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Electron injection from an adsorbed molecule to the substrate (heterogeneous electron transfer) is studied. One reaction coordinate is used to model this process. The surface phonons and/or the electron-hole pairs together with the internal…

Chemical Physics · Physics 2009-11-07 Michael Schreiber , Ivan Kondov , Ulrich Kleinekathoefer

Is it possible to design a supramolecular cage that would "solvate" the excess electron in the same fashion in which several solvent molecules do that co-operatively in polar liquids? Two general strategies are outlined for "electron…

Chemical Physics · Physics 2016-09-28 Ilya A. Shkrob , Myran C. Sauer,

Spin-polarized first-principles calculations have been performed to tune the electronic and optical properties of graphene (G) and boron-nitride (BN) quantum dots (QDs) through molecular charge-transfer using Tetracyanoquinodimethane (TCNQ)…

Materials Science · Physics 2017-09-13 Arkamita Bandyopadhyay , Sharma SRKC Yamijala , Swapan K Pati

A high-yield production of high-quality boron-nitride nanotubes (BNNTs) was reported recently in several publications. A boron-rich material is evaporated by a laser or plasma in a nitrogen-rich atmosphere to supply precursor gaseous…

In this work, we study the electronic properties of monolayer transition metal dichalcogenide materials subjected to aliovalent doping, using Nb-doped WS2 as an exemplar. Scanning transmission electron microscopy imaging of the as-grown…

Materials Science · Physics 2021-06-16 Siow Mean Loh , Xue Xia , Neil R. Wilson , Nicholas D. M. Hine

New two diemensional structures nanoribbon including phosphorus and germanium atoms are introduced for the nanoelectronic applications. Under various bias voltages, the electronic transport in the systems have been studied within the…

Mesoscale and Nanoscale Physics · Physics 2018-01-09 Maryam Azizi , Badie Ghavami

In all theoretical treatments of electron transport through single molecules between two metal electrodes, a clear distinction has to be made between a coherent transport regime with a strong coupling throughout the junction and a Coulomb…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Robert Stadler , Jerome Cornil , Victor Geskin

The double carrier transport has been observed in thin film black phosphorus (BP) field effect transistor (FET) devices in highly electron doped region. BP thin films with typical thickness of 15 nm were encapsulated by hexagonal boron…

Mesoscale and Nanoscale Physics · Physics 2018-11-08 Kohei Hirose , Toshihito Osada , Kazuhito Uchida , Toshihiro Taen , Kenji Watanabe , Takashi Taniguchi , Yuichi Akahama

We present a theoretical study of the optical absorption spectrum of small boron-nitride and carbon nanotubes using time-dependent density-functional theory and the random phase approximation. Both for C and BN tubes, the absorption of…

Materials Science · Physics 2009-11-10 L. Wirtz , V. Olevano , A. G. Marinopoulos , L. Reining , A. Rubio

One of the basic assumptions in organic field-effect transistors, the most fundamental device unit in organic electronics, is that charge transport occurs two-dimensionally in the first few molecular layers near the dielectric interface.…

Mesoscale and Nanoscale Physics · Physics 2016-01-11 Yuhan Zhang , Jingsi Qiao , Si Gao , Fengrui Hu , Daowei He , Bing Wu , Ziyi Yang , Bingchen Xu , Yun Li , Yi Shi , Wei Ji , Peng Wang , Xiaoyong Wang , Min Xiao , Hangxun Xu , Jian-Bin Xu , Xinran Wang

The current rechargeable battery technologies have a failure in their performance at high pressure and temperature. In this article, we have brought theoretical insights on using boron nitride flakes as a protecting layer for a lithium-ion…

Applied Physics · Physics 2021-02-15 Narjes Kheirabadi , Azizollah Shafiekhani

We studied various gas molecules (NO$_2$, O$_2$, NH$_3$, N$_2$, CO$_2$, CH$_4$, H$_2$O, H$_2$, Ar) on single-walled carbon nanotubes (SWNTs) and bundles using first principles methods. The equilibrium position, adsorption energy, charge…

Materials Science · Physics 2009-11-07 Jijun Zhao , Alper Buldum , Jie Han , Jian Ping Lu

We report the results of our first-principles study based on density functional theory on the interaction of the nucleic acid base molecules adenine (A), cytosine (C), guanine (G), thymine (T), and uracil (U), with a single-walled carbon…

Soft Condensed Matter · Physics 2008-02-21 S. Gowtham , Ralph H. Scheicher , Ravindra Pandey , Shashi P. Karna , Rajeev Ahuja

Quantum mechanical methods based on the density functional theory (DFT) offer a realistic possibility of first-principles design of organic donor-acceptor systems and engineered band-gap materials. This promise is contingent upon the…

Chemical Physics · Physics 2013-12-03 Marcin Modrzejewski , Grzegorz Chałasiński , Małgorzata M. Szczęśniak

We report a comprehensive study on the electrochemical performance of four different Transition Metal Oxides encapsulated inside carbon nanotubes (CNT). Irrespective of the type of oxide-encapsulate, all these samples exhibit superior…

We present an atomistic self-consistent study of the electronic and transport properties of semiconducting carbon nanotube in contact with metal electrodes of different work functions, which shows simultaneous electron and hole doping…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Yongqiang Xue , Mark A. Ratner

Molecule-based devices are envisioned to complement silicon devices by providing new functions or already existing functions at a simpler process level and at a lower cost by virtue of their self-organization capabilities. Moreover, they…

Mesoscale and Nanoscale Physics · Physics 2010-02-04 F. Alibart , S. Pleutin , D. Guerin , C. Novembre , S. Lenfant , K. Lmimouni , C. Gamrat , D. Vuillaume

In the present work we discuss based on extensive fully atomistic molecular dynamics simulations the dynamics of Neon atoms oscillating inside (5,5)single-walled carbon nanotubes (CNTs) and boron-nitride (BNNT) ones. Our results show that…

Materials Science · Physics 2007-07-24 Karl M. Garcez , David L. Azevedo , Douglas S. Galvão

We demonstrate that encapsulation of atomically thin black phosphorus (BP) by hexagonal boron nitride (h-BN) sheets is very effective for minimizing the interface impurities induced during fabrication of BP channel material for quantum…

Mesoscale and Nanoscale Physics · Physics 2016-07-12 Gen Long , Shuigang Xu , Junying Shen , Jianqiang Hou , Zefei Wu , Tianyi Han , Jiangxiazi Lin , Wing Ki Wong , Yuan Cai , Rolf Lortz , Ning Wang

Single layer core/shell structures consisting of graphene as core and hexagonal boron nitride as shell are studied using first-principles plane wave method within density functional theory. Electronic energy level structure is analysed as a…

Mesoscale and Nanoscale Physics · Physics 2014-08-05 S. Cahangirov , S. Ciraci
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