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We theoretically investigate the second harmonic generation (SHG) of topological insulator surface states in a perpendicular magnetic field. Our theory is based on the microscopic expression of the second-order magneto-optical conductivity…

Mesoscale and Nanoscale Physics · Physics 2024-11-27 Kainan Chang , Muhammad Zubair , Jin Luo Cheng , Wang-Kong Tse

We investigate the generation of ultraviolet (UV) second-harmonic radiation on the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By…

Optics · Physics 2016-12-19 Xiaohui Zhao , Yuanlin Zheng , Huaijin Ren , Ning An , Xuewei Deng , Xianfeng Chen

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…

The binary phase diagram of the YAlO3 (YAP) - NdAlO3 (NAP) system was determined by differential thermal analysis (DTA) and X-ray powder diffraction (XRD) measurements. High purity nanocrystalline powders and small single crystals of…

Materials Science · Physics 2011-08-15 A. Szysiak , D. Klimm , S. Ganschow , M. Mirkowska , R. Diduszko , L. Lipińska , A. Kwasniewski , A. Pajączkowska

A comprehensive analysis of optical second harmonic generation (SHG) on an incommensurate (IC) magnetically ordered state is presented using multiferroic MnWO4 as model compound. Two fundamentally different SHG contributions coupling to the…

Strongly Correlated Electrons · Physics 2012-08-08 D. Meier , N. Leo , G. Yuan , Th. Lottermoser , P. Becker , L. Bohaty , M. Fiebig

We present a full formalism for the calculation of the linear and second-order optical response for semiconductors and insulators. The expressions for the optical susceptibilities are derived within perturbation theory. As a starting point…

Materials Science · Physics 2009-11-10 S. Sharma , C. Ambrosch-Draxl

Near-infrared-to-visible second harmonic generation from air-stable two-dimensional polar gallium and indium metals is described. The photonic properties of 2D metals - including the largest second-order susceptibilities reported for metals…

Second harmonic generation (SHG), as one of the most significant \c{hi}(2) nonlinear optical processes, plays crucial roles in a broad variety of optical and photonic applications. Designing various delicate schemes to achieve highly…

Optics · Physics 2021-09-01 Lei Wang , XiuQuan Zhang , Feng Chen

We present a study of second harmonic generation (SHG) and third harmonic generation (THG) in lithium triborate (LBO) crystals using a high-energy, 10-J-class, 10 Hz Yb:YAG laser system. We achieved high conversion efficiencies of 75% for…

Optically anisotropic materials are sought after for tailoring the polarization of light. Recently, colossal optical anisotropy was reported in a quasi-one-dimensional chalcogenide, Sr1.125TiS3. Compared to SrTiS3, the excess Sr in…

Optical properties of semiconductors can exhibit strong polarization dependence due to crystalline anisotropy. A number of recent experiments have shown that the photoluminescence intensity in free standing nanowires is polarization…

Mesoscale and Nanoscale Physics · Physics 2013-03-05 Amrit De , Craig E. Pryor

The magnetic insulator $\alpha$-RuCl$_{3}$ is a promising candidate to realize Kitaev interactions on a quasi-2D honeycomb lattice. We perform extensive susceptibility measurements on single crystals of $\alpha$-RuCl$_{3}$, including…

In this paper we present a theoretical study of the third-order nonlinear optical properties of poly(diphenyl)polyacetylene (PDPA) pertaining to the third-harmonic-generation (THG) process. We study the aforesaid process in PDPA's using…

Materials Science · Physics 2010-01-14 Alok Shukla

Femtosecond pump-probe second-harmonic generation (SHG) and transient linear reflectivity measurements were carried out on polycrystalline Cu, Ag and Au in air to analyze whether the electron temperature affects Fresnel factors or nonlinear…

Condensed Matter · Physics 2015-06-25 J. Hohlfeld , U. Conrad , E. Matthias

We use general symmetry-based arguments to construct an effective model suitable for studying optical properties of lead-halide perovskites. To build the model, we identify an atomic-level interaction between electromagnetic fields and the…

In this paper, we proposed and numerically demonstrated a giant enhancement up to 108 in both forward and backward propagation of the Second Harmonic Generation by combining the high-quality factor cavities of the Bound States in the…

Optics · Physics 2022-06-24 Juan José Robayo Yepes , Fadi Issam Baida , Abdoulaye Ndao

A pure spin current formed by opposite spins moving in opposite directions is a rank-2 axial tensor which breaks the inversion symmetry. Thus a spin current has a second-order optical susceptibility, with unique polarization-dependence…

Other Condensed Matter · Physics 2010-06-30 Jing Wang , Bang-Fen Zhu , Ren-Bao Liu

Within a cavity quantum electrodynamics description, we characterize the fluorescent spectrum from ultracold bosons atoms, in the second harmonic generation (SHG) and resonant cases. Two situations are considered: i) bosons loaded into an…

Quantum Gases · Physics 2024-01-12 Megha Gopalakrishna , Emil Viñas Boström , Claudio Verdozzi

LMTO calculations are presented for the frequency dependent second harmonic generation (SHG) in the polytypes 2H, 4H, 6H, 15R and 3C of SiC. All independent tensor components are calculated. The spectral features and the ratios of the 333…

Condensed Matter · Physics 2009-10-30 Sergey N. Rashkeev , Walter R. L. Lambrecht , Benjamin Segall

We study the linear- and nonlinear-optical lineshapes of metal nanoparticles (theory) and metallic photonic crystal slabs (experiment and theory). For metal nanoparticle ensembles, we show analytically and numerically that femtosecond…

Materials Science · Physics 2007-05-23 M. W. Klein , T. Tritschler , M. Wegener , S. Linden