English

Nearest-neighbour antiferromagnetic interaction as a limiting factor for critical temperature in model DMS system

Materials Science 2016-10-04 v1 Mesoscale and Nanoscale Physics Statistical Mechanics

Abstract

In numerous diluted magnetic semiconductor (DMS) systems, the competition takes place between the short-range antiferromagnetic (AF) superexchange interactions and the long-range Ruderman-Kittel-Kasuya-Yosida (RKKY) coupling mediated by the charge carriers. Such a situation strongly influences the critical temperature, the maximization of which constitutes a challenging task in DMS physics and technology. The aim of the paper is to discuss theoretically the limiting effect of AF interactions between nearest-neighbour magnetic ions on the stability of inhomogeneous ferromagnetic state in a model diluted magnetic system reflecting some crucial features of DMS. The modified molecular field-based model is constructed to account for the magnetic inhomogeneity. The behavior of the system is studied as a function of the ratio of superexchange integral to effective ferromagnetic coupling integral, including the possibility of clustering/anticlustering tendency for the magnetic ions. The ground state of the system is analysed. The critical temperature is found to change non-monotonically with the concentration of magnetic ions and decrease severely for larger concentrations. The behavior of the system significantly differs from the predictions of the usual homogeneous mean-field model. Brief comparison with selected experimental results for (Zn,Mn)Te is provided.

Keywords

Cite

@article{arxiv.1610.00310,
  title  = {Nearest-neighbour antiferromagnetic interaction as a limiting factor for critical temperature in model DMS system},
  author = {K. Szalowski},
  journal= {arXiv preprint arXiv:1610.00310},
  year   = {2016}
}
R2 v1 2026-06-22T16:08:06.788Z