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In this chapter, a study of the glass transitions in colloidal systems is presented, in connection with gelation, mainly from theoretical and simulation results. Mode Coupling Theory, which anticipated the existence of attraction driven…

Soft Condensed Matter · Physics 2008-10-06 Antonio M. Puertas , Matthias Fuchs

We propose a computational strategy to quantify the temperature evolution of the timescales and lengthscales over which dynamic facilitation affects the relaxation dynamics of glass-forming liquids at low temperatures, that requires no…

Soft Condensed Matter · Physics 2024-06-25 Cecilia Herrero , Ludovic Berthier

Vapour deposition can directly produce ultrastable glasses, which are similar to conventional glasses aged over thousands of years. The highly mobile surface layer is believed to accelerate the ageing process of vapour-deposited glasses,…

Soft Condensed Matter · Physics 2016-10-20 Xin Cao , Huijun Zhang , Yilong Han

We investigate the heterogeneous dynamics in a model, where chemical gelation and glass transition interplay, focusing on the dynamical susceptibility. Two independent mechanisms give raise to the correlations, which are manifested in the…

Soft Condensed Matter · Physics 2017-05-09 Antonio de Candia , Annalisa Fierro , Raffaele Pastore , Massimo Pica Ciamarra , Antonio Coniglio

Recent progresses in the description of glassy relaxation and ageing are reviewed for the wide class of network-forming materials such as $GeO_2$, Ge$_x$Se$_{1-x}$, silicates (SiO$_2$-Na$_2$O) or borates (B$_2$O$_3$-Li$_2$O), all of them…

Disordered Systems and Neural Networks · Physics 2016-06-09 M. Micoulaut

The Gilroy-Phillips model of relaxational jumps in asymmetric double-well potentials, developed for the Arrhenius-type secondary relaxations of the glass phase, is extended to a formal description of the breakdown of the shear modulus at…

Disordered Systems and Neural Networks · Physics 2007-05-23 U. Buchenau

Relaxation processes significantly influence the properties of glass materials. However, understanding their specific origins is difficult, even more challenging is to forecast them theoretically. In this study, using microseconds molecular…

Materials Science · Physics 2019-09-09 Yang Sun , Si-Xu Peng , Qun Yang , Feng Zhang , Meng-Hao Yang , Cai-Zhuang Wang , Kai-Ming Ho , Hai-Bin Yu

We present a detailed analysis of the beta-relaxation dynamics of a simple glass former, a Lennard-Jones system with a stochastic dynamics. By testing the various predictions of mode-coupling theory, including the recently proposed…

Statistical Mechanics · Physics 2015-06-25 Tobias Gleim , Walter Kob

There is mounting evidence indicating that relaxation dynamics in liquids approaching their glass transition not only becomes increasingly cooperative (1,2) but the relaxing regions also become more compact in shape(3-7). While the surface…

Statistical Mechanics · Physics 2018-02-21 Divya Ganapathi , Hima K Nagamanasa , A. K. Sood , Rajesh Ganapathy

The dynamics of dislocations is reported to exhibit glassy properties. We study numerically various versions of 2d edge dislocation systems in the absence of externally applied stress. Two types of glassy behavior are identified: (i)…

Disordered Systems and Neural Networks · Physics 2009-11-13 B. Bako , I. Groma , G. Gyorgyi , G. T. Zimanyi

Two-atom systems in small traps are of fundamental interest, first of all for understanding the role of interactions in degenerate cold gases and for the creation of quantum gates in quantum information processing with single-atom traps.…

Molecular dynamics simulations are performed to investigate heterogeneous dynamics in amorphous glassy materials under oscillatory shear strain. We consider three-dimensional binary Lennard-Jones mixture well below the glass transition…

Soft Condensed Matter · Physics 2013-05-10 Nikolai V. Priezjev

We show that the dynamics of a laser driven Rydberg gas in the limit of strong dephasing is described by a master equation with manifest kinetic constraints. The equilibrium state of the system is uncorrelated but the constraints in the…

Atomic Physics · Physics 2015-06-16 Igor Lesanovsky , Juan P. Garrahan

Understanding surface mechanics of soft solids, such as soft polymeric gels, is crucial in many engineering processes, such as dynamic wetting and adhesive failure. In these situations, a combination of capillary and elastic forces drives…

Soft Condensed Matter · Physics 2020-12-02 Qin Xu , Lawrence A. Wilen , Katharine E. Jensen , Robert W. Style , Eric R. Dufresne

We derive an equation for the glass relaxation. In the derivation, the Zwanzig-Mori projection method is not applied explicitly, which makes our equation different from the mode coupling theory. Due to the nonlinearity, it is difficult to…

Disordered Systems and Neural Networks · Physics 2023-02-17 Li Wan

The relaxation dynamics and the vibrational spectra of amorphous solids, such as metal alloys, have been intensely investigated as well separated topics in the past. The aim of this review is to summarize recent results in both these areas…

Materials Science · Physics 2020-03-17 Alessio Zaccone

Studying the primary {\alpha}- and secondary {\beta}-relaxation process has contributed significantly to the understanding of the structure and rheology of metallic glasses. In this letter, we report on a third relaxation mechanism…

Materials Science · Physics 2017-03-28 Stefan Küchemann , Robert Maaß

We use computer simulations to study the dynamics of a physical gel at high densities where gelation and the glass transition interfere. We report and provide detailed physical understanding of complex relaxation patterns for time…

Soft Condensed Matter · Physics 2010-05-07 Pinaki Chaudhuri , Ludovic Berthier , Pablo I. Hurtado , Walter Kob

Low-energy excitations play a key role in all condensed-matter systems, yet there is limited understanding of their nature in glasses, where they correspond to local rearrangements of groups of particles. Here we introduce an algorithm to…

Soft Condensed Matter · Physics 2024-08-27 Wencheng Ji , Massimo Pica Ciamarra , Matthieu Wyart

We provide a theoretical perspective on the glass transition in molecular liquids at thermal equilibrium, on the spatially heterogeneous and aging dynamics of disordered materials, and on the rheology of soft glassy materials. We start with…

Statistical Mechanics · Physics 2011-06-22 Ludovic Berthier , Giulio Biroli