Related papers: Tomographic femtosecond X-ray diffractive imaging
Through examining the product of the mathematical variance of intensity with respect to time and frequency, we arrive at a temporal characterization of laser pulses through parameters for pulse duration, group delay dispersion and temporal…
We present a simple method and its experimental implementation to completely determine the characteristics of the pump-and-probe pulse and the Stokes pulse in a coherent anti-Stokes Raman scattering microscope at sample level without…
Focusing control of ultrashort pulsed beams is an important research topic, due to its impact to subsequent interaction with matter. In this work, we study the propagation near the focus of ultrashort laser pulses of ~25 fs duration under…
We propose a method for a straightforward characterization of the temporal shape of femtosecond pulses in the extreme-ultraviolet/soft X-ray spectral region. The approach is based on the presence of a significant linear frequency chirp in…
Tomography is the three-dimensional reconstruction of an object from images taken at different angles. The term classical tomography is used, when the imaging beam travels in straight lines through the object. This assumption is valid for…
Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…
We present a simple apparatus for femtosecond laser induced generation of X-rays. The apparatus consists of a vacuum chamber containing an off-axis parabolic focusing mirror, a reel system, a debris protection setup, a quartz window for the…
Recently, two novel techniques for the extraction of the phase-shift map (Tomassini {\it et.~al.}, Applied Optics {\bf 40} 35 (2001)) and the electronic density map estimation (Tomassini P. and Giulietti A., Optics Communication {\bf 199},…
We consider the multi-target detection problem of estimating a two-dimensional target image from a large noisy measurement image that contains many randomly rotated and translated copies of the target image. Motivated by single-particle…
X-rays are commonly used in imaging experiments due to their penetration power, which enables non-destructive resolution of internal structures in samples that are opaque to visible light. Time-resolved X-ray tomography is the…
The routine atomic-resolution structure determination of single particles is expected to have profound implications for probing the structure-function relationship in systems ranging from energy materials to biological molecules.…
All-optical Compton sources are innovative, compact devices to produce high energy femtosecond X-rays. Here we present results on a single-pulse scheme that uses a plasma mirror to reflect the drive beam of a laser plasma accelerator and to…
A method for extracting the dark-field signal in propagation-based phase-contrast imaging is proposed. In the case of objects consisting predominantly of a single material, or several different materials with similar ratios of the real…
We report an original method allowing to recover the temporal profile of any kind of soft X-ray laser pulse in single-shot operation. We irradiated a soft X-ray multilayer mirror with an intense infrared femtosecond laser pulse in a…
We experimentally demonstrate that pairs of time-delayed ultrabright and ultrashort X-ray pulses of two different colors, delivered by modern X-ray Free Electron Lasers, can provide two time-delayed snapshots of a sample. We introduce…
Self diffraction is a four-wave mixing process proportional to the square modulus of third-order nonlinearity susceptibility $\chi^{(3)}$, which is related to the material's electronic and thermal properties. In this study, we investigate…
Sub-angstrom spatial resolution of electron density coupled with sub-femtosecond temporal resolution is required to directly observe the dynamics of the electronic structure of a molecule after photoinitiation or some other ultrafast…
X-ray free-electron lasers (XFELs) of high brightness have opened new opportunities for exploring ultrafast dynamical processes in matter, enabling imaging and movies of single molecules and particles at atomic resolution. In this paper, we…
Synchronising ultra-short (~fs) and focussed laser pulses is a particularly difficult task, as this timescale lies orders of magnitude below the typical range of fast electronic devices. Here we present an optical technique that allows for…
This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray Free-Electron Laser. We present results of…