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We make use of the previously developed formalism for a monomer ensemble and include angular dependence of the segments of the polymer chains thus described. In particular we show how to deal with stiffness when the polymer chain is…

Soft Condensed Matter · Physics 2015-06-24 K. K. Muller-Nedebock , H. L. Frisch , J. K. Percus

The aim of this paper is to investigate the distribution of a continuous polymer in the presence of an attractive finitely supported potential. The most intricate behavior can be observed if we simultaneously and independently vary two…

Mathematical Physics · Physics 2020-12-04 L. Koralov , S. Molchanov , B. Vainberg

We consider the complex polymer system, consisting of ring polymer connected to the $f_1$-branched star-like structure, in good solvent in presence of structural inhomogeneities. We assume, that structural defects are correlated at large…

Soft Condensed Matter · Physics 2018-03-14 K. Haydukivska , V. Blavatska

It is commonly accepted that in concentrated solutions or melts high-molecular weight polymers display random-walk conformational properties without long-range correlations between subsequent bonds. This absence of memory means, for…

Soft Condensed Matter · Physics 2009-11-11 J. P. Wittmer , P. Beckrich , F. Crevel , C. C. Huang , A. Cavallo , T. Kreer , H. Meyer

We investigate, using numerical simulations, the conformations of isolated active ring polymers. We find that the their behaviour depends crucially on their size: short rings ($N \lesssim$ 100) are swelled whereas longer rings ($N \gtrsim$…

Soft Condensed Matter · Physics 2021-03-03 Emanuele Locatelli , Valentino Bianco , Paolo Malgaretti

Molecular dynamics simulation of a generic polymer model is applied to study melts of polymers with different types of intrinsic stiffness. Important static observables of the single chain such as gyration radius or persistence length are…

Soft Condensed Matter · Physics 2017-09-13 Roland Faller , Alexander Kolb , Florian Müller-Plathe

We study the dynamics of an ideal polymer chain in a crowded, viscoelastic medium and in the presence of active forces. The motion of the centre of mass and of individual monomers is calculated. On time scales that are comparable to the…

Soft Condensed Matter · Physics 2015-12-23 Hans Vandebroek , Carlo Vanderzande

The number of allowed configurations of a polymer is reduced by the presence of a repulsive surface resulting in an entropic force between them. We develop a method to calculate the entropic force, and detailed pressure distribution, for…

Statistical Mechanics · Physics 2014-02-11 Yosi Hammer , Yacov Kantor

We study dynamics of a Rouse polymer chain, which diffuses in a three-dimensional space under the constraint that one of its ends, referred to as the slip-link, may move only along a one-dimensional line containing randomly placed,…

Statistical Mechanics · Physics 2007-05-23 S. Nechaev , G. Oshanin , A. Blumen

We study the behavior of a flexible polymer chain in the presence of a low-molecular weight solvent in the vicinity of a liquid-gas critical point within the framework of a self-consistent field theory. The total free energy of the dilute…

Statistical Mechanics · Physics 2015-07-29 Yu. A. Budkov , A. L. Kolesnikov , N. Georgi , M. G. Kiselev

We computed the phase-separation behavior and effective interactions of colloid-polymer mixtures in the "protein limit", where the polymer radius of gyration is much larger than the colloid radius. For ideal polymers, the critical colloidal…

Soft Condensed Matter · Physics 2009-11-07 Peter G. Bolhuis , Evert Jan Meijer , Ard A. Louis

Ring polymers remain a major challenge to our current understanding of polymer dynamics. Experimental results are difficult to interpret because of the uncertainty in the purity and dispersity of the sample. Using both equilibrium and…

Soft Condensed Matter · Physics 2015-06-03 Jonathan D. Halverson , Gary S. Grest , Alexander Y. Grosberg , Kurt Kremer

In this paper, we analyze the effect of geometrical constraint on the conformational properties of an infinitely long linear semiflexible polymer chain confined in-between two constraints under good solvent condition in two dimensions. The…

Soft Condensed Matter · Physics 2020-12-29 Pramod Kumar Mishra

Molecular dynamics simulations were conducted to investigate the structural properties of melts of nonconcatenated ring polymers and compared to melts of linear polymers. The longest rings were composed of N=1600 monomers per chain which…

Soft Condensed Matter · Physics 2011-05-02 Jonathan D. Halverson , Won Bo Lee , Gary S. Grest , Alexander Y. Grosberg , Kurt Kremer

We consider the problem of undirected polymers (tied at the endpoints) in random environment, also known as the unoriented first passage percolation on the hypercube, in the limit of large dimensions. By means of the multiscale refinement…

Probability · Mathematics 2020-12-09 Nicola Kistler , Adrien Schertzer

We study the interplay between entropy and topological constraints for a polymer chain in which sliding rings (slip-links) enforce pair contacts between monomers. These slip-links divide a closed ring polymer into a number of sub-loops…

Statistical Mechanics · Physics 2009-11-07 Ralf Metzler , Andreas Hanke , Paul G. Dommersnes , Yacov Kantor , Mehran Kardar

Modeling of polymer chains has received a lot of attention in mathematics. In fact, probabilistic models that naturally arise in statistical mechanics have been widely studied by mathematicians for the very challenging and novel problems…

Probability · Mathematics 2007-05-23 Francesco Caravenna

We perform a Monte Carlo study of $N$-step self-avoiding walks, attached to the corner of an impenetrable wedge in two dimensions ($d=2$), or the tip of an impenetrable cone in $d=3$, of sizes ranging up to $N=10^6$ steps. We find that the…

Statistical Mechanics · Physics 2015-12-22 Yosi Hammer , Yacov Kantor

A cornerstone of modern polymer physics is the `Flory ideality hypothesis' which states that a chain in a polymer melt adopts `ideal' random-walk-like conformations. Here we revisit theoretically and numerically this pivotal assumption and…

Soft Condensed Matter · Physics 2015-06-25 J. P. Wittmer , P. Beckrich , J. Johner , A. N. Semenov , S. P. Obukhov , H. Meyer , J. Baschnagel

In this paper we derive the general equilibrium equations of a polymer chain with a noncircular cross section by the variation of the free energy functional. From the equilibrium equation of the elastic ribbon we derive analytically the…

Soft Condensed Matter · Physics 2008-05-21 Shumin Zhao , Shengli Zhang , Zhenwei Yao , Lei Zhang