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We propose a theoretical approach based on (constrained) density functional theory and the Franck-Condon approximation for the calculation of the temperature dependent photoluminescence of nanostructures. The method is computationally…

Mesoscale and Nanoscale Physics · Physics 2023-11-20 Peng Han , Gabriel Bester

We report experimental measurements of electronic Raman scattering under resonant conditions by electrons in individual single-walled carbon nanotubes (SWNTs). The inelastic Raman scattering at low frequency range reveals a single particle…

Mesoscale and Nanoscale Physics · Physics 2014-05-12 Xi Chen , Bairen Zhu , Anmin Zhang , Hualing Zeng , Qingming Zhang , Xiaodong Cui

We experimentally demonstrate laser-driven deposition of single-walled carbon nanotubes (CNTs) in suspended core fibers (SCFs) for the first time. Two samples for each SCF type with three (SCF1) and four (SCF2) air holes are individually…

Significant understanding has been achieved over the last few decades regarding chirality-dependent properties of single-wall carbon nanotubes (SWCNTs), primarily through single-tube studies. However, macroscopic manifestations of chirality…

A fabrication method for positioning and embedding a single-walled carbon nanotube (SWNT) across the diameter of a solid state nanopore is presented. Chemical vapor deposition (CVD) is used to grow SWNTs over arrays of focused ion beam…

Biological Physics · Physics 2013-08-07 E. S. Sadki , S. Garaj , D. Vlassarev , J. A. Golovchenko , D. Branton

We study 23 to 30 nm long suspended single-wall carbon nanotube quantum dots and observe both their stretching and bending vibrational modes. We use low-temperature DC electron transport to excite and measure the tubes' bending mode by…

Mesoscale and Nanoscale Physics · Physics 2012-09-21 J. O. Island , V. Tayari , A. C. McRae , A. R. Champagne

The strain energies in straight and bent single-walled carbon nanotubes (SWNTs) are calculated by taking account of the total energy of all the occupied band electrons. The obtained results are in good agreement with previous theoretical…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 Zhou Xin , Zhou Jianjun , Ou-Yang Zhong-can

Bandstructure effects in PMOS transport of strongly quantized silicon nanowire field-effect-transistors (FET) in various transport orientations are examined. A 20-band sp3d5s* spin-orbit-coupled (SO) atomistic tight-binding model coupled to…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Neophytos Neophytou , Abhijeet Paul , Gerhard Klimeck

We report on microwave operation of top-gated single carbon nanotube transistors. From transmission measurements in the 0.1-1.6 GHz range, we deduce device transconductance gm and gate-nanotube capacitance Cg of micro- and nanometric…

We introduce the concept of optical control of the fluorescence yield of CdSe quantum dots through plasmon-induced structural changes in random semicontinuous nanostructured gold films. We demonstrate that the wavelength- and polarization…

A freestanding film of vertically aligned single-walled carbon nanotubes (VA-SWNTs) synthesized by the alcohol catalytic chemical vapor deposition (ACCVD) method was observed directly by transmission electron microscopy (TEM). These…

Single-wall carbon nanotubes (SWNTs) are best known in their hollow cylindrical shapes, but the ground state of large-diameter tubes actually corresponds to a collapsed dumbbell-like structure, where the opposite sides of the nanotube wall…

Mesoscale and Nanoscale Physics · Physics 2019-12-20 Rafael R. Del Grande , Alexandre F. da Fonseca , Rodrigo B. Capaz

Fluctuations in the fluorescence from macroscopic ensembles of colloidal semiconductor quantum dots have the spectral form of 1/f noise. The measured power spectral density reflects the fluorescence intermittency of individual dots with…

Materials Science · Physics 2009-11-10 Matthew Pelton , David Grier , Philippe Guyot-Sionnest

Semiconducting nanoparticles are the building blocks of optical nanodevices as their electronic states, and therefore light absorption and emission, can be controlled by modifying their size and shape. CdSe is perhaps the most studied of…

Materials Science · Physics 2015-06-25 Silvana Botti , Miguel A. L. Marques

Their outstanding electrical and optical properties make semiconducting single-walled carbon nanotubes (SWCNTs) highly suitable for charge transport and emissive layers in near-infrared optoelectronic devices. However, the luminescence…

The intrinsic near-infrared photoluminescence observed in long single walled carbon nanotubes is systematically quenched in ultrashort single-walled carbon nanotubes (usCNTs, below 100 nm length) due to their short dimension as compared to…

The thermal properties of single-walled carbon nanotubes (SWNTs) are of significant interest, yet their dependence on SWNT chirality has been, until now, not explored experimentally. Here we used electrical heating and infrared thermal…

Materials Science · Physics 2016-03-23 Feifei Lian , Juan P. Llinas , Zuanyi Li , David Estrada , Eric Pop

It was investigated the possibility of creating NbN superconducting single-photon detectors with saturated dependence of quantum efficiency versus normalized bias current. It was shown that the saturation increases for the detectors based…

Instrumentation and Detectors · Physics 2018-01-16 Konstantin Smirnov , Alexander Divochiy , Yury Vakhtomin , Pavel Morozov , Philipp Zolotov , Andrey Antipov , Vitaliy Seleznev

Electronic structure properties of nanowires (NW) with diameters of 1.5 nm and 3 nm based on semimetallic $\alpha$-Sn are investigated by employing density functional theory and perturbative $GW$ methods. We explore the dependence of…

Materials Science · Physics 2017-01-04 Alfonso Sanchez-Soares , Conor O'Donnell , James C. Greer

The importance of finite-size effects for the electronic structure of long zigzag and armchair carbon nanotubes is studied. We analyze the electronic structure of capped (6,6), (8,0), and (9,0) single walled carbon nanotubes as a function…

Chemical Physics · Physics 2007-05-23 Oded Hod , Juan E. Peralta , Gustavo E. Scuseria