Related papers: An x-ray probe of laser-aligned molecules
The present work reports on the generation of short-pulse coherent extreme ultraviolet radiation of controlled polarization. The proposed strategy is based on high-order harmonics generated in pre-aligned molecules. Field-free molecular…
The spectrum of laser-plasma generated X-rays is very important, it characterizes electron dynamics in plasma and is basic for applications. However, the accuracies and efficiencies of existing methods to diagnose the spectrum of…
We present a novel method for probing the alignment of the molecular axis of an ultracold, nonpolar dimer. These results are obtained using diatomic $^{87}\textrm{Rb}_2$ molecules in the vibrational ground state of the lowest triplet…
It is demonstrated that strong laser pulses can introduce torsional motion in the axially chiral molecule 3,5-diflouro-3',5'-dibromo-biphenyl (DFDBrBPh). A nanosecond laser pulse spatially aligns the stereogenic carbon-carbon (C-C) bond…
Generation of collimated, quasi-monoenergetic electron beams (peak energy ~17-22MeV, divergence ~10mrad, energy spread ~20%) by interaction of Ti:sapphire laser pulse of 200fs duration, focussed to an intensity of ~ 2.1x10^18 W/cm^2,with an…
The pioneering experiments of linear spectroscopy were performed using flames in the 1800s, but nonlinear optical measurements had to wait until lasers became available in the twentieth century. Because the nonlinear cross section of…
We propose a novel approach for strong alignment of gas-phase molecules for experiments at arbitrary repetition rates. A high-intracavity-power continuous-wave laser will provide the necessary ac electric field of $\!10^{10}$-…
Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…
A full density-matrix simulation is performed for optical deflection of a barium monofluoride (BaF) beam. Pairs of counter-propagating laser pulses are used for stimulated absorption followed by stimulated emission. The scheme produces a…
This paper describes a 561 nm laser heterodyne interferometer that provides time-resolved measurements of line-integrated plasma electron density within the range of 10^15-10^18 cm^(-2). Such plasmas are produced by railguns on the Plasma…
Calculations relating to two experiments that demonstrate coherent control of preformed rubidium-85 molecules in a magneto-optical trap using ultrafast laser pulses are presented. In the first experiment, it is shown that pre-associated…
Angle-resolved photoemission spectroscopy with sub-micrometer spatial resolution ({\mu}-ARPES), has become a powerful tool for studying quantum materials. To achieve sub-micrometer or even nanometer-scale spatial resolution, it is important…
We devise a theory of x-ray absorption by symmetric-top molecules which are aligned by an intense optical laser. Initially, the density matrix of the system is composed of the electronic ground state of the molecules and a thermal ensemble…
We demonstrate the experimental realization of impulsive alignment of carbonyl sulfide (OCS) molecules at the Low Density Matter Beamline (LDM) at the free-electron laser FERMI. OCS molecules in a molecular beam were impulsively aligned…
We report the development of a fast rotating target to produce ultrashort incoherent X-ray pulses from bremsstrahlung. These short X-ray pulses are produced in the laser-plasma interaction of a 35 fs, 1 mJ pulse of a Ti:Sa laser of 1 kHz…
Rich soft X-ray emission lines of highly charged silicon ions (Si VI--Si XII) were observed by irradiating an ultra-intense laser pulse with width of 200 fs and energy of $\sim$90 mJ on the solid silicon target. The high resolution spectra…
Imaging the structure of molecules in transient excited states remains a challenge due to the extreme requirements for spatial and temporal resolution. Ultrafast electron diffraction from aligned molecules (UEDAM) provides atomic resolution…
We demonstrate laser cooling of barium monofluoride (138BaF) molecules. We use serrodynes to synthesize time-sequenced optical spectra that can be precisely tailored to the hyperfine structure of this heaviest non-radioactive alkaline earth…
Recent studies have demonstrated the possibility of accelerating electrons to MeV energies in ambient air using tightly focused laser configurations. In this article, we explore possible strategies to control and optimize the resulting…
Unraveling and controlling chemical dynamics requires techniques to image structural changes of molecules with femtosecond temporal and picometer spatial resolution. Ultrashort-pulse x-ray free-electron lasers have significantly advanced…