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Collinear antiferromagnetism in trigonal SrMn$_{2}$As$_{2}$ revealed by single-crystal neutron diffraction

Strongly Correlated Electrons 2016-12-13 v1

Abstract

Fe pnictides and related materials have been a topic of intense research for understanding the complex interplay between magnetism and superconductivity. Here we report on the magnetic structure of SrMn2_{2}As2_{2} that crystallizes in a trigonal structure (P3ˉm1P\bar{3}m1) and undergoes an antiferromagnetic (AFM) transition at TcT_{\textrm c} =118(2)= 118(2) K. The magnetic susceptibility remains nearly constant at temperatures TTNT \le T_{\textrm N} with Hc\textbf{H}\parallel \textbf{c} whereas it decreases significantly with Hab\textbf{H}\parallel \textbf{ab}. This shows that the ordered Mn moments lie in the ab\textbf{ab}-plane instead of aligning along the c\textbf{c}-axis as in tetragonal BaMn2_{2}As2_{2}. Single-crystal neutron diffraction measurements on SrMn2_{2}As2_{2} demonstrate that the Mn moments are ordered in a collinear N\'{e}el AFM phase with 180180^\circ AFM alignment between a moment and all nearest neighbor moments in the basal plane and also perpendicular to it. Moreover, quasi-two-dimensional AFM order is manifested in SrMn2_{2}As2_{2} as evident from the temperature dependence of the order parameter.

Keywords

Cite

@article{arxiv.1605.02004,
  title  = {Collinear antiferromagnetism in trigonal SrMn$_{2}$As$_{2}$ revealed by single-crystal neutron diffraction},
  author = {Pinaki Das and N. S. Sangeetha and Abhishek Pandey and Zackery A. Benson and T. W. Heitmann and D. C. Johnston and A. I. Goldman and A. Kreyssig},
  journal= {arXiv preprint arXiv:1605.02004},
  year   = {2016}
}

Comments

5 pages, 3 figures