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The influence of an electron-vibrational coupling on the laser control of electron transport through a molecular wire that is attached to several electronic leads is investigated. These molecular vibrational modes induce an effective…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jörg Lehmann , Sigmund Kohler , Volkhard May , Peter Hänggi

We study the influence of laser radiation on the electron transport through a molecular wire weakly coupled to two leads. In the absence of a generalized parity symmetry, the molecule rectifies the laser induced current, resulting in…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jörg Lehmann , Sigmund Kohler , Peter Hänggi , Abraham Nitzan

A novel way to induce ultrafast currents in molecular wires using two incident laser frequencies, $\omega$ and $2\omega$, is demonstrated. The mechanism relies on Stark shifts, instead of photon absorption, to transfer population to the…

Quantum Physics · Physics 2009-11-13 Ignacio Franco , Moshe Shapiro , Paul Brumer

The induction of dc electronic transport in rigid and flexible trans-polyacetylene oligomers according to the $\omega$ vs. $2\omega$ coherent control scenario is investigated using a quantum-classical mean field approximation. The approach…

Quantum Physics · Physics 2009-11-13 Ignacio Franco , Moshe Shapiro , Paul Brumer

Nanoscale molecular-electronic devices and machines are emerging as promising functional elements, naturally flexible and efficient, for next generation technologies. A deeper understanding of carrier dynamics in molecular junctions is…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 K. Beltako , F. Michelini , N. Cavassilas , L. Raymond

New features of molecular wires can be observed when they are irradiated by laser fields. These effects can be achieved by periodically oscillating fields but also by short laser pulses. The theoretical foundation used for these…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Sven Welack , Michael Schreiber , Ulrich Kleinekathoefer

The soft character of organic materials leads to strong coupling between molecular nuclear and electronic dynamics. This coupling opens the way to control charge transport in organic electronic devices by inducing molecular vibrational…

Understanding the fundamental mechanisms ruling laser-induced coherent charge transfer in hybrid organic/inorganic interfaces is of paramount importance to exploit these systems in next-generation opto-electronic applications. In a…

Materials Science · Physics 2022-05-12 Matheus Jacobs , Jannis Krumland , Caterina Cocchi

Combining the features of molecular wires and femtosecond laser pulses gives the unique opportunity to optically switch electron currents in molecular devices with very high speed. Based on a weak-coupling approximation between wire and…

Mesoscale and Nanoscale Physics · Physics 2007-08-22 GuangQi Li , Sven Welack , Michael Schreiber , Ulrich Kleinekathoefer

We investigate dynamical transport properties of interacting electrons moving in a vibrating nanoelectromechanical wire in a magnetic field. We have built an exactly solvable model in which electric current and mechanical oscillation are…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Hangmo Yi , Kang-Hun Ahn

The influence of Gaussian laser pulses on the transport through molecular wires is investigated within a tight-binding model for spinless electrons including correlation. Motivated by the phenomenon of coherent destruction of tunneling for…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Ulrich Kleinekathoefer , GuangQi Li , Sven Welack , Michael Schreiber

Vibrationally inelastic electron transport through a molecular bridge that is connected to two leads is investigated. The study is based on a generic model of vibrational excitation in resonant transmission of electrons through a molecular…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Martin Cizek , Michael Thoss , Wolfgang Domcke

We study the interplay between lateral confinement and photon-induced processes on the electronic properties of illuminated graphene nanoribbons. We find that by tuning the device setup (edges geometries, ribbon width and polarization…

Mesoscale and Nanoscale Physics · Physics 2012-12-19 Hernan L. Calvo , Pablo M. Perez-Piskunow , Stephan Roche , Luis E. F. Foa Torres

We analytically tackle opto-vibronic interactions in molecular systems driven by either classical or quantum light fields. In particular, we examine a simple model of molecules with two relevant electronic levels, characterized by potential…

Quantum Physics · Physics 2024-02-28 Q. Zhang , M. Asjad , M. Reitz , C. Sommer , B. Gurlek , C. Genes

Electron transport in a quantum wire with leads is investigated with actual Coulomb interaction taken into account. The latter includes both the direct interaction of electrons with each other and their interaction via the image charges…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 V. A. Sablikov , B. S. Shchamkhalova

We consider several fundamental optical phenomena involving single molecules in biased metal-molecule-metal junctions. The molecule is represented by its highest occupied and lowest unoccupied molecular orbitals, and the analysis involves…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan

We investigate bistability and memory effects in a molecular junction weakly coupled to metallic leads with the latter being subject to an adiabatic periodic change of the bias voltage. The system is described by a simple Anderson-Holstein…

Mesoscale and Nanoscale Physics · Physics 2012-09-20 Andrea Donarini , Abdullah Yar , Milena Grifoni

A molecular wire coupled to two electron reservoirs is investigated within a tight-binding approach including spin and Coulomb interaction. Under the assumption of weak coupling to the electron reservoirs a quantum master equation can be…

Mesoscale and Nanoscale Physics · Physics 2007-08-28 Ulrich Kleinekathoefer , GuangQi Li , Sven Welack , Michael Schreiber

In laser-solid interactions, electrons may be generated and subsequently accelerated to energies of the order-of-magnitude of the ponderomotive limit, with the underlying process dominated by direct laser acceleration. Breaking this limit,…

Plasma Physics · Physics 2020-03-11 Meng Wen , Yousef I. Salamin , Christoph H. Keitel

Femtosecond laser light can transfer spin angular momentum between magnetic subspecies that exhibit hybridized valence bands within an alloy or compound, and represents the fastest route for manipulating the magnetization of a material. To…

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