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Orbital degree of freedom of electrons and its interplay with spin, charge and lattice degrees of freedom are one of the central issues in colossal magnetoresistive manganites. The orbital degree of freedom has until recently remained…

Strongly Correlated Electrons · Physics 2009-11-07 Sumio Ishihara , Sadamichi Maekawa

We have investigated orbital ordering in the half-doped manganite La$_{0.5}$Sr$_{1.5}$MnO$_4$, which displays spin, charge and orbital ordering, by means of unrestricted Hartree-Fock calculations on the multiband $p$-$d$ model. From recent…

Strongly Correlated Electrons · Physics 2009-11-11 K. Ebata , T. Mizokawa , A. Fujimori

Fe pnictides and related materials have been a topic of intense research for understanding the complex interplay between magnetism and superconductivity. Here we report on the magnetic structure of SrMn$_{2}$As$_{2}$ that crystallizes in a…

Strongly Correlated Electrons · Physics 2016-12-13 Pinaki Das , N. S. Sangeetha , Abhishek Pandey , Zackery A. Benson , T. W. Heitmann , D. C. Johnston , A. I. Goldman , A. Kreyssig

Contrary to conventional wisdom, our purified La2-2xSr1+2xMn2O7 crystals exhibit CE-type orbital and charge order as the low-temperature ground state for a hole doping level h = 0.5. For small deviations from h = 0.5, the high temperature…

Strongly Correlated Electrons · Physics 2007-05-23 Qing'An Li , K. E. Gray , H. Zheng , H. Claus , S. Rosenkranz , S. Nyborg Ancona , R. Osborn , J. F. Mitchell , Y. Chen , J. W. Lynn

The phase stability of the MgMn2O4 spinel has been studied by means of high-pressure X-ray diffraction for pressures up to 30 GPa. Two samples with different inversion degrees have been considered. Both spinels undergo a phase transition…

Materials Science · Physics 2009-11-10 Lorenzo Malavasi , Cristina Tealdi , Monica Amboage , M. Cristina Mozzati , Giorgio Flor

We report the observation of a magnetic polarization of the O\,$2p$-states in YMn$_2$O$_5$ through the use of soft X-ray resonant scattering at the oxygen $K$-edge. Remarkably, we find that the temperature dependence of the integrated…

Strongly Correlated Electrons · Physics 2015-03-19 S. Partzsch , S. B. Wilkins , J. P. Hill , E. Schierle , E. Weschke , D. Souptel , B. Büchner , J. Geck

We have analyzed the experimental evidence of charge and orbital ordering in La0.5Sr1.5MnO4 using first principles band structure calculations. Our results suggest the presence of two types of Mn sites in the system. One of the Mn sites…

Strongly Correlated Electrons · Physics 2009-11-07 Priya Mahadevan , K. Terakura , D. D. Sarma

Long range orbital order has been investigated in Fe$_{1-x}$Mn$_x$V$_2$O$_4$ as a function of doping (x) using first principles density functional theory calculations including the effects of Coulomb correlation and spin-orbit interaction…

Strongly Correlated Electrons · Physics 2016-05-25 Dibyendu Dey , T. Maitra , A. Taraphder

Roles of orbital degree of freedom of Mn ions in phase transition as a function of temperature and hole concentration in perovskite manganites are studied. It is shown that the orbital order-disorder transition is of the first order in the…

Strongly Correlated Electrons · Physics 2009-10-31 S. Okamoto , S. Ishihara , S. Maekawa

High energy x-ray diffraction is used to investigate the bulk oxygen ordering properties of YBa_2Cu_3O_{6+x}. Superstructures of Cu-O chains aligned along the b axis and ordered with periodicity ma, along the a axis have been observed. For…

We report powder and single crystal neutron diffraction measurements of the magnetic order in AMnBi2 (A = Sr and Ca), two layered manganese pnictides with anisotropic Dirac fermions on a Bi square net. Both materials are found to order at…

Strongly Correlated Electrons · Physics 2014-08-20 Y. F. Guo , A. J. Princep , X. Zhang , P. Manuel , D. Khalyavin , I. I. Mazin , Y. G. Shi , A. T. Boothroyd

We report a high-resolution neutron diffraction study on the orbitally-degenerate spin-1/2 hexagonal antiferromagnet AgNiO2. A structural transition to a tripled unit cell with expanded and contracted NiO6 octahedra indicates root(3) x…

Strongly Correlated Electrons · Physics 2009-11-13 E. Wawrzynska , R. Coldea , E. M. Wheeler , I. I. Mazin , M. D. Johannes , T. Sorgel , M. Jansen , R. M. Ibberson , P. G. Radaelli

We present our theoretical results on the mechanism of two transitions in vanadium spinel oxides $A$V$_2$O$_4$ ($A$=Zn, Mg, or Cd) in which magnetic V cations constitute a geometrically-frustrated pyrochlore structure. We have derived an…

Strongly Correlated Electrons · Physics 2007-05-23 Yukitoshi Motome , Hirokazu Tsunetsugu

We present neutron scattering measurements on powder samples of the spinel FeSc2S4 that reveal a previously unobserved magnetic ordering transition occurring at 11.8(2)~K. Magnetic ordering occurs subsequent to a subtle cubic-to-tetragonal…

Strongly Correlated Electrons · Physics 2016-12-21 K. W. Plumb , Jennifer Morey , J. A. Rodriguez-Rivera , Hui Wu , A. A. Podlesnyak , T. M. McQueen , C. L. Broholm

By combining first-principles electronic-structure calculations with the model Hamiltonian approach, we systematically study the magnetic properties of sodium superoxide (NaO2), originating from interacting superoxide molecules. We show…

Materials Science · Physics 2013-12-19 I. V. Solovyev , Z. V. Pchelkina , V. V. Mazurenko

By resonant x-ray scattering at the Mn K-edge on La7/8Sr1/8MnO3, we show that an orbital polaron lattice (OPL) develops at the metal-insulator transition of this compound. This orbital reordering explains consistently the unexpected…

Strongly Correlated Electrons · Physics 2007-05-23 J. Geck , P. Wochner , S. Kiele , R. Klingeler , P. Reutler , A. Revcolevschi , B. Buechner

The structural, magnetic, and electronic properties of NdFe$_{0.5}$Mn$_{0.5}$O$_3$ have been studied in detail using bulk magnetization, neutron/x-ray diffraction and first principles density functional theory calculations. The material…

Strongly Correlated Electrons · Physics 2017-10-25 Ankita Singh , A. Jain , Avijeet Ray , B. Padmanabhan , S. M. Yusuf , T. Maitra , V. K. Malik

A-site ordered manganites LnBaMn1.96Fe0.04O5 and LnBaMn1.96Fe0.04O6 are investigated by x-ray full-profile diffraction and Moessbauer spectroscopy. Powder samples were oriented with preferred orientation of platy crystallites in the plane…

Materials Science · Physics 2009-06-21 A. I. Rykov , Y. Ueda , K. Nomura , M. Seto

New metal-ordered manganites RBaMn_{2}O_{6} have been synthesized and investigated in the structures and electromagnetic properties. RBaMn_{2}O_{6} can be classified into three groups from the structural and electromagnetic properties. The…

Strongly Correlated Electrons · Physics 2009-11-07 T. Nakajima , H. Kageyama , H. Yoshizawa , Y. Ueda

We use neutron powder diffraction to study on the non-superconducting phases of ThFeAsN$_{1-x}$O$_x$ with $x=0.15, 0.6$. In our previous results on the superconducting phase ThFeAsN with $T_c=$ 30 K, no magnetic transition is observed by…

Superconductivity · Physics 2019-09-05 Huican Mao , Bingfeng Hu , Yuanhua Xia , Xiping Chen , Cao Wang , Zhicheng Wang , Guanghan Cao , Shiliang Li , Huiqian Luo