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This study investigates the emission of cations from silica samples by single-cycle THz pulses, focusing on the influence of pulse polarity. Negative THz pulses were found to efficiently trigger the evaporation of cations from nanoneedles…

Silicon nanocrystals (Si NCs) have shown great promise for electroluminescent and photoluminescent applications. In order to optimize the properties of Si NC devices, however, electronic transport in Si NCs films needs to be thoroughly…

Mesoscale and Nanoscale Physics · Physics 2014-09-02 Ting Chen , Brian Skinner , Wei Xie , B. I. Shklovskii , Uwe R. Kortshagen

Electronic and optoelectronic devices based on thin films of carbon nanotubes are currently limited by the presence of metallic nanotubes. Here we present a novel approach based on nanotube alkyl functionalization to physically remove the…

Net atomic charges (NACs) are widely used in all chemical sciences to concisely summarize key information about the partitioning of electrons among atoms in materials. Although widely used, there is currently no atomic population analysis…

Chemical Physics · Physics 2015-12-29 Thomas A. Manz , Nidia Gabaldon Limas

The transport of low-energy electrons through the coating of a radiosensitizing metallic nanoparticle under fast ion irradiation is analyzed theoretically and numerically. As a case study, we consider a poly(ethylene glycol)-coated gold…

Atomic and Molecular Clusters · Physics 2018-06-26 Kaspar Haume , Pablo de Vera , Alexey Verkhovtsev , Eugene Surdutovich , Nigel J. Mason , Andrey V. Solov'yov

It has been shown that to calculate the parameters of the electrostatic field of the ion crystal lattice it sufficient to take into account ions located at a distance of 1-2 lattice spacings. More distant ions make insignificant…

General Physics · Physics 2010-01-26 Alexander Ivanchin

When plasmonic nanoparticles are coupled with semiconductors, highly energetic hot carriers can be extracted from the metal-semiconductor interface for various applications in light energy conversion. Hot charge-carrier extraction upon…

Generation of energetic (hot) electrons is an intrinsic property of any plasmonic nanostructure under illumination. Simultaneously, a striking advantage of metal nanocrystals over semiconductors lies in their very large absorption cross…

Mesoscale and Nanoscale Physics · Physics 2017-08-31 Lucas V. Besteiro , Xiang-Tian Kong , Zhiming Wang , Gregory V. Hartland , Alexander O. Govorov

Alkali metal dimers attached to the surface of helium nanodroplets are found to be efficiently doubly ionized by electron transfer-mediated decay (ETMD) when photoionizing the helium droplets. This process is evidenced by detecting in…

Single-walled carbon nanotubes are strongly correlated systems with large Coulomb repulsion between two electrons occupying the same $p_z$ orbital. Within a molecular Hamiltonian appropriate for correlated $\pi$-electron systems, we show…

Materials Science · Physics 2009-02-15 Zhendong Wang , Demetra Psiachos , Roberto F. Badilla , Sumit Mazumdar

Ionization of highly charged relativistic ions by neutral atoms and ions is considered. Numerical results of recently developed computer codes based on the relativistic Born and the equivalent-photon approximations are presented. The…

Atomic Physics · Physics 2013-05-29 G. Baur , I. L. Beigman , V. P Shevelko , I. Yu. Tolstikhina , Th. Stoehlker

We demonstrate the ability to load, cool and detect singly-charged calcium ions in a surface electrode trap using only visible and infrared lasers for the trapped-ion control. As opposed to the standard methods of cooling using…

Atomic Physics · Physics 2017-07-27 F. Lindenfelser , M. Marinelli , V. Negnevitsky , S. Ragg , J. P. Home

Anion and cation emission following water dissociation was studied for 6.6-keV $^{16}$O$^{+}$ + H$_{2}$O collisions. Absolute cross sections for the emission of all positively and negatively charged fragments, differential in both energy…

Charge-coupled devices (CCDs) are a leading technology in direct dark matter searches because of their eV-scale energy threshold and high spatial resolution. The sensitivity of future CCD experiments could be enhanced by distinguishing…

Charge transfer in collisions of Na_n^+ cluster ions with Cs atoms is investigated theoretically in the microscopic framework of non-adiabatic quantum molecular dynamics. The competing reaction channels and related processes affecting the…

Atomic and Molecular Clusters · Physics 2007-05-23 O. Knospe , J. Jellinek , U. Saalmann , R. Schmidt

We demonstrate the possiblity to cool nanoelectronic systems in nonequilibrium situations by increasing the temperature of the environment. Such cooling by heating is possible for a variety of experimental conditions where the relevant…

Mesoscale and Nanoscale Physics · Physics 2018-08-15 R. Härtle , C. Schinabeck , M. Kulkarni , D. Gelbwaser-Klimovsky , M. Thoss , U. Peskin

We propose a new class of nanoscale electro-optical traps for neutral atoms. A prototype is the toroidal trap created by a suspended, charged carbon nanotube decorated with a silver nanosphere dimer. An illuminating laser field, blue…

Atomic Physics · Physics 2009-02-01 Brian Murphy , Lene Vestergaard Hau

The study of cold and controlled molecular ions is pivotal for fundamental research in modern physics and chemistry. Investigations into cooling molecular anions, in particular, have proven to be of key consequence for the production of…

The F' center in an alkali halide forms when an anion vacancy traps two electrons which is the prerequisite of a diatomic molecule. Indeed, the center may displace left or right along <110> in a (110) plane, due to its coupling to the…

Materials Science · Physics 2007-05-23 Mladen Georgiev

Advancing new ideas of rechargeable batteries represents an important path to meeting the ever increasing energy storage needs. Recently we showed rechargeable sodium/chlorine (Na/Cl$_2$) (or lithium/chlorine Li/Cl$_2$) batteries that used…

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