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We study the recently observed orbital excitations, orbitons, and treat electron-electron correlations and lattice dynamics on equal footing. It is shown that the orbiton energy and dispersion are determined by both correlations and…

Strongly Correlated Electrons · Physics 2009-11-07 Jeroen van den Brink

We report on the spin waves and crystal field excitations in single crystal LiFePO$_4$ by inelastic neutron scattering over a wide range of temperatures, below and above the antiferromagnetic transition of this system. In particular, we…

Strongly Correlated Electrons · Physics 2017-03-15 Yuen Yiu , Manh Duc Le , Rasmus Toft-Peterson , Georg Ehlers , Robert McQueeney , David Vaknin

Magnetic rare earth atoms on pyrochlore lattice can produce such exotic magnetic states as spin ice and quantum spin ice. These states are a result of the frustration in the pyrochlore lattice, as well as crystal field degrees of freedom of…

We have measured the doping and temperature dependence of lattice vibrations and magnetic excitations in the prototypical doped spin-orbit Mott insulator Sr$_{2-x}$La$_x$IrO$_4$ (x=0, 0.015, and 0.10). Our findings show that the…

Strongly Correlated Electrons · Physics 2017-09-27 H. Gretarsson , J. Sauceda , N. H. Sung , M. Höppner , M. Minola , B. J. Kim , B. Keimer , M. Le Tacon

We report results of the Raman measurements for SrRu$_2$O$_6$ having extraordinary high N$\acute{\textrm{e}}$el temperature for a layered material. No additional phonon modes were detected at the temperature of magnetic transition thus…

Materials Science · Physics 2019-02-13 Yu. S. Ponosov , E. V. Komleva , D. A. Zamyatin , R. I. Walton , S. V. Streltsov

We report a comprehensive study of the low-level substitution of Mn$^{3+}$ by Fe$^{3+}$ effect on the static and dynamic magnetoelectric coupling in TbMn$_{1-x}$Fe$_x$O$_3$ ($x=0$, 0.02 and 0.04). The cationic substitution has a large…

Materials Science · Physics 2023-03-14 A. Maia , R. Vilarinho , C. Kadlec , M. Lebeda , M. Mihalik, , M. Zentková , M. Mihalik , J. Agostinho Moreira , S. Kamba

Strongly interacting phonons and orbital excitations are observed in the same energy range for CuSb$_2$O$_6$, unlocking a so-far unexplored type of electron-phonon interaction. An orbital wave at $\sim 550$ cm$^{-1}$ softens on warming and…

Strongly Correlated Electrons · Physics 2018-05-17 D. T. Maimone , A. B. Christian , J. J. Neumeier , E. Granado

We used polarization-resolved Raman scattering to study magneto-elastic coupling in Ba(Fe$_{1-x}$Au$_{x}$)$_2$As$_2$ crystals as a function of light Au-doping, materials for which temperatures of the structural transition ($T_S$) and of the…

Superconductivity · Physics 2020-07-15 S. -F. Wu , W. -L. Zhang , L. Li , H. -B. Cao , H. -H. Kung , A. S. Sefat , H. Ding , P. Richard , G. Blumberg

We report on the lattice and spin dynamics in the monopnictide CrAs using polarized Raman scattering. This system exhibits a first-order magneto-structural phase transition at T_N~ 265 K, below which the magnetic moments of Cr form an…

Materials Science · Physics 2019-10-07 K. Sen , Y. Yao , R. Heid , A. Omoumi , F. Hardy , K. Willa , M. Merz , A. A. Haghighirad , M. Le Tacon

Fe3GeTe2 has emerged as one of the most fascinating van der Waals crystals due to its two-dimensional (2D) itinerant ferromagnetism, topological nodal lines and Kondo lattice behavior. However, lattice dynamics, chirality of phonons and…

Temperature-dependent (5 K to 300 K) Raman scattering study of A$_{1g}$/A'$_1$ phonon modes in mono-layer (1L), bilayer (2L), trilayer (3L), and tetralayer (4L) MoTe$_2$ is reported. The temperature evolution of the modes' intensity…

Mesoscale and Nanoscale Physics · Physics 2017-09-19 K. Gołasa , M. Grzeszczyk , M. R. Molas , M. Zinkiewicz , Ł. Bala , K. Nogajewski , M. Potemski , A. Wysmołek , A. Babiński

The recently discovered layered BiS2-based superconductors have attracted a great deal of interest due to their structural similarity to cuprate and iron-pnictide superconductors. We have performed Raman scattering measurements on two…

Superconductivity · Physics 2016-03-08 Yong Tian , Anmin Zhang , Kai Liu , Jianting Ji , Jianzhong Liu , Xiyu Zhu , Hai-Hu Wen , Feng Jin , Xiaoli Ma , Qing-Ming Zhang

Magnetic excitations in van der Waals (vdW) materials, especially in the two-dimensional (2D) limit, are an exciting research topic from both the fundamental and applied perspectives. Using temperature-dependent, magneto-Raman spectroscopy,…

Raman spectroscopy is utilized to study the magnetic characteristics of heteroepitaxial NiO thin films grown by plasma-assisted molecular beam epitaxy on MgO(100) substrates. For the determination of the N\'eel temperature, we demonstrate a…

Materials Science · Physics 2020-07-24 J. Feldl , M. Budde , C. Tschammer , O. Bierwagen , M. Ramsteiner

Polarization-resolved Raman spectroscopy was performed and analyzed from large, high quality, mono-domain single crystal of {\alpha}-RuCl3, a proximate Kitaev quantum spin liquid. Spectra were collected with laser polarizations parallel and…

We present a detailed temperature dependent Raman light scattering study of optical phonons in Ba{1-x}K{x}Fe{2}As{2} (x ~ 0.28, superconducting Tc ~ 29 K), Sr{1-x}K{x}Fe{2}As{2} (x ~ 0.15, Tc ~ 29 K) and non-superconducting BaFe{2}As{2}…

Superconductivity · Physics 2009-08-18 M. Rahlenbeck , G. L. Sun , D. L. Sun , C. T. Lin , B. Keimer , C. Ulrich

A Raman scattering study covering the entire substitution range of the FeSe$_{1-x}$S$_x$ solid solution is presented. Data were taken as a function of sulfur concentration $x$ for $0\le x \le 1$, of temperature and of scattering symmetry.…

The Raman scattering response of the biaxial antiferromagnet CoPS$_3$ has been investigated as a function of both magnetic field and temperature. The peaks observed in the low-frequency spectral range (90--200~cm$^{-1}$) have been…

The vibrational properties of ferrimagnetic $\mathrm{Mn_3Si_{2}Te_6}$ single crystals are investigated using Raman spectroscopy and density functional theory calculations. Eighteen Raman-active modes are identified, fourteen of which are…

The observation of strongly coupled lattice and spin dynamics in altermagnet CoF$_2$ is reported. On the background of the expected spin-phonon interaction leading to renormalization of all phonons at the Neel temperature an additional…

Materials Science · Physics 2024-05-14 M. A. Prosnikov , M. Bal , R. V. Pisarev , P. C. M. Christianen , A. M. Kalashnikova