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We investigate electrostatic stability of charged droplets, modeled as permeable, charged spheres, and their encapsidation in thin, arbitrarily charged nano-shells, immersed in a neutralizing asymmetric electrolyte background. The latter…

Soft Condensed Matter · Physics 2013-11-15 Leili Javidpour , Anže Lošdorfer Božič , Ali Naji , Rudolf Podgornik

A monolayer of molecules or quantum dots sandwiched between electrodes can be driven out of equilibrium by the application of a bias voltage between the electrodes. We study charge ordering, i.e., the spontaneous formation of a charge…

Statistical Mechanics · Physics 2016-11-28 Tim Ludwig , Carsten Timm

Using the hypernetted-chain/mean spherical approximation (HNC/MSA) integral equations we study the electrical double layer inside and outside a model charged cylindrical vesicle (nanopore) immersed into a primitive model macroions solution,…

Mesoscale and Nanoscale Physics · Physics 2017-10-04 E. González-Tovar , M. Lozada-Cassou

The response of a suspension under a variety of static or alternating external fields strongly depends on the equilibrium electric double layer that surrounds the colloidal particles in the suspension. The theoretical models for salt-free…

Soft Condensed Matter · Physics 2022-02-11 Jun-Sik Sin , Kwang-Il Kim , Kuk-Chol Ri , Dok-Yong Ju , Nam-Hyok Kim , Chung-Sik Sin

Electrons and holes are locally injected in a single pentacene monolayer island. The two-dimensional distribution and concentration of the injected carriers are measured by electrical force microscopy. In crystalline monolayer islands, both…

Materials Science · Physics 2015-06-24 Thomas Heim , Kamal Lmimouni , Dominique Vuillaume

We investigated the complexation of thermoresponsive anionic poly(N-isopropylacrylamide) (PNiPAM) microgels and cationic $\epsilon$-polylysine ($\epsilon$-PLL) chains. By combining electrophoresis, light scattering, transmission electron…

We investigate numerically and on the scaling level the adsorption of a charged colloid on an oppositely charged flexible membrane. We show that the long ranged character of the electrostatic interaction leads to a wrapping reentrance of…

Biological Physics · Physics 2009-11-10 Christian C. Fleck , Roland R. Netz

Concentrated colloidal suspensions of nanorods often exhibit liquid-crystalline (LC) behavior. The transition to a nematic LC phase, with long-range orientational order of the particles, is usually well captured by Onsager's theory for hard…

Soft Condensed Matter · Physics 2023-10-13 Jeongmo Kim , Zijun Wang , Khalid Lahlil , Patrick Davidson , Thierry Gacoin , Jongwook Kim

We present a theory that enables us to calculate the effective surface charge of colloidal particles and to efficiently obtain titration curves for different salt concentrations. The theory accounts for the shift of pH of solution due to…

Soft Condensed Matter · Physics 2022-11-01 Amin Bakhshandeh , Derek Frydel , Yan Levin

We study the influence of airborne CO2 on the charge state of carboxylate stabilized polymer latex particles suspended in aqueous electrolytes. We combine conductometric experiments interpreted in terms of Hessinger's conductivity model…

Soft Condensed Matter · Physics 2024-11-19 Peter Vogel , David Beyer , Christian Holm , Thomas Palberg

A simple model was constructed to describe the polar ordering of non-centrosymmetric supramolecular aggregates formed by self assembling triblock rodcoil polymers. The aggregates are modeled as dipoles in a lattice with an Ising-like…

Soft Condensed Matter · Physics 2009-10-31 M. Sayar , F. J. Solis , M. Olvera de la Cruz , S. I. Stupp

The behavior of highly charged short rod-like polyelectrolytes near oppositely charged planar surfaces is investigated by means of Monte Carlo simulations. A detailed microstructural study, including monomer and fluid charge distribution,…

Soft Condensed Matter · Physics 2009-11-11 Rene Messina

Competing charge and spin orders are central to uncovering the nature of unconventional superconductivity. Here we utilize synchrotron X-ray diffraction on a high-quality single crystal to reveal the charge order of La$_3$Ni$_2$O$_7$ at…

Charged colloidal dispersions make up the basis of a broad range of industrial and commercial products, from paints to coatings and additives in cosmetics. During drying, an initially liquid dispersion of such particles is slowly…

Soft Condensed Matter · Physics 2019-01-07 Lucas Goehring , Joaquim Li , Pree-Cha Kiatkirakajorn

We report on the electrostatic complexation between polyelectrolyte-neutral copolymers and oppositely charged 6 nm-crystalline nanoparticles. For two different dispersions of oxide nanoparticles, the electrostatic complexation gives rise to…

Soft Condensed Matter · Physics 2007-09-10 J. -F. Berret , A. Sehgal , M. Morvan , O. Sandre , A. Vacher , M. Airiau

We investigate the complexation of a highly charged sphere with a long flexible polyelectrolyte, \textit{both negatively charged} in salt free environment. Electroneutrality is insured by the presence of divalent counterions. Using…

Soft Condensed Matter · Physics 2007-05-23 Rene Messina , Christian Holm , Kurt Kremer

This chapter deals with charged polymers (polyelectrolytes) in solution and at surfaces. The behavior of polyelectrolytes is markedly different from that of neutral polymers. In bulk solutions, i.e. disregarding the surface effect, there…

Soft Condensed Matter · Physics 2009-09-25 Roland R. Netz , David Andelman

We study a new type of 2D active material that exhibits macroscopic phases with two emergent broken symmetries: self-propelled achiral particles that form dense hexatic clusters, which spontaneously rotate. We experimentally realise active…

Equal volume mixtures of small and large polytetrafluorethylene (PTFE) spheres are shaken in an atmosphere of controlled humidity which allows to also control their tribo-charging. We find that the contact numbers are charge-dependent: as…

Soft Condensed Matter · Physics 2017-06-21 Andre Schella , Simon Weis , Matthias Schroeter

The issues of electronic polarizability in molecular dynamics simulations are discussed. We argue that the charges of ionized groups in proteins, and charges of ions in conventional non-polarizable force fields such as CHARMM, AMBER,…

Chemical Physics · Physics 2017-09-13 Igor Leontyev , Alexei Stuchebrukhov