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We study the carrier dynamics in epitaxially grown graphene in the range of photon energies from 10 - 250 meV. The experiments complemented by microscopic modeling reveal that the carrier relaxation is significantly slowed down as the…

The ultrafast relaxation and recombination dynamics of photogenerated electrons and holes in epitaxial graphene are studied using optical-pump Terahertz-probe spectroscopy. The conductivity in graphene at Terahertz frequencies depends on…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Paul A. George , Jared Strait , Jahan Dawlaty , Shriram Shivaraman , Mvs Chandrashekhar , Farhan Rana , Michael G. Spencer

Nonlinear optical properties and carrier relaxation dynamics in graphene, suspended in three different solvents, are investigated using femtosecond (80 fs pulses) Z-scan and degenerate pumpprobe spectroscopy at 790 nm. The results…

Materials Science · Physics 2015-05-14 Sunil Kumar , M. Anija , N. Kamaraju , K. S. Vasu , K. S. Subrahmanyam , A. K. Sood , C. N. R. Rao

We perform a femtosecond-THz optical pump-probe spectroscopy to investigate the cooling dynamics of hot carriers in quasi-free standing bilayer epitaxial graphene. We observed longer decay time constants, in the range of 2.6 to 6.4 ps,…

Mesoscale and Nanoscale Physics · Physics 2023-02-03 Sachin Sharma , Rachael L. Myers-Ward , David Kurt Gaskill , Ioannis Chatzakis

We report an optical study of charge transport in graphene. Diffusion of hot carriers in epitaxial graphene and reduced graphene oxide samples are studied using an ultrafast pump-probe technique with a high spatial resolution.…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 Brian A. Ruzicka , Shuai Wang , Lalani K. Werake , Ben Weintrub , Kian Ping Loh , Hui Zhao

Using ultrafast optical pump-probe spectroscopy, we study the relaxation dynamics of hot optical phonons in few-layer and multi-layer graphene films grown by epitaxy on silicon carbide substrates and by chemical vapor deposition on nickel…

A degenerate pump--probe technique is used to investigate the non equilibrium carrier dynamics in multi--layer graphene. Two distinctly different dynamics of the carrier relaxation are observed. A fast relaxation ($\sim 50$ fs) of the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 P. Plochocka , P. Kossacki , A. Golnik , T. Kazimierczuk , C. Berger , W. A. de Heer , M. Potemski

Using optical-pump terahertz-probe spectroscopy, we study the relaxation dynamics of photoexcited carriers in graphene at different temperatures. We find that at lower temperatures the tail of the relaxation transients as measured by the…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Jared H. Strait , Haining Wang , Shriram Shivaraman , Virgil B. Shields , Michael G. Spencer , Farhan Rana

Understanding the ultrafast carrier dynamics of graphene on a substrate is a fundamental step in the development of graphene based opto-electronic devices. Here, we present ultrafast pump-probe measurements of supported graphene on quartz…

Mesoscale and Nanoscale Physics · Physics 2021-02-16 Rustam Gatamov , Andrey Baydin , Halina Krzyzanowska , Norman Tolk

Femtosecond time-resolved spectroscopy using 400 nm-pump and 800 nm-probe in CVD-grown multilayer graphene provides strong evidence for isotropic distribution of photoexcited carrier after initial relaxation. Indicative of such isotropic…

Mesoscale and Nanoscale Physics · Physics 2013-12-24 Xiao-Qing Yan , Zhi-Bo Liu , Jun Yao , Xin Zhao , Xu-Dong Chen , Yongsheng Chen , Jian-Guo Tian

In order to exploit the intriguing optical properties of graphene it is essential to gain a better understanding of the light-matter interaction in the material on ultrashort timescales. Exciting the Dirac fermions with intense ultrafast…

The energy relaxation of carriers in reduced graphene oxide thin films is studied using optical pump-probe spectroscopy with two probes of different colors. We measure the time difference between peaks of the carrier density at each probing…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Brian A. Ruzicka , Nardeep Kumar , Shuai Wang , Kian Ping Loh , Hui Zhao

We report ultrafast response of femtosecond photoexcited carriers in single layer reduced graphene oxide flakes suspended in water as well as few layer thick film deposited on indium tin oxide coated glass plate using pump-probe…

Materials Science · Physics 2011-06-30 Sunil Kumar , N. Kamaraju , K. S. Vasu , A. K. Sood

For most optoelectronic applications of graphene a thorough understanding of the processes that govern energy relaxation of photoexcited carriers is essential. The ultrafast energy relaxation in graphene occurs through two competing…

We study the broadband optical conductivity and ultrafast carrier dynamics of epitaxial graphene in the few-layer limit. Equilibrium spectra of nominally buffer, monolayer, and multilayer graphene exhibit significant terahertz and…

Materials Science · Physics 2009-05-02 H. Choi , F. Borondics , D. A. Siegel , S. Y. Zhou , M. C. Martin , A. Lanzara , R. A. Kaindl

Recent pump-probe experiments performed on graphene in a perpendicular magnetic field have revealed carrier relaxation times ranging from picoseconds to nanoseconds depending on the quality of the sample. To explain this surprising…

We report on spectroscopy results from the mid- to far-infrared on wafer-scale graphene, grown either epitaxially on silicon carbide, or by chemical vapor deposition. The free carrier absorption (Drude peak) is simultaneously obtained with…

Mesoscale and Nanoscale Physics · Physics 2011-11-17 Hugen Yan , Fengnian Xia , Wenjuan Zhu , Marcus Freitag , Christos Dimitrakopoulos , Ageeth A. Bol , George Tulevski , Phaedon Avouris

The dynamics of photocarriers in reduced graphene oxide thin films is studied by using ultrafast pump-probe spectroscopy. Time dependent differential transmissions are measured with sample temperatures ranging from 9 to 300 K. At each…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Brian A. Ruzicka , Lalani K. Werake , Hui Zhao , Shuai Wang , Kian Ping Loh

Room temperature, wavelength non-degenerate ultrafast pump/probe measurements were performed on GaN and InGaN epilayers and an InGaN multiple quantum well structure. Carrier relaxation dynamics were investigated as a function of excitation…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Umit Ozgur , Henry O. Everitt

Since graphene has no band gap, photoluminescence is not expected from relaxed charge carriers. We have, however, observed significant light emission from graphene under excitation by ultrashort (30-fs) laser pulses. Light emission was…

Mesoscale and Nanoscale Physics · Physics 2010-09-20 Chun Hung Lui , Kin Fai Mak , Jie Shan , Tony F. Heinz
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