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We demonstrate second harmonic generation in photonic crystal cavities in (001) and (111)B oriented GaAs. The fundamental resonance is at 1800 nm, leading to second harmonic below the GaAs bandgap. Below-bandgap operation minimizes…

Intense laser-driven nonlinear optical phenomena in two-dimensional (2D) nodal-line semimetals (NLS) exhibit complex mechanisms, particularly in the NbSi$_{x}$Te$_{2}$ material systems characterized by nonsymmorphic symmetry-protected band…

Optics · Physics 2025-08-25 Navdeep Rana , M. S. Mrudul , Amar Bharti , Sucharita Giri , Gopal Dixit

The transition metal monopnictide family of Weyl semimetals recently has been shown to exhibit anomalously strong second-order optical nonlinearity, which is theoretically attributed to a highly asymmetric polarization distribution induced…

Strongly Correlated Electrons · Physics 2022-07-21 Chen Li , Xiang Li , T. Deshpande , Xinwei Li , N. Nair , J. G. Analytis , D. M. Silevitch , T. F. Rosenbaum , D. Hsieh

We investigated in detail the optical properties of several Cu(1-delta)Mg(delta)GeO3 (with delta=0,0.01), and CuGe(1-x)B(x)O3 with B=Si (x=0,0.007,0.05,0.1), and Al (x=0,0.01) single crystals, in the frequency range 20-32000 cm^-1. We…

Strongly Correlated Electrons · Physics 2009-10-31 A. Damascelli , D. van der Marel , G. Dhalenne , A. Revcolevschi

We show that the lack of inversion symmetry in monolayer MoS2 allows strong optical second harmonic generation. Second harmonic of an 810-nm pulse is generated in a mechanically exfoliated monolayer, with a nonlinear susceptibility on the…

Materials Science · Physics 2015-06-15 Nardeep Kumar , Sina Najmaei , Qiannan Cui , Frank Ceballos , Pulickel M. Ajayan , Jun Lou , Hui Zhao

Motivated by the search for type-II multiferroics, we present a comprehensive optical study of a complex oxide family of type-II multiferroic candidates: RbFe(MoO4)2, RbFe(SeO4)2, and RbFe(SO4)2. We employ rotational-anisotropy second…

Second harmonic generation (SHG) is a fundamental nonlinear optical phenomenon widely used both for experimental probes of materials and for application to optical devices. Even-order nonlinear optical responses including SHG generally…

Mesoscale and Nanoscale Physics · Physics 2021-10-13 Kazuaki Takasan , Takahiro Morimoto , Joseph Orenstein , Joel E. Moore

Resonant optical excitation of apical oxygen vibrational modes in the normal state of underdoped YBa2Cu3O6+x induces a transient state with optical properties similar to those of the equilibrium superconducting state. Amongst these, a…

We have studied second harmonic generation (SHG) in a polar ferrimagnet GaFeO_3, employing a FeO_6 cluster model in which the Fe atom is slightly shifted from the center of the octahedron. The electric-dipole transition could take place…

Strongly Correlated Electrons · Physics 2015-05-19 Jun-ichi Igarashi , Tatsuya Nagao

An interesting property of high harmonic generation in solids is its laser polarization dependent nature which in turn provides information about the crystal and band structure of the generation medium. Here we report on the linear…

Second-order optical nonlinear effects (second-harmonic and sum-frequency generation) are demonstrated in the telecommunication band by periodic poling of thin films of lithium niobate wafer-bonded on silicon substrates and rib-loaded with…

The ferro-rotational order, whose order parameter (OP) is an axial vector invariant under both time reversal (TR) and spatial inversion (SI) operations, is the last remaining category of ferroics to be observed after the ferroelectric,…

We demonstrate a new, nonlinear optical effect of electric currents. First, a steady current is generated by applying a voltage on a doped GaAs crystal. We demonstrate that this current induces second-harmonic generation of a probe laser…

Materials Science · Physics 2015-06-03 Brian A. Ruzicka , Lalani K. Werake , Guowei Xu , Jacob B. Khurgin , E. Ya. Sherman , Judy Z. Wu , Hui Zhao

A theoretical study of the newly identified Ti5Al2C3 belonging to the MAX phases has been performed by using the first-principles pseudopotential plane-wave method within the generalized gradient approximation (GGA). The energy band…

Materials Science · Physics 2012-06-19 M. S. Ali , A. K. M. A. Islam , M. A. Hossain

To add the detailed information to the existed knowledge of nonlinear optics field, the nonlinear optical processes of the second and third order have been discussed in their respective susceptibility tensors in the presence of degenerate…

Optics · Physics 2018-01-29 A Srinivasa Rao

We present a comprehensive model for predicting the full performance of a second harmonic generationoptical parametric amplification system that aims at enhancing the temporal contrast of laser pulses. The model simultaneously takes into…

Optics · Physics 2016-01-22 A. B. Sharba , G. Nersisyan , M. Zepf , M. Borghesi , G. Sarri

We theoretically predict efficient optical second-harmonic generation (SHG) from a few hundred nanometer thick slab consisting of a quadratic nonlinear anisotropic medium whose linear principal permittivities are, at the fundamental…

Optics · Physics 2011-03-16 Alessandro Ciattoni

Second-order nonlinear optical materials enable frequency doubling of light (second-harmonic generation, SHG), which is essential for optoelectronic applications ranging from materials characterization to quantum technologies. However,…

Materials Science · Physics 2026-03-25 Aubrey G. J. Nyiri , Michael J. Waters , James M. Rondinelli

The BiTeX family of polar van der Waals (vdW) semiconductors offers a unique platform for exploring the interplay between polar crystalline structure and nonlinear optical phenomena. Here, we utilize second harmonic generation (SHG)…

We describe a compact and stable setup for detecting the optical second harmonics, in which the incident plane rotates with respect to the sample. The setup is composed of rotating Fresnel-rhomb optics and a femtosecond ytterbium-doped…

Instrumentation and Detectors · Physics 2021-04-23 S. H. Kim , S. Jung , B. Seok , Y. S. Kim , H. Park , T. Otsu , Y. Kobayashi , C. Kim , Y. Ishida