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Thermodynamic experiments as well as Raman scattering have been used to study the magnetic instabilities in the spin-tetrahedra systems Cu_2Te_2O_5X_2, X=Cl and Br. While the phase transition observed in the Cl system at T_o=18.2 K is…

Strongly Correlated Electrons · Physics 2009-11-07 P. Lemmens , K. -Y. Choi , E. E. Kaul , Ch. Geibel , K. Becker , W. Brenig , R. Valenti , C. Gros , M. Johnsson , P. Millet , F. Mila

We present a theory of spin and orbital states in Mott insulator $LaTiO_3$. The spin-orbital superexchange interaction between $d^1(t_{2g})$ ions in cubic crystal suffers from a pathological degeneracy of orbital states at classical level.…

Strongly Correlated Electrons · Physics 2009-10-31 G. Khaliullin , S. Maekawa

The pyrochlore compound \tbti\ is known to remain in a spin-liquid state down to the lowest attainable temperature (0.05\,K), whereas current theories predict it should order into an antiferromagnetic structure. A number of models have been…

Strongly Correlated Electrons · Physics 2011-04-11 P. Bonville , I. Mirebeau , A. Gukasov , S. Petit , J. Robert

The charge ordered structure of ions and vacancies characterizing rare-earth pyrochlore oxides serves as a model for the study of geometrically frustrated magnetism. The organization of magnetic ions into networks of corner-sharing…

PbCuTe2O6 is a rare example of a spin liquid candidate featuring a three dimensional magnetic lattice. Strong geometric frustration arises from the dominant antiferromagnetic interaction which generates a hyperkagome network of Cu2+ ions…

Strongly Correlated Electrons · Physics 2016-03-14 P. Khuntia , F. Bert , P. Mendels , B. Koteswararao , A. V. Mahajan , M. Baenitz , F. C. Chou , C. Baines , A. Amato , Y. Furukawa

On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

Gapped Z_2 spin liquids have been proposed as candidates for the ground-state of the S=1/2 quantum antiferromagnet on the Kagome lattice. We extend the use of Projected Entangled Pair States to construct (on the cylinder)Resonating Valence…

Strongly Correlated Electrons · Physics 2013-05-14 Didier Poilblanc , Norbert Schuch

We have studied the spin correlations with $\bf{k}$= ($\frac12$, $\frac12$, $\frac12$) propagation vector which appear below 0.4\, K in \tbti\ spin liquid by combining powder neutron diffraction and specific heat on…

Strongly Correlated Electrons · Physics 2015-10-28 S. Guitteny , I. Mirebeau , P. Dalmas de Réotier , C. Colin , P. Bonville , F. Porcher , B. Grenier , C. Decorse , S. Petit

Spiral spin liquids are unique classical spin liquids that occur in many frustrated spin systems, but do not comprise a new phase of matter. Owing to extensive classical ground-state degeneracy, the spins in a spiral spin liquid thermally…

Strongly Correlated Electrons · Physics 2021-06-01 Xu-Ping Yao , Jian Qiao Liu , Chun-Jiong Huang , Xiaoqun Wang , Gang Chen

Recent experiments on the organic compound \kappa-(ET)_2Cu_2(CN)_3 have provided a promising example of a two dimensional spin liquid state. This phase is described by a two-dimensional spinon Fermi sea coupled to a U(1) gauge field. We…

Strongly Correlated Electrons · Physics 2009-11-13 Victor Galitski , Yong Baek Kim

Stabilizing exotic quantum phases of matter, e.g. spin liquid, is an attractive topic in condensed matter. Here, by a Monte Carlo study of a two-orbital spin-fermion model on a honeycomb lattice, we show the cooperative effects of the…

Strongly Correlated Electrons · Physics 2025-01-13 Kaidi Xu , Shan-Shan Wang , Rong Yu , Shuai Dong

The origin of quantum fluctuations responsible for the spin liquid state in Tb$_2$Ti$_2$O$_7$ has remained a long standing problem. By synchrotron-based terahertz measurements, we show evidence of strong coupling between the magnetic and…

Materials Science · Physics 2017-02-17 E. Constable , R. Ballou , J. Robert , C. Decorse , J. -B. Brubach , P. Roy , E. Lhotel , L. Del-Rey , V. Simonet , S. Petit , S. deBrion

The Dirac spin liquid ground state of the spin 1/2 Heisenberg kagome antiferromagnet has potential instabilities[1-4]. This has been suggested as the reason why it is not strongly supported in large-scale numerical calculations[5]. However,…

Strongly Correlated Electrons · Physics 2013-11-13 Bryan Clark , Jesse Kinder , Eric Neuscamman , Garnet Kin-Lic Chan , Michael J. Lawler

Spin liquid ground states are predicted to arise within several distinct scenarios in condensed matter physics. The observation of these disordered magnetic states is particularly pervasive amongst a class of materials known as frustrated…

We report neutron scattering studies of the spin correlations of the geometrically frustrated pyrochlore Tb2Mo2O7 using single crystal samples. This material undergoes a spin-freezing transition below Tg~24 K, similar to Y2Mo2O7, and has…

Strongly Correlated Electrons · Physics 2009-11-13 D. K. Singh , J. S. Helton , S. Chu , T. H. Han , C. J. Bonnoit , S. Chang , H. J. Kang , J. W. Lynn , Y. S. Lee

With electron filling $n=1$ in the $\rm Sr_2VO_4$ compound, the octahedrally coordinated $t_{\rm 2g}$ orbitals are strongly active due to tetragonal distortion induced crystal field tuning by external agent such as pressure. Considering the…

Strongly Correlated Electrons · Physics 2022-02-25 Shubhajyoti Mohapatra , Dheeraj Kumar Singh , Rajyavardhan Ray , Sayandip Ghosh , Avinash Singh

At low temperatures, Tb$_2$Ti$_2$O$_7$ enters a spin liquid state, despite expectations of magnetic order and/or a structural distortion. Using neutron scattering, we have discovered that in this spin liquid state an excited crystal field…

Strongly Correlated Electrons · Physics 2014-01-16 T. Fennell , M. Kenzelmann , B. Roessli , H. Mutka , J. Ollivier , M. Ruminy , U. Stuhr , O. Zaharko , L. Bovo , A. Cervellino , M. K. Haas , R. J. Cava

Spin liquids represent exotic types of quantum matter that evade conventional symmetry-breaking order even at zero temperature. Exhaustive classifications of spin liquids have been carried out in several systems, particularly in the…

Strongly Correlated Electrons · Physics 2014-11-19 Johannes Reuther , Shu-Ping Lee , Jason Alicea

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

Strongly Correlated Electrons · Physics 2013-07-19 Tian-Heng Han , Joel S. Helton , Shaoyan Chu , Daniel G. Nocera , Jose A. Rodriguez-Rivera , Collin Broholm , Young S. Lee

Ho2Ti2O7 and Dy2Ti2O7 spin ices exhibit elementary excitations akin to magnetic monopoles. Here we focus on Tb2Ti2O7 spin liquid, where correlated magnetic moments keep fluctuating down to very low temperatures. Using a monopole picture, we…

Strongly Correlated Electrons · Physics 2015-06-05 A. P. Sazonov , A. Gukasov , I. Mirebeau , P. Bonville