-22 M. Loretz , H. Takahashi , T. F. Segawa , J. M. Boss , C. L. Degen

In systems with spin-momentum locking, such as the surface states of three-dimensional topological insulators, a charge current is spin-polarized and spin-flip interactions between electron and nuclear spins can transfer this polarization…

Mesoscale and Nanoscale Physics · Physics 2025-06-18 Sofie Kölling , İnanç Adagideli , Alexander Brinkman

We polarize nuclear spins in a GaAs double quantum dot by controlling two-electron spin states near the anti-crossing of the singlet (S) and m_S=+1 triplet (T+) using pulsed gates. An initialized S state is cyclically brought into resonance…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. R. Petta , J. M. Taylor , A. C. Johnson , A. Yacoby , M. D. Lukin , C. M. Marcus , M. P. Hanson , A. C. Gossard
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