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How fast can a laser pulse ionize an atom? We address this question by considering pulses that carry a fixed time-integrated energy per-area, and finding those that achieve the double requirement of maximizing the ionization that they…

Atomic Physics · Physics 2017-06-07 David Kammerlander , Alberto Castro , Miguel A. L. Marques

We revisit the stabilization of ionization of atoms subjected to a superintense laser pulse using nonlinear dynamics. We provide an explanation for the lack of complete ionization at high intensity and for the decrease of the ionization…

Chaotic Dynamics · Physics 2015-06-23 Michael Norman , C. Chandre , T. Uzer , Peijie Wang

Based on numerical solutions of the time-dependent Schr\"odinger equation for either one or two active electrons, we propose a method for observing instantaneous level shifts in an oscillating strong infrared (IR) field in time, using a…

Atomic Physics · Physics 2015-05-28 Feng He , Camilo Ruiz , Andreas Becker , Uwe Thumm

A general method for solving numerically the time-dependent Schr\"odinger equation, that is based on the Suzuki-Trotter scheme with the split-step Fourier approach, is introduced. The method relies on a Hamiltonian decomposition, where…

Atomic Physics · Physics 2022-11-29 M. C. Suster , J. Derlikiewicz , K. Krajewska , F. Cajiao Vélez , J. Z. Kamiński

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

Atomic Physics · Physics 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

We investigate the effects of the multielectron polarization of the ion described by the induced dipole potential in photoelectron momentum distributions produced in ionization of the CO molecule by a strong laser field. We present results…

Atomic Physics · Physics 2024-04-23 Mahmoud Abu-samha , L. B. Madsen , N. I. Shvetsov-Shilovski

We theoretically investigate the mechanism of enhanced ionization in two-electron molecules by analyzing Bohmian trajectories for a one-dimensional H2 in an intense laser field. We identify both types of ionizing trajectories corresponding…

Quantum Physics · Physics 2015-06-17 Ryohto Sawada , Takeshi Sato , Kenichi L. Ishikawa

A simplified model of quantum electrodynamics involving a charged two-state system interacting with an electromagnetic field mode is examined. By extending the Schrodinger equation to include stochastic and nonlinear terms the dynamical…

Quantum Physics · Physics 2009-11-13 D. J. Bedingham

Ionization, excitation, and de-excitation to the ground state is studied theoretically for the first excited singlet state B $^1\Sigma_u^+$ of H$_2$ exposed to intense laser fields with photon energies in between about 3 eV and 13 eV. A…

Atomic Physics · Physics 2015-05-18 Manohar Awasthi , Alejandro Saenz

We study theoretically the dipole radiation of a hydrogen atom driven by an intense sub-cycle pulse. The time-dependent Schr\"odinger equation for the system is solved by ab initio calculation to obtain the dipole response. Remarkably, a…

Atomic Physics · Physics 2016-02-05 Wei-Chun Chu , John C. Travers , Philip St. J. Russell

We demonstrate how the shape of femtosecond laser pulses can be tailored in order to obtain maximal ionization of atoms or molecules. For that purpose, we have overlayed a direct-optimization scheme on top of a fully unconstrained…

Computational Physics · Physics 2015-05-13 A. Castro , E. Rasanen , A. Rubio , E. K. U. Gross

The time-dependent Schr\"odinger equation for atomic hydrogen in few-cycle laser pulses is solved numerically. Introducing a positive definite quantum distribution function in energy-position space, a straightforward comparison of the…

Atomic Physics · Physics 2009-11-11 D. Bauer

We study numerically stabilization against ionization of a fully correlated two-electron model atom in an intense laser pulse. We concentrate on two frequency regimes: very high frequency, where the photon energy exceeds both, the…

Atomic Physics · Physics 2009-10-31 D. Bauer , F. Ceccherini

We investigate the stabilization of a hydrogen atom in circularly polarized laser fields. We use a time-dependent, fully three dimensional approach to study the quantum dynamics of the hydrogen atom subject to high intensity, short…

Quantum Physics · Physics 2009-11-07 Dae-Il Choi , Will Chism

The frequency dependence of (nonsequential) double ionization is studied in fully quantum mechanical calculations using a (1+1)-dimensional model atom. Other time-dependent effects such as the influence of the number of field cycles are…

Quantum Physics · Physics 2025-11-10 Jan H. Thiede , Jakub S. Prauzner-Bechcicki

A nonlocal quantum model is presented for calculating the atomic dielectric response to a strong laser electric field. By replacing the Coulomb potential with a nonlocal potential in the Schrodinger equation, a 3+1D calculation of the…

Atomic Physics · Physics 2015-06-18 T. C. Rensink , T. M. Antonsen , J. P. Palastro , D. Gordon

In order to elucidate the correlated motion of atomic electrons, we investigate the attosecond-scale dynamics of their entanglement arising due to nonsequential ionization driven by a strong, linearly-polarized laser field. The calculation…

Atomic Physics · Physics 2024-03-18 Daniel Younis , Songbo Xie , Joseph H. Eberly

A new theoretical approach to the description of the attosecond streaking measurements of atomic photoionization is presented. It is a fully quantum mechanical description based on numerical solving of the time-dependent Schroedinger…

Atomic Physics · Physics 2007-05-23 A. K. Kazansky , N. M. Kabachnik

Using a three-dimensional quasiclassical technique we explore molecular double ionization by a linearly polarized, infrared (800~nm) 27~fs laser pulse. For intensities ranging from the tunneling to the over-the-barrier regime, we identify…

Atomic Physics · Physics 2011-01-27 A. Emmanouilidou , D. S. Tchitchekova

The influence of electron-electron Coulomb repulsion on nonsequential double ionization of rare-gas atoms is investigated. Several variants of the quantum-mechanical transition amplitude are evaluated that differ by the form of the…

Atomic Physics · Physics 2007-05-23 C. Figueira de Morisson Faria , X. Liu , H. Schomerus , W. Becker
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