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PbTiO$_3$ is a ferroelectric perovskite semiconductor with favourable electronic and optical properties, making it suitable for a wide range of applications, including photo-catalysis and (opto)electronic devices. Despite its relevance, an…

Materials Science · Physics 2025-12-03 Pietro Pacchioni , Lorenzo Varrassi , Cesare Franchini

The structural and polar properties of BiFeO3 at finite temperature are investigated using an atomistic shell model fitted to first-principles calculations. Molecular Dynamics simulations show a direct transition from the low-temperature…

Materials Science · Physics 2015-06-23 M. Graf , M. Sepliarsky , S. Tinte , M. G. Stachiotti

Ferroelectricity has been believed unable to coexist with metallicity since the free carriers can screen the internal coulomb interactions of dipoles. Very recently, one kind of materials called as ferroelectric metal was reexamined. Here,…

Materials Science · Physics 2017-11-08 Jun-xing Gu , Kui-juan Jin , Chao Ma , Qing-hua Zhang , Lin Gu , Chen Ge , Jie-su Wang , Hai-zhong Guo , Guo-zhen Yang

Ferroelectricity-the switchable intrinsic electric polarization-has not yet been attained in a metal experimentally and is in fact generally deemed irreconcilable with free carriers, although polar metal has been achieved recently.…

Recent advances in moire engineering provide new pathways for manipulating lattice distortions and electronic properties in low-dimensional materials. Here, we demonstrate that twisted stacking can induce dipolar vortices in metallic SrRuO3…

\ We combine density functional theory and molecular dynamics simulations to investigate the impact of Sr concentration and atomic ordering on the structural and ferroelectric properties of (Ba, Sr)TiO$_3$. On one hand, the macroscopic…

Materials Science · Physics 2023-08-28 Aris Dimou , Ankita Biswas , Anna Gruenebohm

Macroscopic polarization, both of intrinsic and piezoelectric nature, is unusually strong in III-V nitrides, and the built in electric fields in the layers of nitride-based nanostructures, stemming from polarization changes at…

Materials Science · Physics 2009-10-31 Fabio Bernardini , Vincenzo Fiorentini

The intrinsic d.c. electrical resistivity ($\rho$) - measurable on single crystals only - is often the quantity first revealing the properties of a given material. In the case of CH$_3$NH$_3$PbI$_3$ perovskite measuring $\rho$ under white…

Strongly Correlated Electrons · Physics 2016-04-20 A. Pisoni , J. Jacimovic , B. Náfrádi , P. Szirmai , M. Spina , R. Gaál , K. Holczer , E. Tutis , L. Forró , E. Horváth

Magnetic Tunnel Junctions whose basic element consists of two ferromagnetic electrodes separated by an insulating non-magnetic barrier have become intensely studied and used in non-volatile spintronic devices. Since ballistic tunnel of…

A method for the calculation of the temperature dependence of dielectric and piezoelectric responses, based on the use of a first-principles effective Hamiltonian, is described. Results are presented for the ferroelectric perovskite PbTiO3.…

Materials Science · Physics 2009-10-31 Karin M. Rabe , Eric Cockayne

This review devoted to multiferroic properties of Bismuth-based perovskites falls into two parts. The first part focuses on BiFeO3 and summarizes the recent progress made in the studies of its pressure-temperature phase diagram and…

Materials Science · Physics 2015-02-03 Mael Guennou , Michel Viret , Jens Kreisel

Polar topologies, such as vortex and skyrmion, have attracted significant interest due to their unique physical properties and promising applications in high-density memory devices. Currently, most polar vortices are observed in…

Applied Physics · Physics 2024-04-15 Haozhi Sha , Yixuan Zhang , Yunpeng Ma , Wei Li , Wenfeng Yang , Jizhe Cui , Qian Li , Houbing Huang , Rong Yu

We study the antiferrodistortive instability and its interaction with ferroelectricity in cubic perovskite compounds. Our first-principles calculations show that coexistence of both instabilities is very common. We develop a…

mtrl-th · Physics 2008-02-03 W. ~Zhong , David Vanderbilt

The occurence of spin-polarization at ZrO$_{2}$, Al$_{2}$O$_{3}$ and MgO surfaces is proved by means of \textit{ab-initio} calculations within the density functional theory. Large spin moments, as high as 1.56 $\mu_B$, develop at O-ended…

Materials Science · Physics 2009-11-11 S. Gallego , J. I. Beltran , J. Cerda , M. C. Munoz

Perovskite metal-organic frameworks (MOFs) have recently emerged as potential candidates for multiferroicity. However, the compounds synthesized so far possess only weak ferromagnetism and low polarization. Additionally, the very low…

Materials Science · Physics 2018-01-24 Paresh Chandra Rout , Varadharajan Srinivasan

We use density functional theory calculations to show that the LaAlO3|SrTiO3 interface between insulating perovskite oxides is borderline in satisfying the Stoner criterion for itinerant ferromagnetism and explore other oxide combinations…

Materials Science · Physics 2014-09-17 Nirmal Ganguli , Paul J. Kelly

A dielectric anomaly has been found near the incommensurate to commensurate antiferromagnetic phase transition (TN2=230 K) in YBaCuFeO5 ceramics, a compound which crystallizes in an ordered perovskite structure. The existence of electric…

Materials Science · Physics 2009-03-13 B. Kundys , A. Maignan , Ch. Simon

The ferroelectric trends of rutile (TiO$_2$) in bulk and at the (110) surface are investigated by means of ab initio density functional theory. We discuss the underlying mechanism of the incipient ferroelectric behavior of rutile in terms…

Materials Science · Physics 2015-06-12 Anna Grünebohm , Peter Entel , Claude Ederer

Ferroelectric materials display exotic polarization textures at the nanoscale that could be used to improve the energetic efficiency of electronic components. The vast majority of studies were conducted in two dimensions on thin films, that…

We use density functional theory to investigate the possibility of polar and multiferroic states in free-standing, perovskite-based nanodots at their limit of miniaturization: single unit cell with termination to allow centrosymmetry. We…

Materials Science · Physics 2019-11-12 Karthik Guda Vishnu , Samuel Temple Reeve , Alejandro Strachan
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