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We derive the low temperature properties of the molecular magnet Mo72Fe30, where 30 Fe(3+) paramagnetic ions occupy the sites of an icosidodecahedron and interact via isotropic nearest-neighbour antiferromagnetic Heisenberg exchange. The…

Materials Science · Physics 2009-11-07 J. Schnack , M. Luban , R. Modler

The magnetic properties and spin dynamics of the spin frustrated polyoxometalate {W72V30}, where 30 V^{4+} ions (s = 1/2) occupy the sites of an icosidodecahedron, have been investigated by low temperature magnetization, magnetic…

Strongly Correlated Electrons · Physics 2013-04-10 J. Schnack , A. M. Todea , A. Müller , H. Nojiri , S. Yeninas , Y. Furukawa , R. Prozorov , M. Luban

The classical Heisenberg model is applied in a Monte Carlo study to investigate the distance dependence of the indirect nearest neighbor (NN) exchange and next-nearest neighbor (NNN) superexchange interaction in EuO, EuS, EuSe and EuTe. For…

Materials Science · Physics 2010-05-10 W. Söllinger , W. Heiss , R. T. Lechner , K. Rumpf , P. Granitzer , H. Krenn , G. Springholz

We have found a class of zero-dimensional geometrically frustrated Heisenberg spin systems exhibiting anomalous behavior in an external magnetic field B similar to that occuring in geometrically frustrated planar antiferromagnetic lattices.…

Materials Science · Physics 2009-11-10 C. Schroeder , H. Nojiri , J. Schnack , P. Hage , M. Luban , P. Koegerler

We show that the magnetism of double perovskite AFe_{1/2}M_{1/2}O_3 systems may be described by the Heisenberg model on the simple cubic lattice, where only half of sites are occupied by localized magnetic moments. The nearest-neighbor…

Materials Science · Physics 2015-01-16 R. O. Kuzian , I. V. Kondakova , A. -M. Dare , V. V. Laguta

The generalized Heusler compounds Mn2CoZ (Z = Al, Ga, In, Si, Ge, Sn, Sb) with the Hg2CuTi structure are of large interest due to their half-metallic ferrimagnetism. The complex magnetic interactions between the constituents are studied by…

Materials Science · Physics 2011-03-07 Markus Meinert , Jan-Michael Schmalhorst , Günter Reiss

The magnetic properties of the diluted magnetic semiconductors (DMS) (Ga, Mn)As and (Ga, Mn)N are investigated by means of an effective Heisenberg model, whose exchange parameters are obtained from first-principle calculations. The…

Materials Science · Physics 2007-05-23 S. Hilbert , W. Nolting

The electronic and magnetic properties of K$_{2}$CuP$_{2}$O$_{7}$ were investigated by means of susceptibility, specific heat and $^{31}$P nuclear magnetic resonance (NMR) measurements and by LDA band structure calculations. The temperature…

Strongly Correlated Electrons · Physics 2009-11-13 R. Nath , Deepa Kasinathan , H. Rosner , M. Baenitz , C. Geibel

Magnetic materials are typically described in terms of the Heisenberg model, which provides an accurate account of thermodynamic properties when combined with first principles calculations. This approach is usually based on an energy…

Materials Science · Physics 2020-12-04 Daniele Torelli , Thomas Olsen

Magnetic properties of a tetrahedral "Ni_4" molecule are discussed in terms of the Heisenberg model, with magnetic anisotropy terms included, and on the basis of first-principle calculations within the density functional theory. It is shown…

Materials Science · Physics 2007-05-23 A. V. Postnikov , M. Brueger , J. Schnack

The two-dimensional (2D) van der Waals ferromagnetic semiconductors, such as CrI$_3$ and Cr$_2$Ge$_2$Te$_6$, and the 2D ferromagnetic metals, such as Fe$_3$GeTe$_2$ and MnSe$_2$, have been obtained in recent experiments and attracted a lot…

Materials Science · Physics 2023-12-29 Jia-Wen Li , Zhen Zhang , Jing-Yang You , Bo Gu , Gang Su

An ab initio study of magnetic exchange interactions in antiferromagnetic and strongly correlated 3d transition metal monoxides is presented. Their electronic structure is calculated using the local self-interaction correction approach,…

The exchange interaction is investigated theoretically for electrons confined to a 2-D sample placed in a linearly varying magnetic field perpendicular to the plane. Unusual and interesting behavior is predicted: starting from zero, as one…

Strongly Correlated Electrons · Physics 2020-12-30 Pervez Hoodbhoy

Defects intentionally introduced into magnetic materials often have a profound effect on the physical properties. Specifically tailored neutron spectroscopic experiments can provide detailed information on both the local exchange…

Materials Science · Physics 2017-02-28 Albert Furrer

We investigate the effect of chemical disorder on the magnetic exchange couplings and the Curie temperature ($T_{\text{c}}$) in L1$_0$-ordered FeNi using first-principles-based calculations. We use supercells to model chemical disorder, to…

Materials Science · Physics 2022-05-11 Ankit Izardar , Claude Ederer

We discuss new high-field magnetization data recently obtained by Tsirlin et al. for layered vanadium phosphates in the framework of the square-lattice model. Our predictions for the saturation fields compare exceptionally well to the…

Strongly Correlated Electrons · Physics 2010-05-07 Burkhard Schmidt , Mohammad Siahatgar , Peter Thalmeier , Alexander A. Tsirlin

Magnetism in single-side hydrogenated (C$_2$H) and fluorinated (C$_2$F) graphene is analyzed in terms of the Heisenberg model with parameters determined from first principles. We predict a frustrated ground state for both systems, which…

Mesoscale and Nanoscale Physics · Physics 2014-06-03 A. N. Rudenko , F. J. Keil , M. I. Katsnelson , A. I. Lichtenstein

In numerous diluted magnetic semiconductor (DMS) systems, the competition takes place between the short-range antiferromagnetic (AF) superexchange interactions and the long-range Ruderman-Kittel-Kasuya-Yosida (RKKY) coupling mediated by the…

Materials Science · Physics 2016-10-04 K. Szalowski

Theoretical prediction of the 2nd-order magnetic transition temperature (TM) used to be arduous. Here, we develop a first principle-based, fully automatic structure-to-TM method for two-dimensional (2D) magnets whose effective Hamiltonians…

Materials Science · Physics 2023-12-08 Haichang Lu , Tai Yang , Zhimei Sun , John Robertson , Weisheng Zhao

A path integral ground state approach has been used to estimate the ground-state energy and structural properties of hydrogen fluoride molecules pinned to a one-dimensional lattice. In the simulations, the molecules are assumed to be rigid,…

Chemical Physics · Physics 2023-08-10 Tapas Sahoo , Gautam Gangopadhyay
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