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We derive a master equation for the electron transport through molecular wires in the limit of strong Coulomb repulsion. This approach is applied to two typical situations: First, we study transport through an open conduction channel for…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Franz J. Kaiser , Michael Strass , Sigmund Kohler , Peter Hänggi

Laser-driven electron transport across a sample has garnered enormous attentions over several decades, as it provides a much faster way to control electron dynamics. Light is an electromagnetic wave, so how and why an electron can acquire a…

Materials Science · Physics 2024-12-09 Robert Meadows , Y. Xue , Nicholas Allbritton , G. P. Zhang

We theoretically examine the effect of the coupling of the transport electrons to a vibrational mode of the molecule on the ac linear-response conductance of molecular junctions. Representing the molecule by a single electronic state, we…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 A. Ueda , O. Entin-Wohlman , A. Aharony

For the study of molecular spin junctions, we take into account two types of couplings between the molecule and the metal leads: (i) electron transfer that gives rise to net current in the biased junction and (ii) energy transfer between…

Mesoscale and Nanoscale Physics · Physics 2009-04-23 M. Jouravlev , Kwang S. Kim

Interfaces between molecules and 2D materials exhibit energy-driven functionalities, wherein charge transfer directs molecular motion. Unlike equilibrium systems, where molecular assemblies settle into static configurations, continuous…

The response of conduction band electrons to a local, pulse-like external excitation is investigated. The charge density wave packets that emerge as a consequence of the excitation leave the interaction region with a speed close to the…

Quantum Physics · Physics 2017-12-06 Istvan Magashegyi , Lorant Zs. Szabo , Peter Foldi

Laser-driven electron transport across a sample has garnered enormous attentions over several decades, because it potentially allows one to control spin transports in spintronics. But light is a transverse electromagnetic wave, how an…

Materials Science · Physics 2023-10-23 Robert Meadows , Y. Xue , Nicholas Allbritton , G. P. Zhang

We describe how to treat the interaction of travelling electrons with localised vibrational modes in nanojunctions. We present a multichannel scattering technique which can be applied to calculate the transport properties for realistic…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 H. Ness , A. J. Fisher

The ultrafast dynamics of ions in solids following intense femtosecond laser excitation is governed by two fundamentally distinct yet interplaying effects. On one hand, the significant generation of hot electron-hole pairs by the light…

Computational Physics · Physics 2024-01-22 Bernd Bauerhenne , Martin E. Garcia

Theoretical foundations of electron transport in mesoscopic systems, based on Landauer theory, Master equations or Onsager linear thermodynamics, are revisited to show that the noniteracting electrons model is insufficient to describe…

Mesoscale and Nanoscale Physics · Physics 2025-07-29 Robert Alicki

Electromigrated nanoscale junctions have proven very useful for studying electronic transport at the single-molecule scale. However, confirming that conduction is through precisely the molecule of interest and not some contaminant or metal…

Mesoscale and Nanoscale Physics · Physics 2008-09-04 D. R. Ward , G. D. Scott , Z. K. Keane , N. J. Halas , D. Natelson

We study linear electron transport through a molecular wire sandwiched between nanotube leads. We show that the presence of such electrodes strongly influences the calculated conductance. We find that depending on the quality and geometry…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 G. Cuniberti , G. Fagas , K. Richter

The conventional picture of the light amplification by stimulated emission of radiation (laser) is broken under the ultrastrong interaction between the electromagnetic fields and matter, and distinct dynamics of the electric field and of…

Quantum Physics · Physics 2016-03-10 Motoaki Bamba , Tetsuo Ogawa

Ultrafast laser excitation can create coherent superpositions of electronic states in molecules and trigger ultrafast flow of electron density on few- to sub-femtosecond time scales. While recent attosecond experiments have addressed…

Chemical Physics · Physics 2020-11-18 Yuki Kobayashi , Daniel M. Neumark , Stephen R. Leone

The orbital angular momenta (OAM) of electrons play an increasingly important role in ultrafast electron and magnetization dynamics. In this theoretical study, we investigate the electron dynamics induced by femtosecond laser pulses in a…

Materials Science · Physics 2023-10-13 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

The influence of the charging effects on the transport characteristics of a molecular wire bridging two metallic electrodes in the limit of weak contacts is studied by generalized Breit-Wigner formula. Molecule is modeled as a quantum dot…

Chemical Physics · Physics 2009-11-10 Kamil Walczak

The influence of multiple vibrational modes on current fluctuations in electron transport through single-molecule junctions is investigated. Our analysis is based on a generic model of a molecular junction, which comprises a single…

Mesoscale and Nanoscale Physics · Physics 2014-09-26 C. Schinabeck , R. Härtle , H. B. Weber , M. Thoss

A case of moving one-dimensional electromagnetic (EM) solitons formed in a relativistic interaction of a linearly polarized laser light with underdense cold plasma is investigated. The relativistic Lorentz force in an intense laser light…

Plasma Physics · Physics 2007-05-23 Ljupco Hadzievski , Ana Mancic , Milos Skoric

Circularly polarized colliding laser pulses can create abundant electron-positron pair plasma [A. R. Bell and J. G. Kirk, Phys. Rev. Lett. 101, 200403 (2008)], which scattering the incoming electromagnetic waves can prevent them from…

The dynamics of transient electric fields generated by the interaction of high intensity laser pulses with underdense plasmas has been studied experimentally with the proton projection imaging technique. The formation of a charged channel,…