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Tunneling between the two lowest energy levels of single molecule magnets with Ising type anisotropy, accompanied by the emission or absorption of phonons, is considered. Quantitatively accurate calculations of the rates for such tunneling…

Mesoscale and Nanoscale Physics · Physics 2015-10-05 Yun Liu , Anupam Garg

First-principles calculations are used to gauge different levels of approximation to calculate the magnetocrystalline anisotropy energies (MAE) of five $L1_0$ FeMe alloys (Me=Co, Cu, Pd, Pt, Au). We find that a second-order perturbation…

Materials Science · Physics 2020-12-14 M. Blanco-Rey , J. I. Cerda , A. Arnau

The realization of spin based devices is one of the most aspiring goals of spintronics research. Single molecule magnets are an important class of nanoscale magnetic systems with potential to realize different spintronic devices where each…

The magnetocrystalline anisotropy energies (MAEs) of the ferromagnetic metals bcc Fe, fcc and hcp Co, and fcc Ni have been calculated by using the {\it ab initio} tight-binding method. Disentangling the strong correlation among the $d$…

Materials Science · Physics 2009-11-10 Yuannan Xie , John A. Blackman

An effective spin model for Mott insulators is determined by the symmetries involved among magnetic sites, electron fillings, and their interactions. Such a spin Hamiltonian offers insight to mechanisms of magnetic orders and magnetic…

Strongly Correlated Electrons · Physics 2022-08-05 Xiaoyu Liu , Derek Churchill , Hae-Young Kee

The effect of a measurement time duration on the parameters of magnetization curves for an ensemble of identical noninteracting single-domain particles with equally oriented axes under the uniaxial anisotropy has been specifed for different…

Mesoscale and Nanoscale Physics · Physics 2008-03-12 A. A. Timopheev , S. M. Ryabchenko

We present an exactly solvable model of equal spin $s_1$ dimer single molecule magnets. The spins within each dimer interact via the Heisenberg and the most general quadratic global and local (single-ion) anisotropic spin interactions, and…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Dmitri V. Efremov , Richard A. Klemm

In intercalated transition metal dichalcogenide $Fe_xTaS_2$ (0.2 $\leq$ x $\leq$ 0.4) single crystals, large magnetic anisotropy is observed. Transport property measurements indicate that heavy Fe-doping leads to a large anisotropy of…

Strongly Correlated Electrons · Physics 2017-05-10 G. Wu , B. L. Kang , Y. L. Li , T. Wu , N. Z. Wang , X. G. Luo , Z. Sun , L. J. Zou , X. H. Chen

For equal-spin $s_1$ tetramer single molecule magnets with ionic point groups $g=T_d, D_{4h}, D_{2d}, C_{4h}, C_{4v}$, and $S_4$, we write the group-invariant single-ion, Dzaloshinskii-Moriya, and symmetric anisotropic near-neighbor and…

Mesoscale and Nanoscale Physics · Physics 2008-05-13 Richard A. Klemm , Dmitri V. Efremov

On the basis of a first-principles, relativistic electronic structure theory of finite temperature metallic magnetism, we investigate the variation of magnetic anisotropy, K, with magnetisation, M, in metallic ferromagnets. We apply the…

Materials Science · Physics 2009-11-10 J. B. Staunton , S. Ostanin , S. S. A. Razee , B. L. Gyorffy , L. Szunyogh , B. Ginatempo , Ezio Bruno

Dimers are the smallest chemical objects that show magnetic anisotropy. We focus on 3$d$ and 4$d$ transition metal dimers that have magnetic ground states in most cases. Some of these magnetic dimers have a considerable barrier against…

Atomic and Molecular Clusters · Physics 2008-04-09 Daniel Fritsch , Klaus Koepernik , Manuel Richter , Helmut Eschrig

We calculate magnetic anisotropy energy of Fe and Ni by taking into account the effects of strong electronic correlations, spin-orbit coupling, and non-collinearity of intra-atomic magnetization. The LDA+U method is used and its equivalence…

Strongly Correlated Electrons · Physics 2009-10-31 Imseok Yang , Sergej Y. Savrasov , Gabriel Kotliar

We report a systematic investigation of anisotropic magnetocaloric effects in single crystal Cr$_2$Te$_3$. Single crystal samples are synthesized by chemical vapor transport and characterized by x-ray and Laue diffraction methods. The…

Materials Science · Physics 2023-12-05 Anirban Goswami , Nicholas Ng , AM Milinda Abeykoon , Emmanuel Yakubu , Samaresh Guchhait

We calculate magnetic anisotropy energy of Fe and Ni by taking into account the effects of strong electronic correlations, spin-orbit coupling, and non-collinearity of intra--atomic magnetization. The LDA+U method is used and its…

Strongly Correlated Electrons · Physics 2007-05-23 Imseok Yang , Sergej Y. Savrasov , Gabriel Kotliar

Electron paramagnetic resonance (EPR) study of MBE grown Mn doped GaAs is presented. The resolved fine structure allows us to evaluate the crystal field parameters of the spin Hamiltonian. The obtained cubic constant is a= -14.1 10^-4/cm.…

Condensed Matter · Physics 2007-05-23 O. M. Fedorych , E. M. Hankiewicz , Z. Wilamowski , J. Sadowski

The main objective of this work is to investigate theoretically how tilting of an easy axis of a single-molecule magnet (SMM) from the orientation collinear with magnetic moments of the leads affects the switching process induced by current…

Mesoscale and Nanoscale Physics · Physics 2016-08-14 Maciej Misiorny , Józef Barnas

The symmetry of magnetic quantum tunneling (MQT) in the single molecule magnet Mn12-acetate has been determined by sensitive low-temperature magnetic measurements in the pure quantum tunneling regime and high frequency EPR spectroscopy in…

Mesoscale and Nanoscale Physics · Physics 2009-09-29 E. del Barco , A. D. Kent , S. Hill , J. M. North , N. S. Dalal , E. M. Rumberger , D. N. Hendrickson , N. Chakov , G. Christou

ZrMnP and HfMnP single crystals are grown by a self-flux growth technique and structural as well as temperature dependent magnetic and transport properties are studied. Both compounds have an orthorhombic crystal structure. ZrMnP and HfMnP…

Due to its strong magnetocrystalline anisotropy, FePt L1$\mathrm{_0}$ phase is considered as a promising magnetic recording media material. Although the magnetic properties of this phase have already been analyzed many times using density…

Materials Science · Physics 2022-05-11 Joanna Marciniak , Wojciech Marciniak , Mirosław Werwiński

A remarkably large magnetic anisotropy energy of 305 K is computed by quantum chemistry methods for divalent Fe$^{2+}$ $d^6$ substitutes at Li-ion sites with $D_{6h}$ point-group symmetry within the solid-state matrix of Li$_3$N. This is…

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