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We report the first theoretical study of hydroxyl vacancies in aluminosilicate and aluminogermanate single-walled metal-oxide nanotubes. The defects are modeled on both sides of the tube walls and lead to occupied and empty states in the…

Materials Science · Physics 2009-11-13 G. Teobaldi , N. S. Beglitis , A. J. Fisher , F. Zerbetto , W. A. Hofer

We investigate the electronic properties of semi-metallic (12,0) carbon nanotubes in the presence of a variety of mono-, di- and hexa-vacancy defects, by using first principle DFT combined with non-equilibrium Green's function technique. We…

Mesoscale and Nanoscale Physics · Physics 2009-10-08 Hui Zeng , Huifang Hu , Jean-Pierre Leburton

The properties of single-walled carbon nanotubes (SWCNTs) and graphene can be modified by the presence of covalently bound impurities. Although this can be achieved by introducing chemical additives during synthesis, that often hinders…

The stability and properties of the monovacancy and the divacancy in single-walled carbon nanotubes (CNTs) are addressed by spin-density functional calculations. We study these defects in four nanotubes, the armchair (6,6) and (8,8) and the…

Materials Science · Physics 2009-11-11 W. Orellana , P. Fuentealba

We present a theoretical study of degeneracy breaking due to short-ranged impurities in finite, single-wall, metallic carbon nanotubes. The effective mass model is used to describe the slowly varying spatial envelope wavefunctions of…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Edward McCann , Vladimir I. Fal'ko

We calculated the effects of structural distortions on the electronic structure of carbon nanotubes. The key modification of the electronic structure brought about by bending a nanotube involves an increased mixing of $\sigma$ and…

Materials Science · Physics 2019-08-17 Alain Rochefort , Dennis R. Salahub , Phaedon Avouris

We report the first observation of substitutional silicon atoms in single-layer hexagonal boron nitride (h-BN) using aberration corrected scanning transmission electron microscopy (STEM). The medium angle annular dark field (MAADF) images…

Materials Science · Physics 2020-01-29 Mohammad Reza Ahmadpour Monazam , Ursula Ludacka , Hannu-Pekka Komsa , Jani Kotakoski

We investigate the nitrogen substitutional impurity in semiconducting zigzag and metallic armchair single-wall carbon nanotubes using ab initio density functional theory. At low concentrations (less than 1 atomic %), the defect state in a…

Materials Science · Physics 2007-05-23 Andriy H. Nevidomskyy , Gábor Csányi , Michael C. Payne

Angular perturbations modify the band structure of armchair (and other metallic) carbon nanotubes by breaking the tube symmetry and may induce a metal-semiconductor transition when certain selection rules are satisfied. The symmetry…

Mesoscale and Nanoscale Physics · Physics 2021-07-02 Yan Li , Slava V. Rotkin , Umberto Ravaioli

In carbon nanotubes, the most abundant defects, caused for example by irradiation or chemisorption treatments, are small perturbing clusters, i.e. bi-site defects, extending over both A and B sites. The relative positions of these…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 M. J. Hashemi , K. Sääskilahti , M. J. Puska

By means of pseudopotential calculations based on density functional theory (DFT) we studied the effect of hydrogenation on electronic properties of armchair single-wall carbon nanotubes. The calculations demonstrate strong preference for…

Materials Science · Physics 2015-05-30 Željko Šljivančanin

The band gap of a semiconducting single wall carbon nanotube decreases and eventually vanishes leading to metalization as a result of increasing radial deformation. This sets in a band offset between the undeformed and deformed regions of a…

Materials Science · Physics 2009-10-31 C. Kilic , S. Ciraci , O. Gulseren , T. Yildirim

The nanostructure of hydrogenated amorphous silicon (a Si:H) is studied by a combination of small-angle X-ray (SAXS) and neutron scattering (SANS) with a spatial resolution of 0.8 nm. The a-Si:H materials were deposited using a range of…

Materials Science · Physics 2020-11-04 Eike Gericke , Jimmy Melskens , Robert Wendt , Markus Wollgarten , Armin Hoell , Klaus Lips

Unusual physical properties of single-wall carbon nanotubes have started a search for similar tubular structures of other elements. In this paper, we present a theoretical analysis of single-wall nanotubes of silicon and group III-V…

Materials Science · Physics 2009-11-11 E. Durgun , S. Tongay , S. Ciraci

The electronic structure of nanocylinder without and with a small perturbation is investigated with the help of calculation of the local density of states. A continuum gauge field-theory model is used for this purpose. In this model, Dirac…

Materials Science · Physics 2014-12-23 R. Pincak , J. Smotlacha , M. Pudlak

Semiconducting single-walled carbon nanotubes show extraordinary electronic and optical properties, such as high charge carrier mobilities and diameter-dependent near-infrared photoluminescence. The introduction of sp3 defects in the carbon…

Optics · Physics 2021-11-10 Jana Zaumseil

Helical method of tube formation for band structure calculations and Hartree-Fock self-consistent field method (HF-SCF) modified for periodic solids have been applied in study of electronic properties of single-wall silicon nanotubes…

Mesoscale and Nanoscale Physics · Physics 2016-01-06 Pavol Banacky , Jozef Noga , Vojtech Szocs

We show that the electronic and atomic structure of carbon nanotubes undergo dramatic changes with hydrogen chemisorption from first principle calculations. Upon uniform exohydrogenation at half coverage, the cross sections of zigzag…

Materials Science · Physics 2016-08-16 O. Gülseren , T. Yildirim , S. Ciraci

The bonding properties of tilt boundary in poly-silicon and the effect of interstitial impurities are investigated by first-principles. In order to obtain thorough information on the nature of chemical bondings in these solid systems, an…

Materials Science · Physics 2022-05-31 Rita Maji , Eleonora Luppi , Elena Degoli , Julia Contreras-García

The synthesis of one-dimensional van der Waals heterostructures was realized recently, which opens up new possibilities for prospective applications in electronics and optoelectronics. The even reduced dimension will enable novel properties…

Mesoscale and Nanoscale Physics · Physics 2026-02-06 Ya Feng , Henan Li , Taiki Inoue , Shohei Chiashi , Slava V. Rotkin , Rong Xiang , Shigeo Maruyama
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