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We use density functional theory (DFT) to study the thermodynamic stability and migration of copper ions and small clusters embedded in amorphous silicon dioxide. We perform the calculations over an ensemble of statistically independent…

Materials Science · Physics 2015-06-11 David M. Guzman , Nicolas Onofrio , Alejandro Strachan

The performance of modern electronics is associated with the multi-layered interconnects, encouraging the development of a low-k dielectrics. Herein, we studied the effects of phase transition from crystalline to amorphous on dielectric,…

It is demonstrated here that growth stress has a substantial effect on the dielectric constant of zirconia thin films. The correct combination of parameters - phase, texture and stress - is shown to yield films with high dielectric constant…

Magnetic dc susceptibility between 1.5 and 800 K, ac susceptibility and magnetization, thermodynamic properties, temperature dependence of radio and audio-wave dielectric constants and conductivity, contact-free dielectric constants at…

Materials Science · Physics 2010-07-22 Jun Lu , A. Günther , F. Schrettle , F. Mayr , S. Krohns , P. Lunkenheimer , A. Pimenov , V. D. Travkin , A. A. Mukhin , A. Loidl

A thorough investigation of the dielectric properties of Cu2Ta4O12, a material crystallizing in a pseudo-cubic, perovskite-derived structure is presented. We measured the dielectric constant and conductivity of single crystals in an…

Materials Science · Physics 2009-11-10 B. Renner , P. Lunkenheimer , M. Schetter , A. Loidl , A. Reller , S. G. Ebbinghaus

An electrode contact-related mechanism for the operational instability of organic electronic devices is proposed and confirmed via observation of a water-induced change in charge-injection barrier eights at the…

Applied Physics · Physics 2020-01-28 Ryo Nouchi

Frequency dependence of the dielectric constant of complex perovskite oxide Ba(1-x)La(x)Ti(1-x)Cr(x)O3 (BLTC) ceramics with the composition ratio 0.4<= x <= 0.7 is precisely measured in the temperature range from 20 K to 300 K, and the…

Materials Science · Physics 2007-05-23 Mamoru Fukunaga , Yoshiaki Uesu

The dielectric properties of molecules or nanostructures are usually modified in a complex manner, when assembled into a condensed phase. We propose a first-principles method to compute polarizabilities of sub-entities of solids and…

Chemical Physics · Physics 2018-09-10 Ding Pan , Marco Govoni , Giulia Galli

Layered narrow band gap semiconductor Bi2Se3 is composed of heavy elements with strong spin-orbital coupling (SOC), which has been identified both as a good candidate of thermoelectric material of high thermoelectric figure-of-merit (ZT)…

Materials Science · Physics 2018-04-04 G. J. Shu , S. C. Liou , S. K. Karna , R. Sankar , M. Hayashi , F. C. Chou

In condensed-matter systems, competition between ground states at phase boundaries can lead to significant changes in material properties under external stimuli, particularly when these ground states have different crystal symmetries. A key…

In the present work we demonstrate that in addition to the well-known colossal-dielectric-constant material CaCu3Ti4O12 also various members of the series Ln2/3Cu3Ti4O12 with Ln = La, Ce, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Ho, Er and Tm, exhibit…

Materials Science · Physics 2010-03-25 J. Sebald , S. Krohns , P. Lunkenheimer , S. G. Ebbinghaus , S. Riegg , A. Reller , A. Loidl

Structural and electronic properties of amorphous and single-phase polycrystalline films of gamma- and kappa-In2Se3 have been measured. The stable gamma phase nucleates homogeneously in the film bulk and has a high resistivity, while the…

Materials Science · Physics 2009-11-10 A. Chaiken , K. Nauka , G. A. Gibson , Heon Lee , C. C. Yang , J. Wu , J. W. Ager , K. M. Yu , W. Walukiewicz

The addition of electron donors to the vacant A site of defect-perovskite structure tungsten trioxide causes a series of structural and chemical phase transitions; for instance, in the well-known case of the sodium tungsten bronzes…

Materials Science · Physics 2009-11-10 Andrew D. Walkingshaw , Nicola A. Spaldin , Emilio Artacho

The coupling between localized spins and phonons can lead to shifts in the dielectric constant of insulating materials at magnetic ordering transitions. Studies on isostructural SeCuO3 (ferromagnetic) and TeCuO3 (antiferromagnetic)…

Materials Science · Physics 2009-04-14 G. Lawes , T. Kimura , C. M. Varma , M. A. Subramanian , R. J. Cava , A. P. Ramirez

Using finite-temperature phonon calculations and the Lyddane-Sachs-Teller relations, we calculate ab initio the static dielectric constants of 78 semiconducting oxides and fluorides with cubic perovskite structures at 1000 K. We first…

Materials Science · Physics 2020-11-26 Ambroise van Roekeghem , Jesús Carrete , Stefano Curtarolo , Natalio Mingo

The octahedron tilt transitions of ABX_3 perovskite-structure materials lead to an anti-polar (or antiferroelectric) arrangement of dipoles, with the low temperature structure having six sublattices polarized along various crystallographic…

Strongly Correlated Electrons · Physics 2013-05-29 Philip B. Allen , Yiing-Rei Chen , Santanu Chaudhuri , Clare P. Grey

We present out-of-plane dielectric and magnetodielectric measurements of single crystallines $\alpha$-RuCl$_3$ with various degrees of stack faults. A frequency dependent, but field independent, dielectric anomaly appears at…

In this paper, we compare the structural features of Ca modified Ba(Ti, Sn)O3 with that of its Ca-free counterpart to understand why the Ca-modified variant of this lead-free piezoelectric gives a much higher piezoelectric response. We…

Materials Science · Physics 2017-09-19 Mulualem Abebe , Kumar Brajesh , Anupam Mishra , Anatoliy Senyshyn , Rajeev Ranjan

Materials with ring-shaped electronic bands are promising thermoelectric candidates, since their unusual dispersion shape is predicted to give large power factors. While previous calculations of these materials have relied on the assumption…

Mesoscale and Nanoscale Physics · Physics 2021-04-14 Cameron Rudderham , Jesse Maassen

An electro-optic modulator offers the function of modulating the propagation of light in a material with electric field and enables seamless connection between electronics-based computing and photonics-based communication. The search for…

Materials Science · Physics 2022-05-11 Yang Liu , Guodong Ren , Tengfei Cao , Rohan Mishra , Jayakanth Ravichandran