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Related papers: Recent advances in pulsed-laser deposition of comp…

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Pulsed laser deposition (PLD) is a popular growth method, which has been successfully used for fabricating thin films. Compared to continuous deposition (like molecular beam epitaxy) the pulse intensity can be used as an additional…

Statistical Mechanics · Physics 2007-05-23 B. Hinnemann , F. Westerhoff , D. E. Wolf

In this chapter we will describe a new development of combinatorial pulsed laser deposition (CPLD) which targets the exploration of interface libraries. The idea is to modulate continuously the composition of interfaces on a few atomic…

Materials Science · Physics 2020-12-08 Jerome Wolfman , Beatrice Negulescu , Antoine Ruyter , Ndioba Niang , Nazir Jaber

This paper shows how data-driven machine learning approaches can improve growth control, reproducibility, and physical insight in the pulsed laser deposition (PLD) growth of correlated oxides. Despite well-known relationships between growth…

A novel continuous-compositional spread technique based on the non-uniformity of the deposition rate typically observed in Pulsed Laser Deposition (PLD) is introduced. The approach uses the spatial variations in the deposition-rate…

Materials Science · Physics 2009-11-07 H. M. Christen , S. D. Silliman , K. S. Harshavardhan

Pulsed laser deposition (PLD) is a versatile technique for growing epitaxial heterostructures of a wide variety of novel materials combinations. Achieving low-defect layers with atomically sharp interfaces by PLD requires careful management…

Applied Physics · Physics 2021-05-12 Sumner B. Harris , Kamron L. Kopekcy , Chandler W. Cotton , Renato P. Camata

Materials synthesis platforms that are designed for autonomous experimentation are capable of collecting multimodal diagnostic data that can be utilized for feedback to optimize material properties. Pulsed laser deposition (PLD) is emerging…

Materials Science · Physics 2024-11-01 Sumner B. Harris , Christopher M. Rouleau , Kai Xiao , Rama K. Vasudevan

Pulsed Laser Deposition (PLD) is widely used to grow epitaxial thin films of quantum materials such as complex oxides. Here, we use in-situ X-ray scattering to study homoepitaxy of SrTiO$_3$ by energetic (e-) and thermalized (th-) PLD. We…

In this article kinetic Monte Carlo simulations for molecular beam epitaxy (MBE) and pulsed laser depositon (PLD) are compared. It will be shown that an optimal pattern conservation during MBE is achieved for a specific ratio of diffusion…

Statistical Mechanics · Physics 2007-05-23 F. Westerhoff , L. Brendel , D. E. Wolf

It has been observed experimentally that under certain conditions pulsed laser deposition (PLD) produces smoother surfaces than ordinary molecular beam epitaxy (MBE). So far the mechanism leading to the improved quality of surfaces in PLD…

Statistical Mechanics · Physics 2009-11-07 Berit Hinnemann , Haye Hinrichsen , Dietrich E. Wolf

Pulsed Laser Deposition (PLD) of homoepitaxial SrTiO3 <001> was studied with in-situ x-ray specular reflectivity and surface diffuse x-ray scattering. Unlike prior reflectivity-based studies, these measurements access both the time- and the…

Materials Science · Physics 2015-05-14 J. D. Ferguson , G. Arikan , D. S. Dale , A. R. Woll , J. D. Brock

A new method for continuous compositional-spread (CCS) thin-film fabrication based on pulsed-laser deposition (PLD) is introduced. This approach is based on a translation of the substrate heater and the synchronized firing of the excimer…

Materials Science · Physics 2009-11-10 H. M. Christen , C. M. Rouleau , I. Ohkubo , H. Y. Zhai , H. N. Lee , S. Sathyamurthy , D. H. Lowndes

Variations in growth conditions associated with different deposition techniques can greatly affect the phase stability and defect structure of complex oxide heterostructures. We synthesized superlattices of the paramagnetic metal LaNiO3 and…

Strongly Correlated Electrons · Physics 2017-01-31 F. Wrobel , A. F. Mark , G. Christiani , W. Sigle , H. -U. Habermeier , P. A. van Aken , G. Logvenov , B. Keimer , E. Benckiser

In this paper, we introduce the proper latent decomposition (PLD) as a generalization of the proper orthogonal decomposition (POD) on manifolds. PLD is a nonlinear reduced-order modeling technique for compressing high-dimensional data into…

Machine Learning · Computer Science 2024-12-03 Daniel Kelshaw , Luca Magri

Here we systematically explore the use of pulsed laser deposition technique (PLD) to grow three basic oxides that have rocksalt structure but different chemical stability in the ambient atmosphere: NiO (stable), MnO (metastable) and EuO…

Materials Science · Physics 2020-01-08 Alireza Kashir , Hyeon-Woo Jeong , Gil-ho Lee , Pavlo Mikheenko , Yoon Hee Jeong

Recently, Bi2O2Se is discovered as a promising two-dimensional (2D) semiconductor for next generation electronics, due to its moderate bandgap size, high electron mobility and pronounced ambient stability. Meanwhile, it has been predicted…

Materials Science · Physics 2020-02-19 Yekai Song , Zhuojun Li , Hui Li , Shujie Tang , Gang Mu , Lixuan Xu , Wei Peng , Dawei Shen , Yulin Chen , Xiaoming Xie , Mianheng Jiang

The authors report in situ Auger electron spectroscopy (AES) of the surfaces of complex oxides thin films grown by pulsed laser deposition (PLD). The authors demonstrate the utility of the technique in studying chemical composition by…

Materials Science · Physics 2021-02-10 Thomas Orvis , Mythili Surendran , Yang Liu , Austin Cunniff , Jayakanth Ravichandran

We report that epitaxial Sr2IrO4 thin-films can be selectively grown using pulsed laser deposition (PLD). Due to the competition between the Ruddlesden-Popper phases of strontium iridates (Sr_{n+1}Ir_{n}O_{3n+1}), conventional PLD methods…

Strongly Correlated Electrons · Physics 2016-12-06 S. S. A. Seo , J. Nichols , J. Hwang , J. Terzic , J. H. Gruenewald , M. Souri , J. Thompson , J. G. Connell , G. Cao

A template-free process for the synthesis of nanocrystalline TiO2 hierarchical microstructures by reactive Pulsed Laser Deposition (PLD) is here presented. By a proper choice of deposition parameters a fine control over the morphology of…

Materials Science · Physics 2013-11-28 F. Di Fonzo , C. S. Casari , V. Russo , M. F. Brunella , A. Li Bassi , C. E. Bottani

Two-dimensional (2D) Ruddlesden-Popper (RP) Metal Halides present unique and tunable properties. However, direct and oriented synthesis is challenging due to low formation energies that lead to rapid, uncontrolled growth during…

In this paper, we report the growth of NaxCoO2 thin films by pulsed-laser deposition (PLD). It is shown that the concentration of sodium is very sensitive to the substrate temperature and the target-substrate distance due to the evaporation…

Materials Science · Physics 2007-05-23 X. P. Zhang , Y. S. Xiao , H. Zhou , B. T. Xie , C. X. Yang , Y. G. Zhao
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