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We formulate a general three-dimensional semiclassical model for the study of correlated multielectron escape during fragmentation of molecules driven by intense infrared laser pulses, while fully accounting for the magnetic field of the…

Atomic Physics · Physics 2023-11-30 Georgios Petros Katsoulis , Matthew Benjamin Peters , Agapi Emmanouilidou

We investigate the time-evolution of quantum entanglement between an electron, liberated by a strong few-cycle laser pulse, and its parent ion-core. Since the standard procedure is numerically prohibitive in this case, we propose a novel…

Quantum Physics · Physics 2017-10-18 Szilárd Majorosi , Mihály G. Benedict , Attila Czirják

We solve the three-dimensional time-dependent Schr\"{o}dinger equation for a few-cycle circularly polarized femtosecond laser pulse interacting with an oriented target exemplified by an Argon atom, initially in a $3\text{p}_{x}$ or…

Atomic Physics · Physics 2015-05-18 C. P. J. Martiny , M. Abu-samha , L. B. Madsen

We perform a systematic analysis of how nonsequential double ionization in intense, linearly polarized laser fields is influenced by the initial states in which both electrons are bound, and by the residual ionic potential. We assume that…

Atomic Physics · Physics 2009-11-10 C. Figueira de Morisson Faria , M. Lewenstein

Strong field processes in the non-relativistic regime are insensitive to the electron spin, i.e. the observables appear to be independent of this electron property. This does not have to be the case for several active electrons where Pauli…

We present an ab initio study of the nonsequential strong-field ionization dynamics of a model two-electron atom with helium character. Single- and double-ionization events are characterized and displayed using detector signals extracted at…

Atomic Physics · Physics 2023-06-14 Daniel Younis , Joseph H. Eberly

We investigate the laser-assisted single XUV photon double ionization of ground state helium. By solving full six-dimensional time-dependent schr{\"o}dinger equation, we study the correlation and angular distribution. The discussion in…

Atomic Physics · Physics 2020-03-24 Fengzheng Zhu , Genliang Li , Aihua Liu

A two-dimensional model atom is employed to study the ionization behavior of initially excited atomic states in highly-frequent intense laser pulses beyond the dipole approximation. An additional regime of ionization suppression is found at…

Atomic Physics · Physics 2009-11-11 Andreas Staudt , Christoph H. Keitel , John S. Briggs

A review of some recently developed methods of calculating multiple differential cross-sections of photoionization and electron impactionization of atoms and molecules having two active electrons is presented. The methods imply original…

We investigate two-photon double ionization of helium by intense ($10^{15} W/cm^2$) ultrashort ($\approx 300$ as) soft X-ray pulses (E = 91.6 eV). The time-dependent two-electron Schr\"odinger equation is solved using a coupled channel…

Atomic Physics · Physics 2007-05-23 I. F. Barna , J. Wang , J. Burgdoerfer

We investigate the photoionization dynamics of atoms subjected to intense, ultrashort laser pulses through the use of quantum trajectories. This method provides a unique and consistent framework for examining electron dynamics within a…

Atomic Physics · Physics 2024-08-01 Taylor Moon , Klaus Bartschat , Nicolas Douguet

Ionization and excitation of water molecules in intense laser pulses is studied theoretically by solving the three-dimensional time-dependent electronic Schr\"odinger equation within the single-active-electron approximation. The possibility…

Atomic Physics · Physics 2011-12-13 Simon Petretti , Alejandro Saenz , Alberto Castro , Piero Decleva

A model describing the electronic transitions in an atom subject to a strong high frequency laser pulse is proposed in the velocity gauge. The model accounts for the initial state coupling with the the remaining discrete and continuum…

Atomic Physics · Physics 2016-05-10 V. D. Rodríguez

The ionization of two-active-electron systems by intense laser fields is investigated theoretically. In comparison with time-dependent Hartree-Fock and exact two electron simulation, we show that the ionization rate is overestimated in SAE…

Atomic Physics · Physics 2015-06-18 Zengxiu Zhao , Jianmin Yuan

We study the effects of spin degrees of freedom and wave function symmetries on double ionization in three-electron systems. Each electron is assigned one spatial degree of freedom. The resulting three-dimensional Schr\"odinger equation is…

Joint electron-ion energy spectra for the dissociative ionization of a model H$_2^+$ in few-cycle, infrared laser pulses are calculated via the numerical ab initio solution of the time-dependent Schr\"odinger equation. A strong,…

Atomic Physics · Physics 2017-11-21 V. Mosert , D. Bauer

We discuss the final stages of the simultaneous ionization of two or more electrons due to a strong laser pulse. An analysis of the classical dynamics suggests that the dominant pathway for non-sequential escape has the electrons escaping…

Quantum Physics · Physics 2009-11-06 Bruno Eckhardt , Krzysztof Sacha

The ionization of H2 in intense laser pulses is studied by numerical integration of the time-dependent Schr\"odinger equation for a single-active-electron model including the vibrational motion. The electron kinetic-energy spectra in…

Atomic Physics · Physics 2009-11-13 Stefan Pieper , Manfred Lein

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

In this paper we discuss how through the process of applying the Fourier transform to solutions of the Schr\"odinger equation in the Close Coupling approach, good results for the ionization differential cross section in energy for electrons…

Atomic Physics · Physics 2016-01-25 A. Amaya-Tapia , A. Antillón