Fe pnictides and related materials have been a topic of intense research for understanding the complex interplay between magnetism and superconductivity. Here we report on the magnetic structure of SrMn2As2 that crystallizes in a trigonal structure (P3ˉm1) and undergoes an antiferromagnetic (AFM) transition at Tc=118(2) K. The magnetic susceptibility remains nearly constant at temperatures T≤TN with H∥c whereas it decreases significantly with H∥ab. This shows that the ordered Mn moments lie in the ab-plane instead of aligning along the c-axis as in tetragonal BaMn2As2. Single-crystal neutron diffraction measurements on SrMn2As2 demonstrate that the Mn moments are ordered in a collinear N\'{e}el AFM phase with 180∘ AFM alignment between a moment and all nearest neighbor moments in the basal plane and also perpendicular to it. Moreover, quasi-two-dimensional AFM order is manifested in SrMn2As2 as evident from the temperature dependence of the order parameter.
@article{arxiv.1605.02004,
title = {Collinear antiferromagnetism in trigonal SrMn$_{2}$As$_{2}$ revealed by single-crystal neutron diffraction},
author = {Pinaki Das and N. S. Sangeetha and Abhishek Pandey and Zackery A. Benson and T. W. Heitmann and D. C. Johnston and A. I. Goldman and A. Kreyssig},
journal= {arXiv preprint arXiv:1605.02004},
year = {2016}
}