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Improper ferroelectricity (trimerization) in the hexagonal manganites RMnO$_3$ leads to a network of coupled structural and magnetic vortices that induce domain wall magnetoelectricity and magnetization neither of which, however, occurs in…

Materials Science · Physics 2015-06-12 Hena Das , Aleksander L. Wysocki , Yanan Geng , Weida Wu , Craig J. Fennie

The search for new materials for energy-efficient electronic devices has gained unprecedented importance. Among the various classes of magnetic materials driving this search are antiferromagnets, magnetoelectrics, and systems with…

A new type of multiferroicity was experimentally discovered in 2003 in a perovskite manganite TbMnO$_3$ where its ferroelectricity is induced by cycloidally ordered Mn spins. Susequently, such spin-cycloid multiferroic phase was also…

Strongly Correlated Electrons · Physics 2025-02-14 Masahito Mochizuki

Magnetic structures are investigated by means of neutron diffraction to shine a light on the intricate details that are believed to be key to understanding the magnetoelectric effect in LiCoPO$_4$ . At zero field, a spontaneous spin canting…

Spin-orbit coupling introduces chirality into electronic structure. This can have profound effects on the magnetization induced by orbital motion of electrons. Here we derive a formula for the orbital magnetization of interacting electrons…

Strongly Correlated Electrons · Physics 2014-09-23 R. Nourafkan , G. Kotliar , A. -M. S. Tremblay

Spin density waves, based on modulated local moments, are usually associated with metallic materials, but have recently been reported in insulators which display coupled magnetic and structural order parameters. We discuss one such example,…

Materials Science · Physics 2020-07-30 N. Giles-Donovan , N. Qureshi , R. D. Johnson , L. Y. Zhang , S. -W. Cheong , S. Cochran , C. Stock

In rhombohedral CaMn7O12, an improper ferroelectric polarization of magnitude 2870 {\mu}C m-2 is induced by an incommensurate helical magnetic structure that evolves below TN1 = 90 K. The electric polarization was found to be constrained to…

Strongly Correlated Electrons · Physics 2015-05-30 R. D. Johnson , L. C. Chapon , D. D. Khalyavin , P. Manuel , P. G. Radaelli , C. Martin

We combine the anisotropy of magnetic interactions and the point symmetry of finite solids in the study of dipolar clusters as new basic units for multiferroics metamaterials. The hamiltonian of magnetic dipoles with an easy axis at the…

Materials Science · Physics 2020-12-03 Paula Mellado , Andres Concha , Sergio Rica

A microscopic model for the room-temperature multiferroic BiFeO$_3$ that includes two Dzyaloshinskii-Moriya interactions and single-ion anisotropy along the ferroelectric polarization predicts both the zero-field spectroscopic modes as well…

Strongly Correlated Electrons · Physics 2015-10-28 Randy S. Fishman , Jun Hee Lee , Sándor Bordács , István Kézsmárki , Urmas Nagel , Toomas Rõõm

Below its N\'eel temperature, the frustrated magnet CdCr$_2$O$_4$ exhibits an antiferromagnetic spin-spiral ground state. Such states can give rise to a sizable magnetoelectric coupling. In this report, we measure the electric polarization…

Materials Science · Physics 2020-07-15 L. Rossi , D. Brüning , H. Ueda , Y. Skourski , T. Lorenz , B. Bryant

We have studied the magnetic structure of the ferroelectric frustrated spin-1/2 chain material LiCuVO4 in applied electric and magnetic fields using polarized neutrons. A symmetry and mean-field analysis of the data rules out the presence…

Strongly Correlated Electrons · Physics 2011-03-23 M. Mourigal , M. Enderle , R. K. Kremer , J. M. Law , B. Fåk

We have investigated the role of the 4$f$ moment on the magnetoelectric (ME) effect of orthorhombic $R$MnO$_{3}$ ($R$=rare earth ions). In order to clarify the role of the 4$f$ moment, we prepared three samples: (Eu,Y)MnO$_{3}$ without the…

Strongly Correlated Electrons · Physics 2007-05-23 K. Noda , M. Akaki , F. Nakamura , D. Akahoshi , H. Kuwahara

Spin-orbit coupling in inversion-asymmetric magnetic crystals and structures has emerged as a powerful tool to generate complex magnetic textures, interconvert charge and spin under applied current, and control magnetization dynamics.…

Mesoscale and Nanoscale Physics · Physics 2019-10-02 A. Manchon , J. Zelezný , I. M. Miron , T. Jungwirth , J. Sinova , A. Thiaville , K. Garello , P. Gambardella

The magnetic polarization induced by nonmagnetic impurities such as Zn in high Tc cuprate compounds is studied by the variational Monte Carlo simulation. The variational wave function is constructed from the eigenstates obtained from…

Strongly Correlated Electrons · Physics 2009-11-07 Shi-Dong Liang , T. K. Lee

Within the broad class of multiferroics (compounds showing a coexistence of magnetism and ferroelectricity), we focus on the subclass of "improper electronic ferroelectrics", i.e. correlated materials where electronic degrees of freedom…

Materials Science · Physics 2012-07-26 Silvia Picozzi , Alessandro Stroppa

The magnetoelectric coupling effect with profound physics and enormous potential applications has provoked a great number of research activities in materials science. Here, we report that the reversible orbital reconstruction driven by…

Strongly Correlated Electrons · Physics 2015-09-08 Bin Cui , Cheng Song , Haijun Mao , Huaqiang Wu , Fan Li , Jingjing Peng , Guangyue Wang , Fei Zeng , Feng Pan

Electric control of multiferroic domains is demonstrated through polarized magnetic neutron diffraction. Cooling to the cycloidal multiferroic phase of Ni3V2O8 in an electric field (E) causes the incommensurate Bragg reflections to become…

Strongly Correlated Electrons · Physics 2009-08-23 I. Cabrera , M. Kenzelmann , G. Lawes , Y. Chen , W. C. Chen , R. Erwin , T. R. Gentile , J. B. Leão , J. W. Lynn , N. Rogado , R. J. Cava , C. Broholm

The $\beta$ and $\gamma$ phases of methylammonium chloride CH$_3$NH$_3$Cl and methylammonium bromide CH$_3$NH$_3$Br are identified to be ferroelectric $via$ pyroelectric current and dielectric constant measurements. The magnetic…

Materials Science · Physics 2024-05-17 Chu Xin Peng , Lei Meng , Yi Yang Xu , Tian Tian Xing , Miao Miao Zhao , Peng Ren , Fei Yen

The present paper proposes the direct calculation of the microscopic contributions to the magneto-electric coupling, using ab initio methods. The electrostrictive and the Dzyaloshinskii-Moriya contributions were evaluated individually. For…

Strongly Correlated Electrons · Physics 2015-06-17 J. Varignon , S. Petit , A. Gellé , M. -B. Lepetit

Electrical manipulation of spins is essential to design state-of-the-art spintronic devices and commonly relies on the spin current injected from a second heavy-metal material. The fact that chiral antiferromagnets produce spin current…

Materials Science · Physics 2022-10-26 Hang Xie , Xin Chen , Qi Zhang , Zhiqiang Mu , Xinhai Zhang , Binghai Yan , Yihong Wu