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The ultrafast switching of magnetization in multiferroic materials by a femtosecond laser could provide various advantages in photonics and magnonics. An efficient approach to control the light matter interaction is the modulation of…

We report results of an investigation of the temperature dependence of the magnon and phonon frequencies in NiO. A combination of Brillouin - Mandelstam and Raman spectroscopies allowed us to elucidate the evolution of the phonon and magnon…

Materials Science · Physics 2017-10-25 M. M. Lacerda , F. Kargar , E. Aytan , R. Samnakay , B. Debnath , J. X. Li , A. Khitun , R. K. Lake , J. Shi , A. A. Balandin

We report results of Raman scattering experiments on twin-free BaFe$_{2}$As$_{2}$ with the main focus placed on understanding the influence of electronic and spin degrees of freedom on the lattice dynamics. In particular, we scrutinize the…

Strongly Correlated Electrons · Physics 2018-08-15 A. Baum , Ying Li , M. Tomić , N. Lazarević , D. Jost , F. Löffler , B. Muschler , T. Böhm , J. -H. Chu , I. R. Fisher , R. Valentí , I. I. Mazin , R. Hackl

The discovery of 2-dimensional (2D) materials, such as CrI3, that retain magnetic ordering at monolayer thickness has resulted in a surge of research in 2D magnetism from both pure and applied perspectives. Here, we report a magneto-Raman…

Raman scattering is used to observe pronounced electronic excitations around 230 meV - well above the two-phonon range - in the Mott insulators LaTiO$_3$ and YTiO$_3$. Based on the temperature, polarization, and photon energy dependence,…

Strongly Correlated Electrons · Physics 2007-05-23 C. Ulrich , A. Gössling , M. Grüninger , M. Guennou , H. Roth , M. Cwik , T. Lorenz , G. Khaliullin , B. Keimer

We report on the optical properties of undoped single crystal LaMnO_3, the parent compound of the colossal magneto-resistive manganites. Near-Normal incidence reflectance measurements are reported in the frequency range of 20-50,000 cm-1…

Strongly Correlated Electrons · Physics 2009-11-07 M. A. Quijada , J. R. Simpson , H. D. Drew , J. W. Lynn , L. Vasiliu-Doloc , Y. M. Mukovskii , S. G. Karabashev

We report inelastic light scattering studies on Ca(Fe0.97Co0.03)2As2 in a wide spectral range of 120-5200 cm-1 from 5K to 300K, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at Tsm ~ 160K. The…

Superconductivity · Physics 2014-07-11 Pradeep Kumar , D. V. S. Muthu , L. Harnagea , S. Wurmehl , B. Büchner , A. K. Sood

Two distinct ferromagnetic phases of LaMn$_{0.5}$Co$_{0.5}$O$_{3}$ having monoclinic structure with distinct physical properties have been studied. The ferromagnetic ordering temperature $\textit{T}_{c}$ is found to be different for both…

Strongly Correlated Electrons · Physics 2010-09-08 M. Viswanathan , P. S. Anil Kumar , Venkata Srinu Bhadram , Chandrabhas Narayana , A. K. Bera , S. M. Yusuf

We report a comprehensive Raman study of the phonon behaviour in PdSe$_2$ in the temperature range of 5 K to 300 K. A remarkable change in the Raman spectrum is observed at 120 K: a significant enhancement of the out-of-plane phonon…

Spin and lattice dynamics of CaMn7O12 ceramics were investigated using infrared, THz and inelastic neutron scattering (INS) spectroscopies in the temperature range 2 to 590 K, and, at low temperatures, in applied magnetic fields of up to 12…

We used a combination of polarized Raman spectroscopy and spin wave calculations to study magnetic excitations in the strong spin-orbit-coupled (SOC) bilayer perovskite antiferromagnet $Sr_3Ir_2O_7$. We observed two broad Raman features at…

Strongly Correlated Electrons · Physics 2020-08-24 Siwen Li , Elizabeth Drueke , Zach Porter , Wencan Jin , Zhengguang Lu , Dmitry Smirnov , Roberto Merlin , Stephen D. Wilson , Kai Sun , Liuyan Zhao

We present optical measurements of phononic excitations in La$_{2/3}$Ca$_{1/3}$MnO$_{3}$ (LCMO) and La$_{2/3}$Sr$_{1/3}$MnO$_{3}$ (LSMO) thin films covering the full temperature range from the metallic ferromagnetic to the insulating…

Strongly Correlated Electrons · Physics 2010-05-24 Ch. Hartinger , F. Mayr , A. Loidl , T. Kopp

Fe$^{3+}$ $S = 5/2$ ions form saw-tooth like chains along the $a$ axis of the oxo-selenite Fe$_2$O(SeO$_3$)$_2$ and an onset of long-range magnetic order is observed for temperatures below $T_C = 105$ K. This order leads to distinct…

The lattice dynamics of the $\rm YMnO_3$ magneto-electric compound has been investigated using density functional calculations, both in the ferroelectric and the paraelectric phases. The coherence between the computed and experimental data…

Materials Science · Physics 2012-03-09 Julien Varignon , Sébastien Petit , Marie-Bernadette Lepetit

We report on resonance Raman spectroscopy measurements with excitation photon energy down to 1.16 eV on graphene, to study how low-energy carriers interact with lattice vibrations. Thanks to the excitation energy close to the Dirac point at…

Lattice dynamics and magnetic excitations are investigated to elucidate the origin of magneto-dielectric effects in the S=1/2 two-dimensional quantum spin compound K$_2$V$_3$O$_8$. We find evidence for lattice instabilities at 110 K and 60…

Strongly Correlated Electrons · Physics 2015-06-04 K. -Y. Choi , P. Lemmens , V. P. Gnezdilov , B. C. Sales , M. D. Lumsden

We report a Raman scattering investigation of multiferroic bismuth ferrite BiFeO3 epitaxial (c-axis oriented) thin films from -192 to 1000C. Phonon anomalies have been observed in three temperature regions: in the gamma-phase from 930C to…

Materials Science · Physics 2015-05-14 R. Palai , J. F. Scott , R. S. Katiyar

Spin-phonon coupling originated from spin-lattice correlation depends upon different exchange interactions in transition metal oxides containing 3d magnetic ions. Spin-lattice coupling can influence the coupling mechanism in magnetoelectric…

Strongly Correlated Electrons · Physics 2021-09-09 P. Pal , Shalini Badola , P. K. Biswas , Ranjana R. Das , Surajit Saha , S. D. Kaushik , P. N. Vishwakarma , A. K. Singh

Low-energy magnon excitations in multiferroic BiFeO$_3$ were measured in detail as a function of temperature around several Brillouin zone centers by inelastic neutron scattering experiments on single crystals. Unique features around 1 meV…

Materials Science · Physics 2014-09-15 Jaehong Jeong , Manh Duc Le , P. Bourges , S. Petit , S. Furukawa , Shin-Ae Kim , Seongsu Lee , S-W. Cheong , Je-Geun Park

Multiferroics possess two or more switchable states such as polarization, magnetization, etc. Phonon excitations in multiferroic phase are strongly modified by magnetoelectric coupling, spin-phonon coupling, and anharmonic phonon-phonon…

Materials Science · Physics 2021-10-26 Bommareddy Poojitha , Ankit Kumar , Anjali Rathore , Surajit Saha
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